THERMAL CALCULATIONS PERTAINING TO A PROPOSED YUCCA .../67531/metadc... · Prepared by Yucca...

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UCRL-ID-103534 THERMAL CALCULATIONS PERTAINING TO A PROPOSED YUCCA MOUNTAIN NUCLEAR WASTE REPOSITORY Gary L. Johnson Donald N. Montan February 1990 his is an informal report intended primarily for internal or limited external istribution. The opinions and conclusions stated are those of the author and may r may not be those of the Laboratory. Work performed under the auspices of the U.S. Department of Energy by the awrence Livermore National Laboratory under Contract W-7405-Eng-48. i , , ! !'

Transcript of THERMAL CALCULATIONS PERTAINING TO A PROPOSED YUCCA .../67531/metadc... · Prepared by Yucca...

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UCRL-ID-103534

THERMAL CALCULATIONS PERTAINING TO APROPOSED YUCCA MOUNTAINNUCLEAR WASTE REPOSITORY

Gary L. JohnsonDonald N. Montan

February 1990

his is an informal report intended primarily for internal or limited externalistribution. The opinions and conclusions stated are those of the author and mayr may not be those of the Laboratory.Work performed under the auspices of the U.S. Department of Energy by theawrence Livermore National Laboratory under Contract W-7405-Eng-48.

i , ,!

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DISCLAIMER

This document was prepared as an account of work sponsored by an agency of the United States Government.

Neither the United States Government nor the University of California nor any of their employees, makes any

warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or

usefulness of any information, apparatus, product, or process disclosed, or represents thai its use would not

infringe privately owned rights. Reference herein to any specific commercial products, process, or service by

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recommendation, or favoring by the United States Government or the University of California. The views and

opinions of authors expressed herein do not necessarily state or reflect those of the United States Government

or the University of California, and shall not be used for advertising or product endorsement purposes.

i,

This report has been reproduceddirectly from the bestavailable copy,

Available to DOE and DO_ contractors from the '"Office of Scientific and Technical Information

P.O. Box 62, Oak Ridge, TN 37831Prices available from (blS) 576-fl401, FTS 626-8401/

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Prepared by Yucca Mountain Project CYMP) participants as part of the Civilian Radioactive Waste ManagementProgram. The Yucca Mountain Projects in managed by the Yucca Mountain Project Office of the U.S. Departmentof Energy, IAs Vegas, Nevada.

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/

,_ UCRL-ID--103534

DE91 001082

Abstracti

In support to the Yucca Mountain Project waste package and repository

design efforts, LLNL conducted heat-transfer modeling of the volcanic tuff in the

repository. The analyses quantify: (a) the thermal response of a finite size,

uniformly loaded repository where each panel of emplacement drifts contains

' the same type of heat source; (b) the response given a realistic waste stream

inventory to show the effect of inter-panel variations; and (c) the intra-panel

response for various realistic distributions of sources within the panel. The

calculations, using the PLUS family of computer codes, are based on a linear

superposition, in time and in space, of the analytic solution of individual,

constant output point sources located in an infinite, isotropic, and homogeneous

medium with constant thermal properties.

, • .i)..... , •

,,. , L.op.... i:.... _' lr , ....I i,ii (." _""•

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TABLE OF CONTENTS

1. Introduction .................................................................................................... 1

2. Problem Definition ........................................................................................ 3

3. Calculational Models ................................................................................... 11

L.

4. Results ............................................................... 15

5. Conclusions ................................................................................................... 42

References ..................................................................................................... 44

] O

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ACRONYMS

APD areal power density

ARRAYF computer code

BWR boiling water reactor

CDR Conceptual Design_Report

DAYLITE computer code

' DHLW defense high-level wasteFD finite difference

- FE finite elementFIFO first in-first out

GWD gigawatt-days

LLNL Lawrence Livermore National LaboratoryMTU metric tons of uranium ,

ORIGEN computer code

ORNL Oak Ridge National Laboratory

PLUS computer code

PWR power water reactor

SF spent fuel

TWIGS compLJtercodeYMP Yucca ,,,lountainProject

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1. Introduction

Researchers in the Yucca Mountain Project (YMP) are designing an

underground fa_.ility and containers for the long-term disposal of spent nuclear fuel

and high-level radioactive waste, lt is proposed to bury these waste containers in a

mined underground repository in the unsaturated volcanic tuff above the local water

table under Yucca Mountain, Nevada. The underground portion of the repository is

o approximately 1000 ft below the surface and covers approximately three square miles.

This repository is designed to accommodate about 63,000 metric tons of spent reactor- fuel in more than 25,000 containers and about 7,000 tons of vitrified defense high-level

waste (i.e., waste suspended in a glass matrix)in approximately 14,000 packages.

The containerized waste is to be emplaced over a 25-year period. During the first 300

years after the repository is filled, the emplaced waste will deposit ,-,6 GW-yr of decay

heat into the rock. This will raise the temperature of the rock well above ambient

temperature for extended times.r

Lawrence Livermore National Laboratory (LLNL) has been responsible for

designing, modeling, and testing the waste forms and containment barriers. Data from

these efforts will be incorporated in the final waste package designs and

specifications. The current design approach for nuclear waste containment at the

proposed Yucca Mountain Repository makes use of the thin wall of the metalliccontainers as a containment barrier. Ensuring acceptable waste containment periods

with these containers is mainly dependent on minimizingthe corrosion experienced

during long-term disposal. The Yucca Mountain site, with its unsaturated volcanic tuff,

was chosen because it is expected to provide with an environment with little

movement of liquid water, well suited for disposal.

During the period when container wall temperatures are highest (i.e.,

approximately the first 300 years after emplacement), the presence of liquid water nearthe container would increase corrosive degradation of the containment barrier. A

licensing strategy has established a tentative go_,l that 95% of the emplacemento

boreholes have no liquid water in contact with their containers for these first 300 years.

