Flexible organic transistors on standard printing paper...
Transcript of Flexible organic transistors on standard printing paper...
Flexible organic transistors on standard printing paper and
memory properties induced by floated gate electrode
By: Peng, BY (Peng, Boyu)[ 1 ] ; Chan, PKL (Chan, Paddy K. L.)[ 1 ]
ORGANIC ELECTRONICS
Volume: 15 Issue: 1 Pages: 203-210
DOI: 10.1016/j.orgel.2013.11.006
Published: JAN 2014
View Journal Information
Abstract
Integrating electronic devices with unconventional substrate has been a popular research direction.
Among these substrates, cellulose fiber paper has advantages in low-cost, recyclable and
bio-degradable. We demonstrated directing printing of all contact electrodes on standard untreated Fuji
Xerox printer paper without using planarization layer. The screen-printed gate electrodes based on silver
nanoparticles can smooth out the paper substrate surface by two orders of magnitude and allow us to
use parylene and DNTT as the dielectric and active layer directly. The transistors show average mobility
of 0.297 cm(2) V-1 s(-1) and on/off ratio larger than 10(5). The low leakage current allows us to
demonstrate memory properties by employing the floated gate method. The devices show excellent
memory retention time for more than 10,000 s. The unique flexibility and combustibility of the organic
transistors on paper substrate manifest their applications as next generation of green electronics. (C)
2013 Elsevier B.V. All rights reserved.
Keywords
Author Keywords: Screen-printing; Cellulose fiber paper; Memory; Floated gate
KeyWords Plus: SELF-ASSEMBLED MONOLAYERS; PERFORMANCE; PENTACENE;
HYDROPHILICITY; SEMICONDUCTORS; DIELECTRICS; HYDROLYSIS; ROUGHNESS; CIRCUITS;
LAYER
Author Information
Reprint Address: Chan, PKL (reprint author)
Univ Hong Kong, Dept Mech Engn, Pokfulam Rd, Hong Kong, Hong Kong, Peoples R China.
Addresses:
[ 1 ] Univ Hong Kong, Dept Mech Engn, Hong Kong, Hong Kong, Peoples R China
E-mail Addresses: [email protected]
Funding
Funding Agency Grant Number
University of Hong Kong 201209160033
201210159031
View funding text
Publisher
ELSEVIER SCIENCE BV, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
Categories / Classification
Research Areas: Materials Science; Physics
Web of Science Categories: Materials Science, Multidisciplinary; Physics, Applied
Document Information
Document Type: Article
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Most Recent Citation
Peng, Boyu. High performance organictransistor active-matrix driverdeveloped on paper substrate.SCIENTIFIC REPORTS, SEP 19 2014.
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Language: English
Accession Number: WOS:000328855800030
ISSN: 1566-1199
eISSN: 1878-5530
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Table of Contents: Current Contents Connect ®
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IDS Number: 277YS
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Relationship of Surface Hydrophilicity, Charge, and Roughness
of PET Foils Stimulated by Incipient Alkaline Hydrolysis
By: Skvarla, J (Skvarla, Jiri)[ 1 ] ; Luxbacher, T (Luxbacher, Thomas); Nagy, M (Nagy, Martin)[ 1 ] ; Sisol,
M (Sisol, Martin)[ 1 ]
ACS APPLIED MATERIALS & INTERFACES
Volume: 2 Issue: 7 Pages: 2116-2127
DOI: 10.1021/am100368v
Published: JUL 2010
View Journal Information
Abstract
An enhancement of wettability of PET foils pretreated hydrolytically by immersing in mild alkaline (NaOH)
solutions has been documented by a descending sigmoidal dependence between the interfacial free
energy gamma(SL) of the PET/water interface and the concentration of NaOH solution c(NaOH). An
increase in temperature of the NaOH solution below the glass-transition temperature of PET further
promotes the hydrophilicity, resulting in a proportional shift of the gamma(SL) VS c(NaOH) dependence.
