Time response of a GSO crystal - LHCb Cagliari

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UNIVERSITY OF CAGLIARI Faculty of Mathematical, Physical and Natural Sciences Degree Course in Physics Time response of a GSO crystal Supervisor: Prof. Biagio Saitta Candidate: Giacomo Caria Academic Year 2011-2012

Transcript of Time response of a GSO crystal - LHCb Cagliari

Page 1: Time response of a GSO crystal - LHCb Cagliari

UNIVERSITY OF CAGLIARI

Faculty of Mathematical, Physical and Natural Sciences

Degree Course in Physics

Time response of a GSO crystal

Supervisor:Prof. Biagio Saitta

Candidate:Giacomo Caria

Academic Year 2011-2012

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Acknowledgements

Foremost, I would like to express my sincere gratitude to my supervisor Prof.Biagio Saitta, for his patience, motivation, expertise and wide knowledge. Hisguidance deeply helped me in all the time of experimental work and writingof this thesis.

I am also grateful to Prof. Alessandro Cardini, for his useful help for bothexperimental and theoretical matters.

Last but not least, I would like to thank my family for the essentialsupport provided throughout all these years and for letting me free to choosemy personal path.

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Contents

Introduction 1

1 Methods and materials 31.1 Scintillation mechanism in inorganic crystals . . . . . . . . . . 31.2 TCSPC method . . . . . . . . . . . . . . . . . . . . . . . . . . 41.3 Experimental setup . . . . . . . . . . . . . . . . . . . . . . . . 5

2 Results 92.1 Detectors timing performance . . . . . . . . . . . . . . . . . . 92.2 Test setup using fast plastic scintillator . . . . . . . . . . . . . 112.3 Measurement of GSO decay time . . . . . . . . . . . . . . . . 162.4 Conclusions . . . . . . . . . . . . . . . . . . . . . . . . . . . . 19

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vi CONTENTS

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List of Figures

1.1 Experimental setup used for the measurement of the decaytime of GSO . . . . . . . . . . . . . . . . . . . . . . . . . . . 7

2.1 Coincidence resolution time for EJ-200 scintillator . . . . . . . 102.2 Coincidence resolution time for GSO crystal . . . . . . . . . . 102.3 ∆t distribution of EJ-200 scintillator for d = 1 cm . . . . . . . 122.4 ∆t distribution of EJ-200 scintillator for d = 6 cm . . . . . . . 122.5 ∆t distribution of EJ-200 scintillator for d = 16 cm . . . . . . 132.6 ∆t distribution of EJ-200 scintillator for d = 68 cm . . . . . . 132.7 Exponential fit to data for EJ-200 scintillator and d = 1 cm . 142.8 Exponentials sum fit to data for EJ-200 scintillator and d = 6

cm . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 142.9 Exponentials sum fit to data for EJ-200 scintillator and d =

16 cm . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 152.10 Exponential fit to data for EJ-200 scintillator and d = 68 cm . 152.11 ∆t distribution of GSO crystal for d = 1 cm . . . . . . . . . . 172.12 ∆t distribution of GSO crystal for d = 6 cm . . . . . . . . . . 172.13 ∆t distribution of GSO crystal for d = 16 cm . . . . . . . . . 182.14 ∆t distribution of GSO crystal for d = 68 cm . . . . . . . . . 182.15 ∆t distribution of GSO crystal for d = 16 cm with pinhole . . 192.16 Exponential fit to data for GSO crystal for d = 1 cm . . . . . 202.17 Exponentials sum fit to data for GSO crystal and d = 6 cm . 202.18 Exponentials sum fit to data for GSO crystal and d = 16 cm . 212.19 Exponentials sum fit to data for GSO crystal and d = 68 cm . 212.20 Exponentials sum fit to data for GSO crystal and d = 16, with

pinhole . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 222.21 Comparison of time distributions at different distances for

small ∆t . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 232.22 Comparison of time distributions at different distances for

large ∆t . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 24

vii

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viii LIST OF FIGURES

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List of Tables

2.1 Results of the fit for EJ-200 scintillator . . . . . . . . . . . . . 162.2 Results of the fit for GSO crystal . . . . . . . . . . . . . . . . 19

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x LIST OF TABLES

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Introduction

The aim of this work is a measurement of the decay time of a crystalof the inorganic scintillator GSO, Cerium-doped Gadolinium orthosilicate,Gd2SiO5:Ce, in the context of a project which studies the feasibility of an ac-tive, electron polarized detector to be used with neutrino (and anti-neutrino)beams [1],[2].