As a goal for our early design analyses, we chose to ensure this "no-liquid"

condition in the heated boreholes by establishing a minimum-allowable borehole wall

temperature of 97°C for the first 300 years. Since 97°C is about the boiling point of

water at the altitude of the underground repository, this will preclude any liquid water

from collecting in the borehole. Two other temperature conditions were also evaluated

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during the early design analysis work to clarily whether the predicted peak

temperature of the power water reactor (PWR) or boiling water ieactor (BWR) fuel

cladding ever exceeds 350°C and whether the tuff temperature 1 m (3.3 ft) from the

borehole wall exceeds 200°C. The 350°C spent fuel (SF) cladding limit is set to

minimize creep in the fuel rod's cladding, which provides another containment barrier

for the radioactive material. The 200°C limit helps avoid stresses in the tuff from 'the

dispersed mineral crystoballte which changes phase and expands by 5% between200°C and 250°C. 1

Previous thermal analyses, documented in the Conceptual Design Report

(CDR) 2, provided some preliminary evaluation of the effects of container load and

spacing with variable areal power density (APD). The CDR thern'lal model assumes

an infinite array of equally spaced and equally loaded containers in boreholes with no

packing or borehole liner. The thermal effects 6re documented in terms of the

temperatures in the mined drifts providing access to the emplaced containers, the

peak cladding temperature of the SF waste, and the temperature of the tuff 1 m fromthe bore_;_olewall. The CDR also documents the results of studies of the effects of

horizontal and vertical emplacement. Some effort was made to model the effect of

heat removal by the ventilation in the drifts. The CDR reports the transient thermal

response during the first 100 years after emplacement. The analyses were done using

the ARRAYF computer code from Sandia along with some simple finite elementmodels.

To support the waste package and reposltory design effort, LLNL has

conducted additional thermal modeling of the repository. This report documents the

results of a series of transient conduction heat-transfer analyses to predict the thermal

response of the tuff. These LLNL analyses quantified: (a) the panel edge and

repository boundary effects if the model assumes a finite repository with each panel

containing a distribution of the same heat sources; (b) the effect of inter-panel

variations by using a realistic non-uniform panel-by-panel distribution of heat sources

(where the modeled sources in any given panel are set equal to the panel average);

and (c) the effect of intra-panel variations by using a realistic distribution of sources

within the panel. These recent analyses are compared in terms of borehole wall (or

inter-panel) temperature variations and determinations of the major contributingfactors to the predicted temperature rises.

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In this study, the PLUS family of computer codes was used to determine the

temperature-time histories from emplacement up to 10,000 years after emplacementfor the rock surrounding the waste containers. Evaluation of the performance limiting

regions can be established by borehole wall temperature distributions at the time of

peak local temperature, at 300 years after emplacement, and at 1000 years after

emplacement.

II

2. Problem Definition

2.1 Panel and Source Description

The calculational models use a "nominal" set of repository dimensions and

waste characteristics. 2 The panel and drift layout in the repository is shown in planview in Fig. 1. The repository conceptual design contains 17 panels. Each panel

contains 10 to 29 parallel emplacement drifts on 126-ft spacings. The major

emplacement drifts contain 75 to 150 SF containers emplaced in vertical boreholes+

spaced up to 15 ft apart along the drifts. Some of these drifts have provisions for, commingling the defense high-level waste (DHLW) in boreholes at midpoints between

SF containers.

In this design, most of the SF containers contain groups of fuel rods

consolidated to twice the density of an intact reactor fuel bundle. Panels 1 and 2 arefilled before facilities are available for fuel rod consolidation. The fuel bundles in these

panels (stored intact from the reactor) have one-half as much SF per container as do

the other panels. Thus, the boreholes in each drift of these two panels are 7.5 ft apart

to give the same local power density as the other panels. There are 340 drifts in this

basic repository layout, containing the equivalent of 24,628 SF containers. Eachcontainer has an average of 2.64 metric tons of uranium (MTU), except in Panels 1

and 2, which have 1.32 MTU per container.

o

The APD is a parameter documenting the average energy deposited over the

entire repository plane, lt includes the effects of drift and panel geometry and

nonstorage work areas, lt basically controls the overall thermal response of the

repository (in particular, the average wall temperature for boreholes in the repository).

A given container's thermal output in addition to the thermal output and the proximity

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(inter-borehole and drift spacing) of its neighbors govern its own borehole wall

temperature.

Because of the relatively low thermal conduct!vtty of the host rock, the short-term

package temperature response (eg., peak cladding temperatule) is determinedprimarily by the container's own thermal output. The waves of heat from neighboring

containers arrive years after the period of peak cladding temperature. Thermal output

of SF waste is determined by its age (time out-of-core) and burn-up (energy output _,

while in the reactor core). Centuries after emplacement, borehole wall temperature

will be controlled chiefly by the spacings and thermal outputs of the array ofsurrounding containers. The burn-up of the SF waste primarily controls Its long-term

thermal output.

2.2 Source Thermal Output ';

The SF waste stream ranges In age from 5 to 35 years out-of-core and In burn-

up from 5 to 60 gigawatt-days per metric ton of uranium (GWD/MTU).3 Figure 2 shows

the distribution in burn-up of the oldest 63,000 tons of SF waste tn the national

inventory. Its average age is 18years and its average burn-up is 33.6 GWD/MTU. By

comparison, the analyses in the CDR usually assumed a waste stream 10 years out-

of-core and with 30 GWD/MTU burn-up.

For this report's studies, the nominal thermal output at emplacement is 3300 W

per package for the consolidated SF and 470 W per package for the DHLW.Packages containing only unconsolidated SF emit one-half of the consolidated value,

or 1650 W. Table I, also derived from Ref. 3 anGthe emplacement schedule from Ref.

4, shows one possible "realistic" emplacement schedule with its wasta characteristics.

In this table, 5 years have been added to the emplacement dates used in Ref. 4. The

SF burn-up, age, and emplacement date are based on a panel average. In reality,

each panel will be filled over a year or two and will contain a distribution of fuel ages

and burn-up. The column labelled "Areal Power Density" gives the initial kilowatts per

acre at emplacement in each panel that would result if ali the SF is 10 years out-of-core.

The thermal outp!Jt from the PWR and the BWR SF derived from ORNL's

ORIGEN calculations,3 is represented in terms of power vs time per MTU at various

burn-ups. For ease of calcLllation, we further normalized the output from the 12 burn--4-

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up ranges (over 20-40 GWD/MTU for both BWR and PWR SF) to a unit burn-up

(Fig, 3). Figure 4 shows the corresponding power curve In terms of watts per canisterfor DHLW.5 In the case of SF, the power output per unit burn-up is approximately

proportional to the age to the minus two-thirds power. The SF thermal output

decreases very rapidly In the early years after removal from the reactor.

2.3 Additional Model Data

The thermal properties of the host rock (i.e., thermal conductivity, k, and thermaldiffusivity, _, of the unsaturated volcanic tuff) are given in the 1985 verslon of the

Keystone document. 6 These values are:

k = 1.84 W/m-K = 0.5608 W/ft-K, and

_: = 8.52 X 10-7 m2/s = 289.36 ft2/yr.