The limiting hydrophilicity of PET is thermodynamically predicted to occur at gamma(SL) -> 0,
corresponding to the advancing water contact angle theta(a) approximate to 50 degrees (for 6% NaOH
and 60 degrees C). The surface roughness due to the partial hydrolytic degradation as well as the weight
loss (dissolution) of PET are found to reach a maximum value just when the latter dependence goes
through its inflection. Assuming a general parallelism between the interfacial free energy and the
dissolution kinetics, we propose the hydrolytically stimulated formation and growth of pits on the PET
surface to cause the initial acceleration as well as subsequent retardation of dissolution as c(NaOH),
increases, leading to the S-shaped gamma(SL) VS c(NaOH) dependence with the inflection for a specific
c(NaOH). Moreover, the zeta potential measured by the streaming current method also attains a
maximum at the same specific concentration of NaOH. It would indicate that the largest amount of
electric charges is populated via polar carboxyl and hydroxyl groups created by chemical scissions of
PET polymer chains when a change in the dissolution rate increases to the utmost. In such a way, partial
hydrolysis restricted to the uppermost part of moderately hydrophobic surface of solid PET allowed us to
better understand the intermingled role of thermodynamic and physical aspects in surface wettability
itself:
Keywords
Author Keywords: PET; hydrolysis; wettability; surface roughness; interfacial free energy; contact
angle; alkaline degradation; dissolution
KeyWords Plus: SPUN POLY(ETHYLENE-TEREPHTHALATE) FIBERS; MOISTURE-RELATED
PROPERTIES; FROTH FLOTATION; POLYVINYL-CHLORIDE; POLYMER SURFACES; CONTACT
ANGLES; FREE-ENERGY; ELECTROKINETIC MEASUREMENTS; PVC/PET MIXTURES; FTIR-ATR
Author Information
Reprint Address: Skvarla, J (reprint author)
Tech Univ Kosice, Inst Montaneous Sci & Environm Protect, Ctr Primary & Secondary Raw Mat
Proc, Pk Komenskeho 19, Kosice 04384, Slovakia.
Addresses:
[ 1 ] Tech Univ Kosice, Inst Montaneous Sci & Environm Protect, Ctr Primary & Secondary Raw
Mat Proc, Kosice 04384, Slovakia
E-mail Addresses: [email protected]
Funding
Funding Agency Grant Number
Scientific Grant Agency of the Slovak Republic (VEGA) 2/0159/08
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Most Recent Citation
Peng, Boyu. Flexible organictransistors on standard printing paperand memory properties induced byfloated gate electrode. ORGANICELECTRONICS, JAN 2014.
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Slovak Research and Development Agency APVV-0598-07
View funding text
Publisher
AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Categories / Classification
Research Areas: Science & Technology - Other Topics; Materials Science
Web of Science Categories: Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
Document Information
Document Type: Article
Language: English
Accession Number: WOS:000280367000048
ISSN: 1944-8244
Journal Information
Table of Contents: Current Contents Connect ®
Impact Factor: Journal Citation Reports ®
Other Information
IDS Number: 631SB
Cited References in Web of Science Core Collection: 74
Times Cited in Web of Science Core Collection: 4
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Electrokinetic Potential for Characterization of
Nanosctructured Solid Fiat Surfaces
By: Kolska, Z (Kolska, Zdenka)[ 1 ] ; Kasalkova, NS (Kasalkova, Nikola Slepickova)[ 2 ] ; Siegel, J (Siegel,
Jakub)[ 2 ] ; Svorcik, V (Svorcik, Vaclav)[ 2 ]
JOURNAL OF NANO RESEARCH
Volume: 25 Pages: 31-39
DOI: 10.4028/www.scientific.net/JNanoR.25.31
Published: 2013
View Journal Information
Abstract
Electrokinetic potential (zeta potential) is a characteristic parameter for description of the surface
chemistry of solid flat materials and it can be used for a fast analysis of materials modified by different
chemical or physical methods. Due to its sensitivity, zeta potential is able to distinguish surface modified
by coating with monolayers of various materials or nanostructures created after plasma treatment. Also
metal nanostructures deposited on surfaces can be characterized by zeta potential. It can also be used
for isoelectric point determination of materials. We present data on zeta potential in 0.001 mol/dm(3) KCl
at constant pH approximate to 7.0 and also in pH range (2.5-7.0) for isoelectric point determination for
pristine polymers PET, PTFE, PS, LDPE, HDPE, PLLA, PVF, PVDF, PMP and polyimides (Upilex R,
Upilex S, Kapton). The zeta potential of selected polymers, modified by plasma and by chemical coatings
(e.g. by biphenyldithiol or polyethyleneglycol) or by gold deposition was measured too. Zeta potentials of
these modified materials were also studied to confirmation that electrokinetic analysis is acceptable
method for their fast description.