One of the interesting characteristics of the GSO in fact is that, beinga paramagnetic crystal, it can be temporarily polarized, albeit only for asmall electron fraction; the polarization changes the cross-sections and thusprovides a new degree of freedom in the understanding of the properties of theinteracting particles. The properties of GSO have been extensively studiedsince its discovery in 1983 by Takagi and Fukazawa [3]; the value of the decaytime has been measured and found to depend on the Ce concentration [5],[6], therefore it is of interest to perform an independent measurement on theactual crystal used to study the magnetic properties.

The technique used for this work is known as time-correlated single pho-ton counting (TCSPC) and it is based on the theoretical consideration thatthe function describing the rate of photons emitted per second by a scin-tillator must have, apart for a normalization factor, the same shape of theprobability distribution function (PDF) of the emitting process. As a conse-quence, recording a large number of elapsed times between the scintillationevents and the emission of single and randomly independent photons, it ispossible to construct an experimental PDF histogram, and its fit with atheoretical model will provide the decay process characteristic time.

One of the features of the experimental setup is that it has to recordsingle photons which are casually uncorrelated with one another. This resultis achieved by placing a detector at a proper distance from the GSO crystal,so that at most one photon will reach, at a very slow rate, the device foreach scintillation event. In general as single-photon sensitive detector a Pho-tomultiplier Tube (PMT), a Micro Channel Plate (MCP) or a Single PhotonAvalanche Diode (SPAD) can be used. Also, to reduce light intensity, aneutral density filter can be inserted between the PMT and the GSO crys-

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2 LIST OF TABLES

tal, as used in other measurements. In our experimental setup a PMT wasused, in some instances with the photocathode partially masked to reducethe sensitive area.

Among the possible methods to measure the excitation time, for practicalreasons, a PMT attached to the GSO was used.

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Chapter 1

Methods and materials

1.1 Scintillation mechanism in inorganic crys-

tals

Energy release in a material, which will consequentially emit light, can occurin different ways. Incandescence is the process where thermal motion istransformed into electromagnetic radiation, while we refer to luminescence forall the other processes which do not involve heat. For instance, energy maybe released in the material by a mechanical action as in triboluminescence, orsupplied by chemical reaction as in chemiluminescence, while when excitationis caused by incident electromagnetic radiation we have photoluminescence.More in detail, we define fluorescence as photoluminescence or scintillationwhich presents a fast decay time, approximately 10−9 to 10−7 sec, while longertimes are the main characteristics of phosphorescence, 10−6 to 103 sec.

Scintillation, i.e. light emission yielded by ionization radiations of chargedparticle which excite the material, differs for the following materials: inor-ganic crystals, organic crystals, noble gases and liquids, plastic scintillators.We will examine further how light emission occurs in inorganic crystals [4],since the topic of this thesis is the GSO scintillator. In these substances scin-tillation depends strongly on the crystal band structure. In fact, ionizationcauses the transfer of electrons from the valence band into the conductionband, and consequentially vacancies (known as holes) are left in the valenceband, for many purposes can be thought as physical particles with positivecharge +e which are free to move in the valence band.