This conductivity is about 10 percent lower than that used in the CDR. 1

An upper limit to a repository-wide APD can be set by varying the container

spacing and loads such that the coolest borehole wall temperature always exceeds

97°C for the first 300 years. However, this would probably result in many containers

whose SF cladding temperature exceeds the 350°C limit. A more acceptable

repository-wide APD could be similarly set such that the average borehole wall

temperature always exceeds 97°C for the first 300 years. But at this APD, there would

be several sections where the borehole wall temperatures are less than the 97°C

desired condition. These overcooled boreholes occur in groupings of containers with

thermal loads well below the mean load (i.e., "cold" loads) or in groupings of

containers located near the edges of drifts or panels in the repository (i.e., decreased

communal warming).

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Table I.

Panel by Panel Heat Source Descriptions

The areal power density is the initial kW/acre if ali the SF Is

10 years out-of-core at emplacement.O

Panel The=ii _¢e LK,tlem i Output 9ynoptlt - _RPRvpotilo_/ I_tt_ I Plus Finlly _iel

(1kit IS In •=|enel•el of MO_tln (ate (itNi/31)ulS/

Unlttl t_tr_turl.i_),ClPo_..Mllenqth,lltlee.Vr ICOnductlvlty.illt-£1dtttuslv ty.tt'71yr

TuI( _il!utlvlty Conluctlvlty |-i|bien|

Prop•rtr. 289,36 0,5600 75 ._ p e n t F u e "1

ai,, X , Zfi 1,,.)mid Ymtd i d ,o, or,ft 8,,,,,.,ot,l.n,,o,o_,,,_,,o_,,,MTU.,,Tu.,. ,.,.e IMtU,,U,Y,,,.it 'Be. Y,,*',.,,1Po.,._. lit ro= lit rol _t row d¢litt tpitlnQ _pic|_q sour(e per drllt per plnel tOn|liner panel lurnip per panel rme enplate_nt tlpllced 8tetslty

_i_U__x_x_a_|x_|_|_x_|_|a_|_x_Qe_v_q|_qx_|_|_u_|_u_g_n__1|=_e_n_|_|_

1 172,5 191B "11,5 10 125 7,50 532,5 11 710 IoJ_1 931,9 16,6 1556_ 1_/I,7 32,5 2004°7 33,12 |4_0,0 2512 -I1,_ I_ 126 1,50 937,_ 125 1675 1,3_1 2146,& 18,5 39/13 1916,1 _0,1 7006,_ 31,6

3 2800,0 _161 -17,5 ?_ 1_6 15,00 1175,0 75 IBO0 2,642 4/55.6 26, 3 125072 1900,8 20,0 7000,8 5],B4 8200,0 3287 -17,5 75 126 15,00 1175,0 75 1875 ?,64? 495]oB _1, 7 147i2& 1908,9 25,4 2010,3 60,3

5 5600,0 3035 -17,5 7] 126 15,00 1125,0 /5 1725 2,6(2 4557,5 32,_ IA7206 1988,1 73,_ ?017,0 65,6i 7000,0 25_1 -17°5 17 1,2 eepl_l 126 15 or 7,5 1125,0 75 or 151 1427 2,619 37_7°B 33,B 174829 19_0,4 ?2.8 201_,2 67,8

&1Al 6485°0 2531 -17,5 6 126 15,00 1175,0 75 450 3,000 1350,0 33,4 45090 1990,¢ 22,8 201302 61,8

6(_1 6B37°5 1775 -17,5 7 6_0 7,50 1175,0 151 302 I,?O0 362,4 33,B 17108 19_ _ 72,8 2013.? 67,0

6ICI 6445,0 1649 -17,5 4 176 15,00 1175,0 75 300 3.000 90n,o 33.4 _0060 199(, 22,0 2013,2 67,86101 &445,0 1019 -17,5 5 126 15,00 1125,0 75 315 _,000 1125,0 33.4 37575 19qth4 22,9 2013,2 67,8

7 8400,0 1775 -17,5 i) i_6 15,00 ii?5,0 75 975 2,647 _516,0 34.6 89128 1992,, _1,6 ?014,5 70,2

8 98_,0 1_49 -17,5 17 126 15,00 1125,0 15 900 2,6B_* 23/7,8 35,5 84412 19_4,8 20,4 2015,2 72,19 10915.0 1901 -)7,5 )B 1_6 15,00 555,0 ]7 518 ?,_42 lJ68,6 3_.8 4_29d 1995,6 19,4 2015,0 72,7

10 _8OO,0 -i]97 -17,5 I0 126 15,00 1125,0 75 750 7,642 1981,5 36.4 72127 1997,6 10,7 2016,5 73,_

II 1400,0 -221q -17,5 17 126 15,00 il25,0 75 1275 ?,642 3368,5 36,5 172957 1999,B 17,8 ?017,2 7A, l12 7000°0 -2703 -11.5 21 126 15,00 1125,0 75 1575 2,647 4161,2 36,5 15100? 2007,5 16.0 2018,5 74°1

I) 5600,0 -3287 -11°5 ?5 126 15,00 1175,0 75 1875 7,682 4_53,8 36,5 180812 2006,3 13,6 201%_ 74,114 4700,0 -3/91 -17,5 ?9 176 15.00 1125,0 15 2175 2,642 5/16,3 36,5 ?09742 2010,1 11,6 202_,7 74,1

15 2800,0 -3791 -17,5 ?9 126 15,00 il75,0 75 7175 2,642 5186o3 3_,5 209742 2013.1 10o5 2023,6 74,=li 1400,0 -3791 -17,5 29 12_ 15.00 1125,0 75 2125 2,6d2 5786,3 36.5 20_742 2015,5 I0,0 20_°5 74, I

17 285,0 -37_1 -11,5 79 126 t5,00 555,0 37 1073 ?,_B? 2834,9 ]6,5 lO]Bl] 2016,_ 10,0 ?026,_ 74,1

•oA • • ma _ @_uu woe um _ amwowe agg • bn o_esaeeneeeete|a p ao e eeq ae a mm ee IIIIIIIMIOIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIII=I IIII llll •II li I a III •• llmmmll I• ) l_llelllllllllallllnlllllnlle mII

,o_,,, .o D H L W ._2o _,.B.. _3_ ?o._2o ,0, .2

"'"X Ym Zm,°-1mid id id _. Or,,t g.r(e rot,len, No,source =,sm_r(e Year.lt A_e°t YearNo, Isr r o_ Isr ro. Isr _o= drift s spictn_ 5paci_ source per drift per pinel ¢o_e eiplace, ••laced• w =xi= • •_e== _| xm• •• _x. • • ••0•_ • • a_•==e|=t===•t _ el | Bl•ac|t|| = msxam • • | a e .#=ms•||_ew• _ml|_u_= • u_e_•_m¢_l=||¢•_e|=u_ n _m =•|a_lm • xwa