Keywords
Author Keywords: electrokinetic potential; polymers; surface modification; plasma treatment; gold
deposition; cell adhesion and proliferation
KeyWords Plus: CELL-ADHESION; POLYETHYLENE; POLYTETRAFLUOROETHYLENE;
PROLIFERATION; POLYMERS; CHARGE
Author Information
Reprint Address: Kolska, Z (reprint author)
Univ JE Purkyne, Fac Sci, Ceske Mladeze 8, Usti Nad Labem 40096, Czech Republic.
Addresses:
[ 1 ] Univ JE Purkyne, Fac Sci, Usti Nad Labem 40096, Czech Republic
[ 2 ] Inst Chem Technol, Dept Solid State Engn, CR-16628 Prague, Czech Republic
E-mail Addresses: [email protected]; [email protected]; [email protected];
Funding
Funding Agency Grant Number
Grant Agency of Czech Republic 13-06609S
P108/10/1106
View funding text
Publisher
TRANS TECH PUBLICATIONS LTD, LAUBISRUTISTR 24, STAFA-ZUERICH, CH-8712,
SWITZERLAND
Categories / Classification
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1 Times Cited
20 Cited References
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1 in All Databases
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Most Recent Citation
Reznickova, Alena. Characterization ofSurface Nanostructures on "Thin"Polyolephine Foils. JOURNAL OFNANO RESEARCH, 2014.
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Research Areas: Science & Technology - Other Topics; Materials Science; Physics
Web of Science Categories: Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
Document Information
Document Type: Article
Language: English
Accession Number: WOS:000327907800004
ISSN: 1662-5250
eISSN: 1661-9897
Journal Information
Impact Factor: Journal Citation Reports ®
Other Information
IDS Number: 264UZ
Cited References in Web of Science Core Collection: 20
Times Cited in Web of Science Core Collection: 1
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Cited References: 20(from Web of Science Core Collection)
From: Electrokinetic Potential for Characterization of Nanosctructured Solid Fiat Surfaces ...More
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OCT 1 2003
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Title: [not available]
By: Hiemenz, P.C.; Rajagopalan, R.
Principles of Colloid and Surface Chemistry Published: 1997
Publisher: Marcel Dekker, New York
Times Cited: 1,205
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(from Web of Science Core
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Cell adhesion and proliferation on polyethylene grafted with Au nanoparticlesBy: Kasalkova, N. Slepickova; Slepicka, P.; Kolska, Z.; et al.
Conference: 17th International Conference on Ion Beam Modification of Materials (IBMM) Location: Montreal, CANADA
Date: AUG 22-27, 2010
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH
MATERIALS AND ATOMS Volume: 272 Pages: 391-395 Published: FEB 1 2012
Full Text from Publisher View Abstract
Times Cited: 6
(from Web of Science Core
Collection)
Zeta potential of microfluidic substrates: 1. Theory, experimental techniques, and effects on
separationsBy: Kirby, BJ; Hasselbrink, EF
ELECTROPHORESIS Volume: 25 Issue: 2 Pages: 187-202 Published: JAN 2004
View Abstract
Times Cited: 363
(from Web of Science Core
Collection)
Surface characterization of polymer foils
By: Kolska, Z.; Reznickova, A.; Svorcik, V.