Although this mechanism creates a pair of electron and hole that are notcoupled, in other cases, i.e. the formation of an exciton, the pair can betightly bound and move as a single particle in the crystal, with the electronexcited to an energy level just below the conduction band, in that region

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4 CHAPTER 1. METHODS AND MATERIALS

known as forbidden band. Impurities play a fundamental role in the scintil-lation process, since they provide a site for the recombination of electron-holepairs. In fact, this can happen when a hole free to move in the valence bandcomes close to an atom impurity, also called activator site. The latter willbe ionized by a migrating free hole or a hole from an exciton pair , as one ofits electrons escapes from the fundamental state. As a consequence electronscan be captured in the activator excited states and decay in the activatorground state, with the emission of scintillation light. Impurities centers arestrongly efficient since the dopant atom is left in its original state so thateach center may partecipate in many recombination.

When the electron is placed in an activator excited states with forbiddentransitions to the ground state, known as metastable states, it requires anadditional energy to move into another excited state where it is finally free todecay, or may decay spontaneously, but the latter options is highly improb-able . This mechanism needs a long time that is, as previously stated, themain property of phosphorescence. Another reason for slow light emissionis the formation of traps, which may be defined as sites with energies in theforbidden band, where only one type of charge carrier is accepted, avoidingtherefore the possibility of recombination. Such centers hold the electron orthe hole and release it after a certain characteristic time.

Our energy source is a γ-ray emitter, therefore we will not have manyinelastic collisions with atomic electrons, a typical property of charged par-ticles. Instead, photons interact with matter by:

1. Photoelectric effect

2. Compton scattering

3. Pair production

The interaction cross section through each of these mechanisms is energydependent, photoelectric effect and Compton scattering being dominant atlow and medium energy and pair production at high energy with an onset at1.02 MeV, the mass energy of an electron-positron pair at rest.

1.2 TCSPC method

The easiest method for measuring the time decay of the scintillation processwould be to directly fit a pulse shape, i.e. the number of photons emitted perunit time as a function of time, recorded as electronic signal, by a theoreticalfunction. Nevertheless, for the intrinsic limits of electronic devices, we cannot rely on this procedure. The solution to this problem is the technique

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1.3. EXPERIMENTAL SETUP 5

called time-correlated single photon counting, described by Bollinger andThomas [7].

We define a probability distribution function (PDF) p(t, tstart) such thatthe probability of emitting a single scintillation photon in the time intervalt, t + dt after the interaction of a γ-photon with a crystal scintillator atthe time tstart is equal to p(t, tstart) · dt. This distribution is equal to thescintillation pulse shape, except for a normalization factor, therefore our goalof measuring the decay time of the GSO crystal may be achieved recording alarge number of single scintillation photons and constructing empirically thePDF.

In more detail, we are interested in the time elapsed between the absorp-tion of the incident radiation by the crystal (which defines t = 0) and theemission of these single scintillation photons, whose distribution is indeedprobabilistically determined. It is important to stress that the photons reg-istered by the stop detector have to be not only single but also statisticallyindependent. Consider the case where several photons produced by the samescintillation event reach the stop detector. It will be triggered by the firstphoton in arrival order, which will be also the only one providing an arrivaltime for calculating the requested time difference with the start time.

It is easy to see how this affects the statistical foundation of the TCSPCmethod. Recording only the first photons, we have an over-representationof early arrival times, an effect called pile-up, since all the other later timescan not be collected and are in fact discarded, so that the true randomnessof essential value for this technique is lost.

In order to avoid biasing the data which will fill the histogram and in turnpermit to draw the pulse shape, the experimental setup must be designedin such a way that even the possibility of detecting one single photon perscintillation event is low. As a consequence, this ensures that probabilitiesfor the stop detector to detect two or more photons are absolutely negligible.

1.3 Experimental setup

As start and stop detectors for the TCSPC measurements two photomul-tiplier tubes HAMAMATSU H6533 have been used. This device, sensitivebetween 300 to 650 nm, with a wavelength of maximum response of 420 nmclose to the GSO emission wavelength, has been chosen mainly for its fastresponse, which includes a rise time and a transit time spread (TTS) of 0.7ns and 0.16 ns respectively.