_,I, ft,i, n.l, _,i, _,I, _,I, h,l, n,l, n,i, n,i, _,I, n,i,

2 _,1, h,°, _,a, h,a m,i, n,a, h,l, _,a, h,I, .,i, ft,a, til°,

] _00,0 3161 -15,0 4 126 15,00 1140,00 76 304 1914,0 35.0 20#9°04 42_.0 3281 -15,0 9 126 i5,00 1{40,00 76 6fl4 1915,4 35,0 2010,4

5 5600,0 3035 -15,0 9 126 15,00 1140,00 76 684 {976,0 35,0 2011,0

6 _4_1,5 7_31 -15,0 _ 126 15,00 I1_0,00 ?6 456 1978,4 35,0 2013o4

7 8400,0 1775 -15,0 5 126 15,00 1140,00 76 _80 1979,5 35,0 2014,58 9800,0 164_ "15,0 _ 176 15,00 1140,00 76 ' 390 1980,5 35,0 2015,5

9 10qlS°O 1901 _15,0 5 126 15,00 570,00 38 190 1981,? 35,0 2016,2

10 _000,0 -1327 -15,0 B 126 15.00 1140o00 16 304 1981,6 35,0 2016,6II 8400,0 -227q -15,0 5 I?_ 15,00 1140.00 76 380 I_82,5 J5,0 2017,5

I? 7nO0,O -2783 -)_,0 6 1_6 15,00 1140,00 7_ 45_ 1984,4 _B,2 ?018,_13 56OO,0 -3287 -15,0 9 176 15,00 1140,00 76 604 199J,4 26,6 ?020.0

14 4200,0 -3791 -15,0 II I/6 15,00 1_40,00 76 _36 199B,6_ 23,2 2021,8

15 2800,0 -]711 -15,0 II 126 15,00 1140,00 16 836 2000,0 23,0 2023°BI_ IBO0,0 :3191 -15.0 11 176 15,o0 1140,00 16 HS& ?002,9 23,0 20_5,9

II 285.0 -3191 -15,0 II 126 15.00 510,00 ]8 418 2004,4 23,0 2027,4

Se*•O_QIO•. • W••uaaeoauw@x_oaa*ea|x| _aw•o_w@owaw•

Total• lt• 7820 71,1

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Figure 1. The layout of the modeled repository includes 17 panels.

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Figure 2. The distributionin terms of burn-upof the first 62Ktons of SFwaste inventoryrangesfrom 3 to 57 GWD/MTU.

"8"

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Figure 3. The power output of the spent fuel is modeled as a single

curve per unit weight and burn-up vs its age.

"9"

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DHLWPOWER' .......

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YEARSOUTOFCORE

Figure 4. "l'he power output per canister of the DHLW was modeled vs

its age.

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3. Calculational Models

3.1 Numerical Model Requirements

To determine the temperature rise of repositorY rock heated by the energy

emitted from a non-uniform array of nuclear decay ,heatsources of varying age, burn-

up, and emplacement time, our calculational model must include the effects of:

1. The source thermal output nearest the point of interest and the

, sources in neighboring boreholes,

2. Additional sources farther from the point of interest at later times,

3. Variation of each source's output with time,

4. Variation in output from source to source, and

5. Variation in source emplacement date.

Consideration of these effects rule out some common thermal modeling

techniques. One such technique would represent the thermal response of the

repository's host rock and its array of heat-emittlng sources by the response of a

"representative" section of the heat source array. This model would accurately predict

the response everywhere in the repository only if it houses an infinite array of uniformly

spaced, identically loaded sources. One such representative section for this repository

model might be a single container buried in host rock bounded by the planes midway

to adjacent sources.

Finite-difference (FD) or finite-element (FE) numerical methods use this "infinita

array" technique to determine the thermal response at a discrete number of locations

in the representative section for a discrete number of times. Usually only one source is

* modeled when using FD or FE methods. The fine discretization required by these

methods for good accuracy requires an inordinate amount of computer storage spaceand calculational time if more than one source is modeled. In our case where heat

conductir'n is slow and the rate of power deposition drops off rapidly with time, these

infinite al ray models of the repository have been used to predict accurately the

temperature-time histories or steady-state distributions in regions of tuff near the

-11 -

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source being modeled. Experience has shown that the peak borehole wall

temperature occurs relatively soon after emplacement (e.g., 3 - 10 years in our case).

Again, only the local source contributes significantly to the short-term thermal

performance. These discretlzed volume models are especially useful to determine thei

effects of voids in the conduction medium and the effects of temperature- and location-

dependent material properties.

3.2 Analytical Model Description and Limitations

For our study, we have chosen to use a simple, yet powerful, technique to

determlne the thermal response of the repository, lt models the response of the

reposttory's volcanic tuff with itsdiverse array of containerized heat sources by linearly

superimposing, in time and In space, the individual contributions of a series of

constant output sources. The contribution of each source is based on the analytical

solution for conduction of heat from a constant-strength point source into an infinite,

isotroplc, and homogeneous medium with constant thermal properties. The equation

used to evaluate the contribution to the overall temperature change Is

AT = [4_ kr]

where AT equals a point heat source's contribution to the total local temperature rise

at time t and at a distance r away from that heat source of strength Q, initiated at time

to. The ability of the material to conduct heat is defined by its thermal diffusivity, K:,and

its thermal conductivity, k. The par:ameter erfc is the complementary error function.

Solutions embodying this equation are available in the PLUS family of computer

programs. 7 The change in decay heat output with time is modeled by initiating the

heat flow from a package at emplacement, to,o, with a source equal its average

thermal output over some initial time period, Qo. At the end of this initial time period

and at appropriate later times, to,t,additional negative sources of constant strength, -Qi, "

are linearly superimposed on the initial constant strength source to provide the

appropriate lower average heat output over the next time period. A more detailed ..

description of this process in found in Ref. 7. We have used the programs TWIGS and

DAYLITE from the PLUS family oi computer programs.

No voids, such as those representing tunnels or empty boreholes, can be

modeled with this equation. Heat transfer is only by conduction. Neither radiative nor

-12-

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convective heat transfer can be Included, The effect of heat loss/gain by phase

change of the water In the pores and fractures of the tuff also cannot be modeled, This

effect is negligible at short times and less than 10'C at about 300 years,8

3.3 Analytic Model Application

In the repository model, rows of buried waste packages are located Irl the walls

• or floor of a series of underground tunnels (called drifts), These heat-emitting

containers can be modeled by a series of point sources along a finite-length line,

.' These discrete groups of point sources will hereafter be called "line" sources, A drift

containing a series of packages is generally represented by a larger single, horizontal

line source of appropriate length and strength to represent ali the packages containing

the heat sources in that drift, An additional, parallel line source may be added In the

drifts containing commingled DHLW. The depth of the line sources is set to what

would be the midpoint of the vertically emplaced container (i,e., 17,5 ft below the plane

of the repository for SF containers and 15 ft for DHLW), The thermal output from the

SF in a drift or container source is determined by multiplying its age-defined

normalized output (given in Fig. 3) by its total weight of uranium and tts average burn-

up.