E-Polymers Volume: 83 Pages: 1-13 Published: 2012
Times Cited: 10
(from Web of Science Core
Collection)
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TEKSTIL Volume: 58 Issue: 8 Pages: 393-400 Published: AUG 2009
View Abstract
Times Cited: 3
(from Web of Science Core
Collection)
Cell microarrays on photochemically modified polytetrafluorethylene Times Cited: 51
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By: Mikulikova, R; Moritz, S; Gumpenberger, T; et al.
BIOMATERIALS Volume: 26 Issue: 27 Pages: 5572-5580 Published: SEP 2005
Full Text from Publisher View Abstract
(from Web of Science Core
Collection)
Nano-structuring of PTFE surface by plasma treatment, etching, and sputtering with goldBy: Reznickova, Alena; Kolska, Zdenka; Hnatowicz, Vladimir; et al.
JOURNAL OF NANOPARTICLE RESEARCH Volume: 13 Issue: 7 Pages: 2929-2938 Published: JUL 2011
View Abstract
Times Cited: 11
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Comparison of glow argon plasma-induced surface changes of thermoplastic polymersBy: Reznickova, A.; Kolska, Z.; Hnatowicz, V.; et al.
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH
MATERIALS AND ATOMS Volume: 269 Issue: 2 Pages: 83-88 Published: JAN 15 2011
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Times Cited: 27
(from Web of Science Core
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Properties of gold nanostructures sputtered on glassBy: Siegel, Jakub; Lyutakov, Olexiy; Rybka, Vladimir; et al.
NANOSCALE RESEARCH LETTERS Volume: 6 Article Number: 96 Published: 2011
Full Text from Publisher View Abstract
Times Cited: 27
(from Web of Science Core
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Relationship of Surface Hydrophilicity, Charge, and Roughness of PET Foils Stimulated by Incipient
Alkaline HydrolysisBy: Skvarla, Jiri; Luxbacher, Thomas; Nagy, Martin; et al.
ACS APPLIED MATERIALS & INTERFACES Volume: 2 Issue: 7 Pages: 2116-2127 Published: JUL 2010
View Abstract
Times Cited: 4
(from Web of Science Core
Collection)
Properties of Au nanolayers on polyethyleneterephthalate and polytetrafluoroethyleneBy: Slepicka, P.; Kolska, Z.; Nahlik, J.; et al.
SURFACE AND INTERFACE ANALYSIS Volume: 41 Issue: 9 Pages: 741-745 Published: AUG 2009
View Abstract
Times Cited: 28
(from Web of Science Core
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Title: [not available]
By: Svorcik, V; Reznickova, A; Kolska, Z; et al.
e-Polymers Volume: 133 Pages: 1-6 Published: 2010
[Show additional data]
Times Cited: 10
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Plasma-Modified and Polyethylene Glycol-Grafted Polymers for Potential Tissue Engineering
ApplicationsBy: Svorcik, V.; Makajova, Z.; Kasalkova-Slepickova, N.; et al.
Conference: 3rd International Conference on Advanced Nano Materials (ANM) Location: Agadir, MOROCCO Date: SEP
12-15, 2010
JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY Volume: 12 Issue: 8 Pages: 6665-6671 Published: AUG
2012
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Times Cited: 8
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Properties of Au nanolayer sputtered on polyethyleneterephthalateBy: Svorcik, V.; Kolska, Z.; Luxbacher, T.; et al.
MATERIALS LETTERS Volume: 64 Issue: 5 Pages: 611-613 Published: MAR 15 2010
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Times Cited: 21
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Cytocompatibility of Ar(+) plasma treated and Au nanoparticle-grafted PEBy: Svorcik, V.; Kasalkova, N.; Slepicka, P.; et al.