All measurements were performed at room temperature. The power sup-ply is a programmable CAEN model N471. PMTs were operated at different

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6 CHAPTER 1. METHODS AND MATERIALS

voltages, 2000 V for the start detector and 2250 V for the stop detector.The GSO crystal, with dimensions 2x2x10 mm3, is excited by a 60Co

radioactive source which is a γ-ray emitter.One of the PMTs, which we will refer to as start detector, is attached

to the GSO crystal and coupled optically to it using a optical grease inorder to optimize the light collection. These conditions permit the startdetector to collect a large amount of light, so that early emitted photons inthe scintillation event hit surely the detector, providing the start time forthe TCSPC method.

From the side of the crystal opposite to the one attached to the startdetector, light can reach the second PMT, which we will refer to as stopdetector. As emphasized in the theoretical section, the rate at which singlephotons arrive at the stop detector must be exceptionally low, so that theprobability for receiving two or more photons emitted in the same scintil-lation event is absolutely negligible, hence ensuring that the fundamentalcondition for the TCSPC technique is satisfied. As a consequence the stopPMT detector has been placed at a variable distance d from the crystal andin one case its aperture has been properly adjusted with a pinhole to reducefurther the light intensity.

In order to avoid false-stop signals, which are time interval measurementsof stop pulses and start signals not causally correlated, mainly due to darknoise, both start an stop PMTs signals were fed into a low threshold CAENN224 discriminator which accepts only events above the thresholds set at10.5 mV and 2.5 mV respectively, and forms NIM pulses (400ns wide).

Discriminator signals were read out by the oscilloscope LeCroy 104MXi,which calculated time difference between the 50% amplitudes and created ahistogram for all measured start-stop differences, yielding the experimentalpulse shape.

The logic of the data acquisition is schematically represented in fig. 1.1.

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1.3. EXPERIMENTAL SETUP 7

Figure 1.1: Experimental setup used for the measurement of the decay timeof GSO

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8 CHAPTER 1. METHODS AND MATERIALS

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Chapter 2

Results

2.1 Detectors timing performance

Values of several tens of nanoseconds for the so-called ”fast” component andseveral hundreds of nanoseconds for the ”slow” component are reported inliterature for GSO scintillator.

To ascertain the capability of our system to measure values of that or-der as well as to estimate its intrinsic time resolution, two additional set ofmeasurements were carried out in the setup:

1. Time difference when both photomultipliers are in contact with thescintillating GSO crystal and

2. a complete set of measurements at various distances, with the GSOreplaced by a small cylinder of plastic scintillator EJ-200 of size similarto that of the inorganic crystal.

For the first set of measurements a slightly modified setup was used, toallow both photomultipliers to be in contact with the scintillator (either GSOor EJ-200) and optically coupled to it. Also the surface of the photocathodenot in contact with the scintillator was protected by a 2-mm thick lead shieldto avoid photons from the Co60 source to reach directly the active surface.

The time difference between the ”start-detector” and the ”stop-detector”for the two cases is shown in figures 2.2 and 2.1.

In both cases the distribution is centered at slightly negative values, indi-cating that the PMT used as ”stop-detector” has a response faster than thePMT used as ”start-detector”.

It is possible to observe that for both materials the time distributions isbest fitted with a sum of gaussian functions. From a physics point of view

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10 CHAPTER 2. RESULTS

sc1 / ndf 2χ 306.8 / 336

Prob 0.8718

t (sec)∆­5 ­4 ­3 ­2 ­1 0 1 2 3 4

# o

f entr

ies

1

10

210

310 sc1 / ndf 2χ 306.8 / 336

Prob 0.8718

CRT for EJ­200 scintillator

Figure 2.1: Coincidence resolution time for EJ-200 scintillator

gs1 / ndf 2χ 110.7 / 68

Prob 0.0008276

t (sec)∆­10 ­5 0 5 10

# o

f entr

ies

1

10

210

310

gs1 / ndf 2χ 110.7 / 68

Prob 0.0008276

CRT for GSO crystal

Figure 2.2: Coincidence resolution time for GSO crystal

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2.2. TEST SETUP USING FAST PLASTIC SCINTILLATOR 11

this is explained with intrinsic differences between the two PMT detectors,and also as an effect of a different voltage they were operated at.