The heat sink provided by a constant 25°C earth's surface is modeled as an

isothermal condition 1000 ft above the repository plane, lt can be generated in the

thermal model by creating a "mirror-image" of container sources with equivalent heat-

absorbing strength at 2000 ft above the repository plane and by assuming a 25°C

initial tuff temperature. For model simplicity, we defined each of the mirror-image

panels as an equivalent single line source at the mirror-image-panel centerline.

Modeling waste containers in the repository as drift-averaged line sources is

acceptably accurate everywhere except close to a borehole. When the thermal

- response in the rock near a borehole is to be determined, the heat from the emplacedsources in the local drift must be modeled as a series of vertical line sources, one for

• each container in the drift. Sources in adjacent drifts are far enough away that they

may be represented as drift-averaged line sources. Representation of the entire localdrift as individual container line sources is really not required. Detailed modeling of a

d

few sources on each side of the point of interest is adequate. For our analyses, ali

sources in the entire drift are modeled for input convenience,

13-

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Our analyses look at three distinct vertical emplacement models, In the firstmodel, the "Uniform Source Model", atl containers, (except those stored tn Panels 1

and 2 of the repository) are stored along the drift on 15-ft centers, These exhibit a

thermal Output representing mean age and burn-up (17.9 years out-of-core and 30.8

GWD/MTU for consolidated SF rods), This type of model Is used In the CDR. The

added thermal output of the commingled DHLW is spread uniformly among ali the

repository containers, Panels 1 and 2 are assumed to contain only packages of intactSF on 7,5-ft centers, generating one-half of the thermal output of a mean container of ,,

consolidated SF. Thus, the local power density In ali panels is the same, Ali the

sources are emplaced tn the year 2017 (the middle point of the planned emplacement

period, which Is 2003 - 2027),

The second model, the "FIFO (First in-First Out) Variable Source Model",

assumes the same spacing and emplacement orientation as in the first model.Howevgr, tile SF packages contain fuel with a distribution In age and a burn-up at

emplacement closer to the actual waste inventor./, lt uses the expected Inventory for

the oldest 63,000 MTU from both BWRs and PWRs. The waste stream Is emplaced

oldest first in sequential panels (First In-First Out), filling roughly one panel per year.

A drift may be composed of only consolidated SF on 15-ft centers, or of consolidated

SF commingled with DHLW on 7.5-ft centers, or of close-spaced intact SF on 7.5-ftcenters_ Panels 1 and 2 contain intact SF as In the first model, The first waste fuel to

be emplaced Is older (appr0xlmately triple the age of the last fuel to be emplaced) and

of lower burn-up (less than one-half that of the last fuel). These conditions were

expected to exaggerate the effects seen in the mean thermal load results.

The third model, the "Enhanced Variable Source Model", looks at "heat

tailoring" the emplacemer_t schedule of the waste stream In a given panel. Heattailoring the emplacement schedule arranges for the containers with low thermal

output to be kept away from the panel and repository edges where possible.

Containers of high burn-up fuel are commingled near panel centers with those

containers with lower thermal output. Where the waste stream permits, the intact SF

occuptes the other third of a drift and the commingled DHLW occupies the center twothirds.

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4. Results

The results of the calculations are presented in two formats, The fit ._tpresents

the thermal response as temperature-time histories at selected locations in the

repository, These temperature-time histories document the analyses of both the

Uniform Source Model (SF of mean age and burn-up for ali containers) and the FIFOVariable Source Model (realistic variation of fuel age and burn-up at emplacement),

,w The second format displays the results as temperature distributions for selected panelsat various times and for ali three models,

i,

4.1 Temperature-Time Histories

The temperature-time histories are plotted for locations within or near Panels 1,

6, 9, and 14 for times up to 10,000 years after emplacement. Table II and Fig, 5

provide detailed Information on the respective locations. Locations A, B, and R are

located on the m!dllne between adjacent panels. The other locations, ali at 1.21-ftradius from the center of the nearest source, are Intended to represent the temperature

of an emplacement borehole wall. Locations H, P, and C are located at a panel

center, Locations S and T lie on the panel centerline at panel ends, Where

appropriate, "300 years" after emplacement ttme and the "97°C'' minimum desired

borehole wall temperature level are Indicated.

For the Uniform Source Model, Panels 3 through 17 vary only in size and

location. Thus, variations in their response would result only from dlfferences in their

size and the fraction of their boundaries that lie on the cooler perimeter of the

repository, For the Variable Source Models, the four monitored panels define the total

range of thermal response. Panel 1, with its older intact SF, was chosen because we

expected that it would help define the borehole lower temperature limit in ali models.

Panel 6 represents a mean panel in the repository, Panel 9, located in the farthest

corner of the repository, tracks the effect of a high heat loss at the perimeter of a small

panel with mean power output sources. Panel 14, containing mostly high burn-up SF,

" usually defines the upper temperature limit, ,

The effect of source array size was determined by a comparison of the response

near the source at the center of an "infinite" panel (about one mile square) with that ofLocation C In the "finite" Panel 14. The model assumes uniform sources. Figure 6

shows no perceptible difference for the first 150 years and only a 10 percent

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overpredlction of temperature rise after 1000 years for the "infinite" panel. On panel

boundaries, the difference Is more significant.

As mentioned in the discussion on calculatlonal methods, a set of negative

source, mirror-Image panels are included In the model to simulate the effect of the

isothermal conditions at the ground surface 1000 ft above the repository, To check the

effect of including this isothermal ground surface, we ran a calculation on the uniform

source model with the repository mirror sources removed, The result, shown in Fig, 7,Indicates that including the isothermal earth's surface In the model ts important only at

late times after emplacement, We kept the mirror source array in the model because

its presence did not significantly increase the computation time, This calculation

comparison also suggests that possible heat removal by the water table 700 ft below

the repository would similarly be of concern only at late times after emplacement (i,e, >

1000 yr),

,For our Uniform Source Model (uniform power density, age and burn-up)In a

finite repository with individual panels, Tables III(a) and III(b) gives the temperatures'

(1) at peak temperature conditions; (2) at 300 years after emplacement; and (3) at

i000 years after emplacement. Plotted temperature-time histories are given in Figs. 8

to 11. These analyses show the following results at 300 years after

emplacement.