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH
MATERIALS AND ATOMS Volume: 267 Issue: 11 Pages: 1904-1910 Published: JUN 1 2009
Full Text from Publisher View Abstract
Times Cited: 36
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Modification of surface properties of high and low density polyethylene by Ar plasma dischargeBy: Svorcik, V; Kolarova, K; Slepicka, P; et al.
POLYMER DEGRADATION AND STABILITY Volume: 91 Issue: 6 Pages: 1219-1225 Published: JUN 2006
Full Text from Publisher View Abstract
Times Cited: 101
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Relationship of Surface Hydrophilicity, Charge, and Roughness
of PET Foils Stimulated by Incipient Alkaline Hydrolysis
By: Skvarla, J (Skvarla, Jiri)[ 1 ] ; Luxbacher, T (Luxbacher, Thomas); Nagy, M (Nagy, Martin)[ 1 ] ; Sisol,
M (Sisol, Martin)[ 1 ]
ACS APPLIED MATERIALS & INTERFACES
Volume: 2 Issue: 7 Pages: 2116-2127
DOI: 10.1021/am100368v
Published: JUL 2010
View Journal Information
Abstract
An enhancement of wettability of PET foils pretreated hydrolytically by immersing in mild alkaline (NaOH)
solutions has been documented by a descending sigmoidal dependence between the interfacial free
energy gamma(SL) of the PET/water interface and the concentration of NaOH solution c(NaOH). An
increase in temperature of the NaOH solution below the glass-transition temperature of PET further
promotes the hydrophilicity, resulting in a proportional shift of the gamma(SL) VS c(NaOH) dependence.
The limiting hydrophilicity of PET is thermodynamically predicted to occur at gamma(SL) -> 0,
corresponding to the advancing water contact angle theta(a) approximate to 50 degrees (for 6% NaOH
and 60 degrees C). The surface roughness due to the partial hydrolytic degradation as well as the weight
loss (dissolution) of PET are found to reach a maximum value just when the latter dependence goes
through its inflection. Assuming a general parallelism between the interfacial free energy and the
dissolution kinetics, we propose the hydrolytically stimulated formation and growth of pits on the PET
surface to cause the initial acceleration as well as subsequent retardation of dissolution as c(NaOH),
increases, leading to the S-shaped gamma(SL) VS c(NaOH) dependence with the inflection for a specific
c(NaOH). Moreover, the zeta potential measured by the streaming current method also attains a
maximum at the same specific concentration of NaOH. It would indicate that the largest amount of
electric charges is populated via polar carboxyl and hydroxyl groups created by chemical scissions of
PET polymer chains when a change in the dissolution rate increases to the utmost. In such a way, partial
hydrolysis restricted to the uppermost part of moderately hydrophobic surface of solid PET allowed us to
better understand the intermingled role of thermodynamic and physical aspects in surface wettability
itself:
Keywords
Author Keywords: PET; hydrolysis; wettability; surface roughness; interfacial free energy; contact
angle; alkaline degradation; dissolution
KeyWords Plus: SPUN POLY(ETHYLENE-TEREPHTHALATE) FIBERS; MOISTURE-RELATED
PROPERTIES; FROTH FLOTATION; POLYVINYL-CHLORIDE; POLYMER SURFACES; CONTACT
ANGLES; FREE-ENERGY; ELECTROKINETIC MEASUREMENTS; PVC/PET MIXTURES; FTIR-ATR
Author Information
Reprint Address: Skvarla, J (reprint author)
Tech Univ Kosice, Inst Montaneous Sci & Environm Protect, Ctr Primary & Secondary Raw Mat
Proc, Pk Komenskeho 19, Kosice 04384, Slovakia.
Addresses:
[ 1 ] Tech Univ Kosice, Inst Montaneous Sci & Environm Protect, Ctr Primary & Secondary Raw
Mat Proc, Kosice 04384, Slovakia
E-mail Addresses: [email protected]
Funding
Funding Agency Grant Number
Scientific Grant Agency of the Slovak Republic (VEGA) 2/0159/08
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Peng, Boyu. Flexible organictransistors on standard printing paperand memory properties induced byfloated gate electrode. ORGANICELECTRONICS, JAN 2014.