The different FWHM reflect the characteristic time properties of the twoscintillating materials.

For the GSO crystal, the coincidence resolving time (CRT) is 2.1 nsFWHM, corresponding to a single detector timing resolution of 1.5 ns FWHM,while for the EJ-200 we obtain, respectively, 0.8 ns and 0.6 ns. These valuesrefer to the blue gaussian curve in both figures.

A time resolution of 1.5 ns for GSO and less than 0.6 ns for EJ-200, seemsto be adequate for our purposes.

2.2 Test setup using fast plastic scintillator

A set of preliminary measurements has been taken with the fast plastic scin-tillator EJ-200 instead of the GSO crystal, while the experimental apparatusdescribed in the previous section remains unchanged. This new material hasa decay time, 2.1 ns [9], sensibly shorter than the one we expect for theGSO, but their wavelength of maximum emission is approximately the sameat around 430 nm. The goal of these measurements is to test whether theTCSPC setup is properly working, and this is done analyzing quantitativelythe data obtained using a material with well-known time characteristics. Thedistance between the start detector, coupled optically to the plastic scintilla-tor, and the stop detector assumes the values 1 cm, 6 cm, 16 cm and 68 cm.Recorded time difference distributions are shown respectively in the figures2.3, 2.4, 2.5 and 2.6.

These time distributions have been analyzed with the software packageROOT [8], which allows, among many other features, to fit histograms withpre-defined or user-defined functions. A single exponential appears to de-scribe well the data at 1cm and 68cm, while the data at 6cm and 16cm seemsto require a more complex function. As previously described, light yield iscomposed by two contributes, the fast and the slow component. Therefore,it is natural to model the decay with a function that represents both, i.e. atwo-component exponential the form:

N = A exp(−t/τslow) +B exp(−t/τfast) (2.1)

where τslow and τfast are the decay constants, A and B magnitudes that varyfrom material to material, although the fast component usually dominates.For a better representation, histogram fittings are plotted with with a loga-rithmic y-axis in figures 2.7, 2.8, 2.9 and 2.10.