1. The borehole wall temperature in the repository ranges from 55 to 125°C.

J

2, The borehole wall temperatures near the center of most "full-sized"

panels are greater than 97°C, Most of the boreholes in Panels 1 and2drop to below the 97°C limit.

3. In Panels 1 and 2, the panel center temperature is 27°C cooler than the

panels containing the youngest, hottest fuel.

4. In Panel 6 (the "average" panel in the repository), the borehole wallw

temperature might vary by as much as 60°C between the coolestborehole and the hottest,

5. The temperatures for points between the panels rise very slowly. They

' reach a peak of less than 80°C well after 300 years.

16-

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6, At the time of peak temperature rise, about 70% of theborehole wall

temperature rise is due to the source in its hole, After 1000 years, only

10% of the rise is due to the output of its local source,

7, Emplacement of the sources in the repository over a 25-year period does

not significantly affect the characteristic borehole wall temperatures at

300 years. At this late time, when sources in most of the repository

contribute to the local tuff temperature rise, conditions are changtr,g so

slowly that the few years difference In emplacement time Is Insignificant,,b

The temperature-time histories also show a maximum 100°C difference in peak

borehole wall temperature. The peak borehole wall temperature occurs shortly afteremplacement.

One current SF baste disposal plan assumes that the oldest SF in the waste

stream will be emplaced in the repository first (as in our FIFO Variable Source Model).

The back-log of the older SF temporarily stored at reactor sites would be dissipated

until an approximate steady-state influx of the younger, more recent fuel waste stream

is reached. In this scenario, the first waste emplaced will be three times older than the

average and about one-half the burn-up of the last emplaced waste. The expectedconsequences of including this distribution of emplacement sources on the thermal

response of individual panels exaggerates the results discussed previously.!

The result_ for the FIFO Variable Source Model analyses are plotted in Figs. 12to 15 (see also Tables III(c) and III(d)). Review of the temperatures at :300 years

after emplacement shows the following results.

1. The resultant hottest borehole wall for this emplacement scheme has

increased by 11°C while the coolest has decreased by 19°C. This

increases the borehole wall temperature range by 47% (42 to 136°C

° compared with 61 to 125°C for the Unff')rm Source Model).

2. Ali of Panels 1 and 2 and much of Panel 9 drop below 97°C. For Panels

6 and 14, only edges and corners drop below 97°C.

3. The representative panel (6p) has a 53°C variation in borehele wall

temperature.

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4, Panels with the same spacing, layout, and average burn-up give the

same long-term thermal response regardless of age of fuel.

During the perlod of peak borehole wall temperatures, boreholes tn Panels 1

and 2 are lower by up to 83°C from the uniform source case. In Panels 6 and 14, the

highest and lowest values of peak borehole wall temperature from the unlforrn source

case have changed by -10°C to +25°C, respectively. ,,

-18-

•,_ - ii ......... i,,, ........o,,...........-.................]111.........................................

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Table II.

Locations where Time.Histories are Described

lD Panel No, Location within Panela Remarksi , , i i i ' d , i ii.,.i ,...li f li i, i .......

A Betw, 4 & 14 Inter-panel main drift Hot panel

d B Betw, 14 & 15 Inter-panel aux,drift Hot panel

C 14 Panel center Hot panel ,

. D 9 End of edge drift Exposed panel

E 1 End of edge drift Intact SF only

H 1 Panel center Intact SF only

P 6 Panel center Average panel

Q 6 End of middle drift Average panel

R Betw. 5 & 6 Inter-panel aux, drift Average panelS 6 Middle of central drift Average panel

T 6 M!ddle of edge drift Average p_,nel

U 6 End of edge drift Average panelV 6 End of central drift Average panel

a Within panels, the actual location is at the borehole wall radius from the centerline of

the nearest source (1,21 ft),

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Figure 5. There are 13 locations where temperature.time history results

are described (see Table II).

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Table III(a)

Temperature Resultsfor Uniform Source Model / cases "ac"

Panel Source Peak Time of Temperature TemperaturelD Location Temperature Peak @ 300 yr @ 1000 yr

..... (°C) Temperature ...... (°C) (°C)

,p 1 H 162 19 98 98

1 E 110 7 61 49

9 D 147 4 68 518

14 C 193 13 125 99

4, 14 A 64 1000 57 64

14, 15 B 78 1000 73 78

J

Table III(b)

Temperature Resultsfor Uniform Source Model / Cases "6p"

Panel Source Peak Time of Temperature TemperaturelD Location Temperature Peak @ 300 yr @ 1000 yr

(°C) Temperature..... (°C) (°C)

6 P 212 30 135 101

6 Q 167 20 105 91

5, 6 R 77 1000 74 776 S 202' 20 105 84

6 T 202 19 103 76

6 U 163 22 75 60

6 V 168 20 87 77

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,J

Table III(c)==

Temperature Resultsfor FIFO Variable Source Output / Cases "be"

,, Panel Source Peak Time of Temperature TemperaturelD Location Temperature Peak @ 300 yr @ 1000 yr

........... (°C) Temperature ,(°C) (°C)........

i 1 H 80 25 59 46i 1 E 59 10 42 37

i 9 D 164 7 72 53 "

J 14 C 219 16 136 107i'

,, 4, 14 A 63 1000 57 63

" 14, 15 B 85 720 79 85

i

i Table Ill(d)

" Temperature Resultsi, for FIFO Variable Source Model / Cases "p6 '°I'

' Panel Source Peak Time of Temperature TemperaturelD Location Temperature Peak @ 300 yr @ 1000 yr

,, (°C) Temperature ,, (,°C) (°C)'i

L

, 6 P 191 30 127 99

, 6 Q 152 20 98. 88

'_ 5, 6 R 75 1000 67 75

6' S 199 20 102 76

6 T 187 19 101 83

6 U 151 22 83 76

6 V 162 20 74 60 ,._=.

Q

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2,t_,_...... t'" v - _ l' " t v _-_--v T:- _-i _ -- v .... ] "' v ........I -- l_ - T''--]- V- - I _ "1....e

220

0 4' 4" _.

120 .

or"

I-- 100

80 -n

t--- 6O

- ----POINT "C"

_°-_l _ + + "INFINITE" ARRAYL I .... J _ _ _. I j ....j J J J. i .. _J_. l .... J i_ I, , ,I , I,,, I , i __i

oI so too _oo 3o_ 400 soo 600 _ 800 900 iooo

EbIFLACEMENT YEAR S

11

Figure 6. The effect of using a "finite" array of sources, such as inPanel 14, vs a simulated "infinite" array of sources is

noticeable after 300 years of emplacement.