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Slovak Research and Development Agency APVV-0598-07
View funding text
Publisher
AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Categories / Classification
Research Areas: Science & Technology - Other Topics; Materials Science
Web of Science Categories: Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
Document Information
Document Type: Article
Language: English
Accession Number: WOS:000280367000048
ISSN: 1944-8244
Journal Information
Table of Contents: Current Contents Connect ®
Impact Factor: Journal Citation Reports ®
Other Information
IDS Number: 631SB
Cited References in Web of Science Core Collection: 74
Times Cited in Web of Science Core Collection: 4
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Impinging jet study of the deposition of colloidal particles on
modified polycarbonate and poly(ethylene terephthalate)
surfaces
By: Lapcik, L (Lapcik, Lubomir, Jr.)[ 1 ] ; Frastik, M (Frastik, Michal)[ 1 ] ; Lapcikova, B (Lapcikova,
Barbora)[ 1 ]
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER
Volume: 55 Issue: 5-6 Pages: 1513-1518
DOI: 10.1016/j.ijheatmasstransfer.2011.11.002
Published: FEB 2012
View Journal Information
Abstract
Main focus of this study was on characterization of surface properties of virgin and 1,2-dipalmitoyl-
sn-glycero-3-phosphocholine (DPPC) phospholipid layer coated poly(ethylene terephthalate) (PET) and
polycarbonate (PC) planar articles. Surface properties were followed measuring static contact angles of
wetting by means of sessile drop method and deposition of negative polystyrene (PS) colloidal particles
followed by impinging jet method at defined flow regimes. It was found that phospholipid coating of both
studied samples (PET, PC) let to the vigorous increase of the surface free energy. For coated samples
major part of the surface free energy was dominated by polar component in contrast to the non-treated
materials. Here the dispersive component was dominating. Results of the deposition experiments of
polystyrene particles of 3 mu m diameter correspond with trends obtained by contact angle
measurements, i.e. the surface treated materials exhibited higher surface activity reflected in increased
particle deposition rates. Simultaneously there was confirmed the fact, that with increasing magnitude of
the Reynolds number of the dispersion flux the higher deposition rates were observed. (C) 2011 Elsevier
Ltd. All rights reserved.
Keywords
Author Keywords: Contact angles of wetting; Impinging jet; Poly(ethylene terephthalate);
Polycarbonate; Phospholipid layer; Polystyrene particles; Deposition kinetics
KeyWords Plus: HYALURONIC-ACID; SOLID-SURFACES; KINETICS; ADSORPTION; WALL
Author Information
Reprint Address: Lapcik, L (reprint author)
Tomas Bata Univ Zlin, Fac Technol, Ctr Polymer Syst, Nam TG Masaryka 5555, Zlin 76005, Czech
Republic.
Addresses:
[ 1 ] Tomas Bata Univ Zlin, Fac Technol, Ctr Polymer Syst, Zlin 76005, Czech Republic
E-mail Addresses: [email protected]
Author Identifiers:
Funding
Funding Agency Grant Number
Operational Program Research and Development for Innovations
European Regional Development Fund (ERDF)
national budget of Czech Republic CZ.1.05/2.1.00/03.0111
View funding text
Publisher
PERGAMON-ELSEVIER SCIENCE LTD, THE BOULEVARD, LANGFORD LANE, KIDLINGTON,
Citation Network
1 Times Cited
26 Cited References
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Most Recent Citation
Vlcek, Jakub. Impinging jet study of thedeposition of colloidal particles onsynthetic polymer (Zeonor).INTERNATIONAL JOURNAL OFHEAT AND MASS TRANSFER, NOV2014.