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12 CHAPTER 2. RESULTS

Mean 1.333e­09

Integral 3.564e+04

t (sec)∆

­1 0 1 2 3 4 5 6 7 8

­910×

# o

f e

ntr

ies

0

100

200

300

400

500

600Mean 1.333e­09

Integral 3.564e+04

d = 1 cm

Figure 2.3: ∆t distribution of EJ-200 scintillator for d = 1 cm

Mean 3.067e­09

Integral 4.041e+04

t (sec)∆

­4 ­2 0 2 4 6 8 10 12 14

­910×

# o

f entr

ies

0

500

1000

1500

2000

2500

3000 Mean 3.067e­09

Integral 4.041e+04

d = 6 cm

Figure 2.4: ∆t distribution of EJ-200 scintillator for d = 6 cm

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2.2. TEST SETUP USING FAST PLASTIC SCINTILLATOR 13

Mean 5.432e­09

Integral 4.611e+04

t (sec)∆

0 2 4 6 8 10 12 14 16 18

­910×

# o

f e

ntr

ies

0

200

400

600

800

1000

1200

1400

1600

1800

2000

2200 Mean 5.432e­09

Integral 4.611e+04

d = 16 cm

Figure 2.5: ∆t distribution of EJ-200 scintillator for d = 16 cm

Mean 8.776e­09

Integral 1.083e+04

t (sec)∆

0 5 10 15 20 25 30

­910×

# o

f entr

ies

0

50

100

150

200

250Mean 8.776e­09

Integral 1.083e+04

d = 68 cm

Figure 2.6: ∆t distribution of EJ-200 scintillator for d = 68 cm

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14 CHAPTER 2. RESULTS

h1 / ndf 2χ 189.7 / 196

Prob 0.6141

t (sec)∆­1 0 1 2 3 4 5 6 7 8

­910×

# o

f entr

ies

1

10

210

310

h1 / ndf 2χ 189.7 / 196

Prob 0.6141

d = 1 cm

0.006) ns± = (0.695 fast

τ

Figure 2.7: Exponential fit to data for EJ-200 scintillator and d = 1 cm

h6 / ndf 2χ 69.44 / 48

Prob 0.02309

t (sec)∆­4 ­2 0 2 4 6 8 10 12 14

­910×

# o

f entr

ies

1

10

210

310

h6 / ndf 2χ 69.44 / 48

Prob 0.02309

d = 6 cm

0.03) ns± = (1.20 fastτ

0.63) ns± = (4.56 slowτ

Figure 2.8: Exponentials sum fit to data for EJ-200 scintillator and d = 6cm

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2.2. TEST SETUP USING FAST PLASTIC SCINTILLATOR 15

h16Prob 0.01549p0 7.735p1 2.612e+08p2 11.75p3 8.673e+08

t (sec)∆

0 2 4 6 8 10 12 14 16 18

­910×

# o

f entr

ies

1

10

210

310

h16Prob 0.01549p0 7.735p1 2.612e+08p2 11.75p3 8.673e+08

d = 16 cm

0.06) ns± = (1.15 fast

τ

0.15)ns± = (3.83 slowτ

Figure 2.9: Exponentials sum fit to data for EJ-200 scintillator and d = 16cm

h68 / ndf 2χ 124.6 / 90

Prob 0.009207

t (sec)∆0 5 10 15 20 25 30

­910×

# o

f e

ntr

ies

1

10

210

h68 / ndf 2χ 124.6 / 90

Prob 0.009207

d = 68 cm

0.06) ns± = (2.82 fast

τ

Figure 2.10: Exponential fit to data for EJ-200 scintillator and d = 68 cm

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16 CHAPTER 2. RESULTS

distance (cm) τfast (ns) τslow (ns)

1 0.695 ± 0.0066 1.20 ± 0.03 4.56 ± 0.6316 1.15 ± 0.06 3.83 ± 0.1568 2.82 ± 0.06

Table 2.1: Results of the fit for EJ-200 scintillator

Since we chose to use the TCSPC method, the most important results weshould discuss are those that are close to the single-photon condition. Hence,the histogram we may assume approximate the probability distribution, i.ethe pulse shape, with our best precision for the fast plastic scintillator hasbeen obtained with d = 68 cm. It is shown in figure 2.10.

The value obtained for the fast component, 2.8 ns, is sufficiently close tothe value provided by the manufacturers, i.e. 2.1 ns. The presence of a slowcomponent was not expected; however since is of order of few nanosecondsdoes not affect the characteristics of this type of scintillator.

In conclusion we have verified it can effectively sample the probabilitydistribution and is therefore appropriate for the next main measurements ofGSO crystal decay times.

Numerical values for fast components obtained fitting the data are sum-marized in table 2.1.

2.3 Measurement of GSO decay time

Measurements have been repeated for different distances between the startand stop detectors, namely 1 cm (fig. 2.11), 6 cm (fig. 2.12), 16 cm (fig.2.13), 68 cm (fig. 2.14), and 16 cm with a pinhole (fig. 2.15) in order to studyquantitatively how time difference distributions change when probabilities forthe single-photon condition increase.

When plotted in a logarithmic scale, these histograms clearly show adouble component behavior, which demonstrates the presence of the twoluminescence processes: the fast luminescence and the slow phosphorescence.As a consequence, the function implemented in the software ROOT for thefit is the same as in the formula 2.1. The two exponentials sum fittings todata are shown, in order of increasing distance between detectors, in figures2.16, 2.17, 2.18, 2.19 and 2.20.

The time distributions at different distances are plotted together in fig.2.21 and 2.22, in order to compare them qualitatively.