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UCED 'P T "A" B-_- _, COOLING PROD AT OZN Y AN -

_. ___ 020 FT, •

,, ,

w _U _ -5

_ oW __ F. _ o_

_ | ,

w _

-i_

w

_-ll

-14 -

, J ......i .1. 1 L l , -J .... A, ' I ..... I , 1 1 1 l l__oI 5o0 Ioo_ 2ooo 3_o 4ooo _ooo _ooo 7ooo 8r,,x)o aooo toooo

EMPLACEMENT

YEARS

Figure 7. The effect of using an equivalent _,ink, mirror image of the

repository sources to model an isothermal ground surface isnoticeable 1000 years after emplacement.

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40 30_ yrA/LL-ILL

2O

0 50 I00 200 300 400 50(3 600 100 800 900 IOCX3

EMPLACEMENT YEARS

Figure 8. Uniform source temperature.time histories; Panels 1, 9, and 14.

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Figure 9, Uniform source temperature-time histories; Panel 6.

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w Un,Form Source Model': Panels I, 6, ILl- Ceqtral Borehole

220 I-'''' i _''"'"-i'' "'' I _ "' i I i'"_ f I i ' ' ' lJ"ill ii ' i"i"i--ri-,-l'Ji',r-r--l'_i - Locat,onlPanel ID

200

18o -_

j"\_.., _"'

©i.- 120 .-.-I

o -1

ioo 97 °C

i- 80 ,.__

60 yr' "

'i

20 I I I t I I l._t._l i 1. i l I l I. i_J i l } i.li,,liiii,t 1 , i i , I.J l,,l I IZt

0 50 I00 200 30_ 400 500 600 "/IX) 800 900 I(.00

EMPLACEMENT YEARSo....

Figure 10. Uniform source temperature-time histories; Panels 1, 6, and

14; centers.

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Un,f'orm Source Model: Panels I, B, 9 -Parl(';I Corner/ReIDo',s_lory I[:1(;_,; t:t,"t

220, _--r_, ':i '''' T"-T'-': _ :':_:i _r_-r-_-._.-T-_-_...F-r_T-r_._-_-_--r-_.-[_-r--_-T_r-_-r_`_._-r--_-._r._. i!]-- Location/Panel lD 1200, -- -

180 .......

160......U

(_

140

120 --

o

_- U _,_ loo '.,../6 97 °C -_

....,:?.

60 _t E/1 "--<--_l-I

40 ,,}'J- 3{_ )Jr --.

LI \"2O

0 50 100 200 300 400 SOC) _ "tO0 800 900 IOOO

EMPLACEMENT YEARS

Figure 11. _,trliform source temperature-time histories; Panels 1, 6, and

9; edges.

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F[FO Var,able Sour ce Model_ Panels 1, 9, 1_t

220 "-" _'kT --r--T--r-'r--T--rT,, I I, i r---[--r-'1--T-",'--Ir-r-- r-.r-r--r--r-r-_- r-.-r_-r-_-r-r--T-F-r-r-_r-T-_-r-T-,-

_"_ - _, IPO V_,lt_llp _¢0 Pl¢<lill Pit, Iii I, I, Iq "

\200, - ---

' _l_

180 ..... k

" \ Locat,on/f'anel I D i,-.- , i o Ii _

- "\, i '® -

EJ 140 -"

_] ....._-- II Ii ii tl 1t n II 1 K I1 II120, \ ---

- \\0/9 _____

100. 97 °C¢_E ",\,\

_- t H/I "x...., -"--.... -.......____ o/i t'}- 15

A/Lt I'Lt _

60, :.rSl_, // .... -- .._.._.__.=..__= _

3[_ yr

it. ,,2O

0 SO I00 200 300 400 500 _ "tOO 800 900 IO00

EMPLACEMENT YEARS

Figure 12. FIFO variable source temperature.time histories; Panels 1,

9, and 14.

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FIFO Var c_b e Source Model' Reference P(.)nel No. 6

220 ._---r-_--r--_T'_--T--T--T"_--r-"T'--r'-T-m--'r---r-'T--]--r-,'--r ---,--]---T---r-'-_--r.......l--r-',"T- 1--r'-r-- ,--"T--l---r---_---r---T'--i- r--r--'r'"T ]" Loca}_on or "Panel 6 " " ,........... ,..... "*................. .° , "

l2o0 S...-_......................., --_-.....-- J

18o _ t,,,_,,o .......-_::_:: w £

160 ' i" _.

(.-,3 ,

140 ,o ,::z..-:T_..!.-T:_ :_,..,___:::Z,::_,\:2:'_I"Z.,-_.\-/.............. -

120

13 \\v"-.... "'-..b--..

F.- 80 - -.... "................

.q

60 - ...z-- 3_fJ ×r" 1

/ -I

40 --

01 50 I00 200 300 400 500 600 'TOO 800 900 100(3

EMPLACEMENT YEARS

Figure 13. FIFO variable source temperature-time histories; Panel 6.

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FIF0 Var ,able 5ourc;e Model: Panels 1, 6, ILl - Central Boreholes

220, _ITr-"T"-T'_I'_---,I l i I'i-F-r--,-r-r-Fr-_--l--,--F-r-r-'T-r-l--i--r-v--l-T-r-'r-r-r-T"_ *-i_i_:_i _ FT-I"-ll--I-[ '

k Location/Panel lD

• \ !, _ao -L

_-_,14o p_ --"---,,. / ) ..........

(ii 'T" ........... -i,_.

._, 120 . "......

I

BO

;ooYR

20 i , I I ,, ._ I l J _J J i J__l_I I 1 i i , i I l.I ±_i_ 1 ,, I .L.I i_li ii. , _1..k..l J_ i JJ _i0 SO I00 200 300 400 SO0 600 100 800 900 I000

EMPLACEMENT YEARS

Figure 14. FIFO variable source temperature-time histories; Panels 1,6, and 14; centers.

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F[FO Var',abl(_ Sour'ce Model: F:'i-_rl(_,l!:_ I, Ii, 'J P',_:)r')(:l Ot_rl',l._r/R_I_(_!_, t, _y td!_('

220 "l-'r'-r-'--l'-'-t-'-'T-'r-T-"-'"'T -'-_'''''_' -1-" " "* '[ _'' " I"' T "'"l""r " ""I _' *' _'-' f "' ' ' l.- I.i.)(;i:_f , ()f_/f-_' jr_(-_l I(I

' 200 *--

180 _---

--_160

c__)40

cUk,..

._ 120o&...

c_ 100

E "\,,0

80•:::QTL'._2II--..........

..... • tj/Ii.. .,1 V..ili/.112"ili i/;i.................................................................................60 ...........

................................................................ t;/l40 -" 300 YR .............................................................................................................:"

om 60 ioo 2oo _oo ,oo _o 6oo 7oo _oo 9o0 jooo

EMPLACEMENT YEAR S

Figure 15. FIFO variable source temperature-time histories; Panels 1,6, and 9; edges.