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OXFORD OX5 1GB, ENGLAND
Categories / Classification
Research Areas: Thermodynamics; Engineering; Mechanics
Web of Science Categories: Thermodynamics; Engineering, Mechanical; Mechanics
Document Information
Document Type: Article
Language: English
Accession Number: WOS:000300333700009
ISSN: 0017-9310
Journal Information
Table of Contents: Current Contents Connect ®
Impact Factor: Journal Citation Reports ®
Other Information
IDS Number: 893CR
Cited References in Web of Science Core Collection: 26
Times Cited in Web of Science Core Collection: 1
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Cited References: 26(from Web of Science Core Collection)
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Role of convection in particle deposition at solid surfacesBy: Adamczyk, Z; Warszynski, P; Szyk-Warszynska, L; et al.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS Volume: 165 Issue: 1-3 Pages:
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Full Text from Publisher View Abstract
Times Cited: 25
(from Web of Science Core
Collection)
Kinetics of particle deposition in the radial impinging-jet cellBy: Adamczyk, Z; Siwek, B; Warszynski, P; et al.
JOURNAL OF COLLOID AND INTERFACE SCIENCE Volume: 242 Issue: 1 Pages: 14-24 Published: OCT 1 2001
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KINETICS OF LOCALIZED ADSORPTION OF COLLOID PARTICLESBy: ADAMCZYK, Z; SIWEK, B; ZEMBALA, M; et al.
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Particles at Interfaces: Interactions, Deposition, StructureBy: Adamczyk, Z
PARTICLES AT INTERFACES: INTERACTIONS, DEPOSITION, STRUCTURE Book Series: Interface Science and
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Publisher: ELSEVIER ACADEMIC PRESS INC, 525 B STREET, SUITE 1900, SAN DIEGO, CA 92101-4495 USA
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COLLOID AND POLYMER SCIENCE Volume: 261 Issue: 8 Pages: 694-707 Published: 1983
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Full Text from Publisher
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(from Web of Science Core
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SLOW VISCOUS MOTION OF A SPHERE PARALLEL TO A PLANE WALL .2. COUETTE FLOW
By: GOLDMAN, AJ; COX, RG; BRENNER, H
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Times Cited: 736
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Zeta potential and surface free energy changes of solid-supported phospholipid (DPPC) layers caused
by the enzyme phospholipase A(2) (PLA(2))By: Jurak, Malgorzata; Chibowski, Emil
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Published: APR 2009
View Abstract
Times Cited: 9
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Wettability and topography of phospholipid DPPC multilayers deposited by spin-coating on glass,
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Hyaluronan: Preparation, structure, properties, and applicationsBy: Lapcik, L; Lapcik, L; De Smedt, S; et al.
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COLLOID AND POLYMER SCIENCE Volume: 269 Issue: 6 Pages: 633-635 Published: JUN 1991
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Relationship of Surface Hydrophilicity, Charge, and Roughness of PET Foils Stimulated by Incipient
Alkaline HydrolysisBy: Skvarla, Jiri; Luxbacher, Thomas; Nagy, Martin; et al.
ACS APPLIED MATERIALS & INTERFACES Volume: 2 Issue: 7 Pages: 2116-2127 Published: JUL 2010
View Abstract
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(from Web of Science Core
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Title: [not available]
By: van de Ven, TGM.
Colloidal hydrodynamics Published: 1989
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10.
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3 z 3 7. 11. 2014 11:08
Relationship of Surface Hydrophilicity, Charge, and Roughness
of PET Foils Stimulated by Incipient Alkaline Hydrolysis
By: Skvarla, J (Skvarla, Jiri)[ 1 ] ; Luxbacher, T (Luxbacher, Thomas); Nagy, M (Nagy, Martin)[ 1 ] ; Sisol,
M (Sisol, Martin)[ 1 ]
ACS APPLIED MATERIALS & INTERFACES
Volume: 2 Issue: 7 Pages: 2116-2127
DOI: 10.1021/am100368v
Published: JUL 2010
View Journal Information
Abstract
An enhancement of wettability of PET foils pretreated hydrolytically by immersing in mild alkaline (NaOH)
solutions has been documented by a descending sigmoidal dependence between the interfacial free
energy gamma(SL) of the PET/water interface and the concentration of NaOH solution c(NaOH). An
increase in temperature of the NaOH solution below the glass-transition temperature of PET further
promotes the hydrophilicity, resulting in a proportional shift of the gamma(SL) VS c(NaOH) dependence.