The resulting parameter values for each measurement are summarized in

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2.3. MEASUREMENT OF GSO DECAY TIME 17

Mean 2.397e­08

Integral 1.349e+05

t (sec)∆

­0.04 ­0.02 0 0.02 0.04 0.06 0.08 0.1 0.12 0.14

­610×

# o

f e

ntr

ies

0

200

400

600

800

1000

1200

1400

1600

1800

2000

2200

2400

Mean 2.397e­08

Integral 1.349e+05

d = 1 cm

Figure 2.11: ∆t distribution of GSO crystal for d = 1 cm

Mean 3.608e­08

Integral 1.738e+05

t (sec)∆

­0.1 0 0.1 0.2 0.3

­610×

# o

f entr

ies

0

1000

2000

3000

4000

5000

6000

7000

8000

9000Mean 3.608e­08

Integral 1.738e+05

d = 6 cm

Figure 2.12: ∆t distribution of GSO crystal for d = 6 cm

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18 CHAPTER 2. RESULTS

Mean 4.381e­08

Integral 1.118e+05

t (sec)∆

­0.1 0 0.1 0.2 0.3 0.4

­610×

# o

f entr

ies

0

500

1000

1500

2000

2500

3000

3500

4000

4500 Mean 4.381e­08

Integral 1.118e+05

d = 16 cm

Figure 2.13: ∆t distribution of GSO crystal for d = 16 cm

Mean 4.867e­08

Integral 7.671e+04

t (sec)∆

­0.1 0 0.1 0.2 0.3 0.4

­610×

# o

f entr

ies

0

1000

2000

3000

4000

5000

Mean 4.867e­08

Integral 7.671e+04

d = 68 cm

Figure 2.14: ∆t distribution of GSO crystal for d = 68 cm

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2.4. CONCLUSIONS 19

Mean 5.082e­08

Integral 3.079e+04

t (sec)∆

­0.05 0 0.05 0.1 0.15 0.2 0.25 0.3 0.35 0.4

­610×

# o

f e

ntr

ies

0

200

400

600

800

1000Mean 5.082e­08

Integral 3.079e+04

d = 16 cm, with pinhole

Figure 2.15: ∆t distribution of GSO crystal for d = 16 cm with pinhole

table 2.2.

2.4 Conclusions

Using the TCSPC method we obtained, for the setup at 16 cm with pinhole,a value of (33.72 ± 0.58) ns and (486.5 ± 34.5) ns respectively for fast andslow components, consistent with other measurements in literature [5], butdifferent from the value of 56 ns and 600 ns quoted for instance in [10],presumably owing the different Ce concentration in the crystal. However, asfar as the fast component is observed, the values at 16 cm, 68 cm and 16 cm

distance (cm) τfast (ns) τslow (ns)

1 12.55 ± 0.70 31.11 ± 0.886 27.91 ± 0.12 221.7 ± 5.716 30.96 ± 0.31 234.3 ± 7.0568 31.35 ± 0.31 374.5 ± 8.5