The limiting hydrophilicity of PET is thermodynamically predicted to occur at gamma(SL) -> 0,
corresponding to the advancing water contact angle theta(a) approximate to 50 degrees (for 6% NaOH
and 60 degrees C). The surface roughness due to the partial hydrolytic degradation as well as the weight
loss (dissolution) of PET are found to reach a maximum value just when the latter dependence goes
through its inflection. Assuming a general parallelism between the interfacial free energy and the
dissolution kinetics, we propose the hydrolytically stimulated formation and growth of pits on the PET
surface to cause the initial acceleration as well as subsequent retardation of dissolution as c(NaOH),
increases, leading to the S-shaped gamma(SL) VS c(NaOH) dependence with the inflection for a specific
c(NaOH). Moreover, the zeta potential measured by the streaming current method also attains a
maximum at the same specific concentration of NaOH. It would indicate that the largest amount of
electric charges is populated via polar carboxyl and hydroxyl groups created by chemical scissions of
PET polymer chains when a change in the dissolution rate increases to the utmost. In such a way, partial
hydrolysis restricted to the uppermost part of moderately hydrophobic surface of solid PET allowed us to
better understand the intermingled role of thermodynamic and physical aspects in surface wettability
itself:
Keywords
Author Keywords: PET; hydrolysis; wettability; surface roughness; interfacial free energy; contact
angle; alkaline degradation; dissolution
KeyWords Plus: SPUN POLY(ETHYLENE-TEREPHTHALATE) FIBERS; MOISTURE-RELATED
PROPERTIES; FROTH FLOTATION; POLYVINYL-CHLORIDE; POLYMER SURFACES; CONTACT
ANGLES; FREE-ENERGY; ELECTROKINETIC MEASUREMENTS; PVC/PET MIXTURES; FTIR-ATR
Author Information
Reprint Address: Skvarla, J (reprint author)
Tech Univ Kosice, Inst Montaneous Sci & Environm Protect, Ctr Primary & Secondary Raw Mat
Proc, Pk Komenskeho 19, Kosice 04384, Slovakia.
Addresses:
[ 1 ] Tech Univ Kosice, Inst Montaneous Sci & Environm Protect, Ctr Primary & Secondary Raw
Mat Proc, Kosice 04384, Slovakia
E-mail Addresses: [email protected]
Funding
Funding Agency Grant Number
Scientific Grant Agency of the Slovak Republic (VEGA) 2/0159/08
Citation Network
4 Times Cited
74 Cited References
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(data from Web of Science TM Core Collection)
All Times Cited Counts
4 in All Databases
4 in Web of Science Core Collection
0 in BIOSIS Citation Index
0 in Chinese Science CitationDatabase
0 in Data Citation Index
0 in SciELO Citation Index
Most Recent Citation
Peng, Boyu. Flexible organictransistors on standard printing paperand memory properties induced byfloated gate electrode. ORGANICELECTRONICS, JAN 2014.
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Slovak Research and Development Agency APVV-0598-07
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Publisher
AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Categories / Classification
Research Areas: Science & Technology - Other Topics; Materials Science
Web of Science Categories: Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
Document Information
Document Type: Article
Language: English
Accession Number: WOS:000280367000048
ISSN: 1944-8244
Journal Information
Table of Contents: Current Contents Connect ®
Impact Factor: Journal Citation Reports ®
Other Information
IDS Number: 631SB
Cited References in Web of Science Core Collection: 74
Times Cited in Web of Science Core Collection: 4
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