16, with pinhole 33.72 ± 0.58 486.5 ± 34.5

Table 2.2: Results of the fit for GSO crystal

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20 CHAPTER 2. RESULTS

g1 / ndf 2χ 369 / 314

Prob 0.01771

t (sec)∆­0.04 ­0.02 0 0.02 0.04 0.06 0.08 0.1 0.12 0.14

­610×

# o

f e

ntr

ies

1

10

210

310

g1 / ndf 2χ 369 / 314

Prob 0.01771

d = 1 cm

0.70) ns± = (12.55 fast

τ

0.88) ns± = (31.11 slow

τ

Figure 2.16: Exponential fit to data for GSO crystal for d = 1 cm

g6e / ndf 2χ 462.4 / 404

Prob 0.02343

t (sec)∆­0.1 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8

­610×

# o

f entr

ies

1

10

210

310

410 g6e / ndf 2χ 462.4 / 404

Prob 0.02343

d = 6 cm

5.7) ns± = (221.7 slow

τ

0.12) ns± = (27.91 fast

τ

Figure 2.17: Exponentials sum fit to data for GSO crystal and d = 6 cm

Page 31: Time response of a GSO crystal - LHCb Cagliari

2.4. CONCLUSIONS 21

g16e / ndf 2χ 429.5 / 383

Prob 0.05036

t (sec)∆­0.1 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8

­610×

# o

f e

ntr

ies

1

10

210

310

g16e / ndf 2χ 429.5 / 383

Prob 0.05036

d = 16 cm

7.0) ns± = (234.3 slow

τ

0.31) ns± = (30.96 fast

τ

Figure 2.18: Exponentials sum fit to data for GSO crystal and d = 16 cm

g68e / ndf 2χ 202.9 / 204

Prob 0.508

t (sec)∆­0.2 0 0.2 0.4 0.6 0.8

­610×

# o

f entr

ies

1

10

210

310

410

g68e / ndf 2χ 202.9 / 204

Prob 0.508

d = 68 cm

8.5) ns± = (274.5 slowτ

0.31 ) ns± = (31.35 fast

τ

Figure 2.19: Exponentials sum fit to data for GSO crystal and d = 68 cm

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22 CHAPTER 2. RESULTS

g16d2 / ndf 2χ 120.4 / 96

Prob 0.04651

t (sec)∆­0.1 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8

­610×

# o

f e

ntr

ies

10

210

310

g16d2 / ndf 2χ 120.4 / 96

Prob 0.04651

d = 16 cm, with pinhole

0.58) ns± = (33.72 slow

τ

34.5) ns± = (486.5 fast

τ

Figure 2.20: Exponentials sum fit to data for GSO crystal and d = 16, withpinhole

Page 33: Time response of a GSO crystal - LHCb Cagliari

2.4. CONCLUSIONS 23

Figure 2.21: Comparison of time distributions at different distances for small∆t

with pinhole are consistent among each other, indicating that the conditionof single-photon is probably reached.

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24 CHAPTER 2. RESULTS

Figure 2.22: Comparison of time distributions at different distances for large∆t

Page 35: Time response of a GSO crystal - LHCb Cagliari

Bibliography

[1] M. P. Mocci, ”Studio per la realizzazione di un bersaglio attivo polariz-zato magneticamente”, Degree Course in Physics Thesis, University ofCagliari, 2010

[2] C. Vacca, ”Fattibilita’ di un esperimento per la diffusione di neutrinisu elettroni polarizzati”, Degree Course in Physics Thesis, University ofCagliari, 2011

[3] K. Takagi and T. Fukazawa, Appl. Phys. Lett., vol 42, no. 1, p.43, 1983

[4] W. R. Leo, ”Techniques for Nuclear and Particle Physics Experiments”,Springer-Verlag, Berlin Heidelberg, 1987

[5] M. Tanaka et al., ”Applications of cerium-doped gadolinium silicateGd2SiO5:Ce scintillator to calorimeters in high-radiation environment”,Nucl. Instr. Meth. A, vol.404, Issue 2-3, p.283-294, 1997

[6] C. L. Melcher, J. S. Schweitzer, T. Utsu, and S. Akiyama, ”Scintillationproperties of GSO”, IEEE Trans. Nucl. Sci. 37, p. 161-164, 1990

[7] L. M. Bollinger, G. E. Thomas, ”Measurement of the Time Dependenceof Scintillation Intensity by a Delayed-Coincidence Method”, Rev. Sci.Instr., vol.32, no.9, p. 1044-1050, 1961

[8] ROOT, A Data Analysis Framework, http://root.cern.ch/drupal/

[9] EJ-200 Plastic Scintillator, G-tech Corp, http://www.ggg-tech.co.jp/maker/eljen/ej-200.html

[10] R. Y. Zhu, C. L. Woody, ”Inorganic scintillators”, Phys. Lett. B, vol.667,Issue 1-5, p.286-8, 2008

25

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26 BIBLIOGRAPHY