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4.2 Intra-Panel Temperature Distributions

After examining the temperature-time histories of "representative" points

discussed In the Section 4,1, we examined the temperature distrlbutlons of

"representative" panels at particular fixed times, Temperature distributions tn thecenturies time frame is of Interest from the standpoint of containment of radioactive

materials In the repository,w

An example of the borehole temperature distribution along an emplacement,, drift Is shown In Fig, 16, These curves present the temperature conditions at 1000

years after assumed repository closure, They occur In one of the warmest places In

the repository, I,e,, the middle drift of Panel 14 which contains point "C", The mc_el

generating the first curve (smooth) assumes ali 75 of the packages contain the sameamount of SF, 2,64 MTU, In a more realistic situation, about 20% of the packages may

contain unconsolidated SF and, thus, generate 33% to 50% as much heat as the

consolidated fuel containers In the drift, In this case (shown by the second curve In

Fig, 16), every fifth package contains 1,2 MTU while the remaining 80% contain

3 MTU, The average remains 2,64 MTU, For the drlft.,averagedcase, only one or two

packages at tile ends are below the boiling point of water (about 97'C at the repositoryelevation) fqr the uniform source case, For the case with dispersed Intact SF, five to

seven packages on each end fall below thts temperature,

Panel 6 was chosen to Investigate the edge effects of finite panels, non-uniform

source output distribution, and heat-tailored emplacement on borehole wall

temperature distributions, This panel Is of average size, stores average burn-up

waste, and is located near the middle of the repository, lt uses 17 of the 19

emplacement drifts, storing 1425 SF containers loaded with an average of 2.64 MTU

(i,e,, 3 MTU In consolidated SF containers and 1,2 MTU in Intact SF containers) and456 containers of DHLW, The SF consists of 80% consolidated fuel containers andv

the remaining 20% Intact fuel assembly containers, The first six emplacement drifts

contain consolidated SF commingled with DHLW, The intact SF containers are storedO

on 7,5-ft centers in Drifts 7 and 12, Drifts 8 through 11 and Drifts 13 through 17 store

only consolidated SF. The layout is shown in Fig. 17,

Isotherms of the borehole wall mldplane temperatures at 300 years after

repository closure for the Panel 6 array of SF sources are shown in Fig. 18, The

contributions of the DHLW heating are Included In the thermal load calculations, The' - 33-

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shaded portion of the drift shows the part of the panel where the borehole mldplanetemperatures at 300 years are less than 97°C, The lower temperatures for the two

drifts contalnlng Intact SF only (Nos, 7 and 12) are cbserv_:l_:_. The containers near

the ends of a large number of drifts in the middle of the panel fall below the 97°C limit,

especially near the "Intact SF" drifts and at the panel ends,

At any given time, the fraction of boreholes with temperatures less than 97°C Is

very sensitive to the assumed conductivity of the tuff, Temperature distributions for this

source layout were calculated at 200, 300, 500, 700, and 1000 years after closure to

determine the fraction of the boreholes with wall temperatures below 97°C, The

results of these calculations are plotted In Fig, 19 for the three package types and theoverall value, The most obvious feature in this figure Is the high percentage of DHLW

packages with borehole wall temperatures below 97°C, Also, after 200 years, morethan 10% of ali the boreholes are cooler than 97°C, At 300 years, this percentage has

risen to 15%, and at 1000 years nearly ali the boreholes In the panel are less than

97°C, The fraction of boreholes greater than 97°C Is extremely sensitive to the

assumed value of thermal conductivity of the tuff, A variation of 10% In the value used

by these analyses (k=1,84 W/m-K) can vary that fraction by a factor of two or more,

We ran an additional model where the source distribution Is arranged to keep

as many boreholes as hot as possible for as long as possible (I,e., heat-tailored

emplacement), In this arrangement (Fig, 20), the low output sources are Isolated from

the panel edges as much as possible, The layout is symmetrical with Intact SF

occupying the center third of a drift, alternating with DHLW occupying the other two-

thirds of a drift. The results of the thermal calculations are shown in Figs. 21 and 22.

They show a marked reduction In the number of containers occupying boreholes with

wall temperature below 97°C, The fraction below 97°C, for this configuration, Is one-

half that for the previous layout up to about 400 years after emplacement. This

suggests that, given the real Inventory, the early storage period temperatures of thelt

low power boreholes could be kept acceptably warm by emplaclng them near the

centc_rof the panel, The fraction of boreholes with temperatutqs less than 97°C could

be further reduced by decreasing the Inter-container spacing tn the drifts near the "panel corners,

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Figure 16. Temperature distribution along a drift.

•,35-

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_.................................................................... _ ...............Con .,-,,-,I d,-+1 ,_,J S F,.j. L

, [C O_;_-blJdEutll

y [::- ..... .x<:'----. "':': '.: .:- ..... -_'-: :-' ...... <'" ::. " :__ :_: :: " +,:' j

I..71 I::1 l_::J 1::3 13 1".'3 I':.:] [--3 L--'-'JI::J 13 I'::.| I::] [..',1 [ .I (" J [:::1 I:::1 I ::] I.::J

Figure 17. Source layout for the FIFO variable source case.

- 36 -

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Figure 18. Isotherms for the FIFO variable source case.

37-

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o!

EMPLACEMENT YEARS

Figure 19. Fraction of boreholes below 97°C at various times after

' emplacement for the FIFO variable source case.

38-

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(lr"II I .....:-:..............'......................-T............= .......................'-:U' _ _ i: ,__[)I-II..tjcorr)Jn!7etI

i..........:.........,':'.";-.-::':::...................•....-::.-._;---:.;:==-........' ':-:.....=:" crillso I_daIed.S [:

It.:lose ,.:.-i,+ --,1:ac ecl I

", ,3"Is' )- . ....

't _............. ._.E--._-_.-_ -:-£:.--:-.-:_..-_..........

' R ,..l _ ..... -.:::_ -_ -.. [:_ .......... .-,::.::- ,

JLI ' - .....;:;-...... _.-.:x::]£.:-x-...._:I(,.-x:._--.$ .......... '

li '-:...........-::-:_................................................._:=:---.......

.... I_.2£........ ...................,":, i':""::. " ::.: .......::':::--::: --_,:-:v:::.u.:-:',..Jr :'_" -1..,'-:'v -'lr ............................ :j

I _ l: . ::. : :: : ' : : . . ... ........... ::::::::::::::::::::::

I _1 ¢ "-- .... r........... : ................. :::::::::::::::::::::: ::-'-_

I Cl I " :: ........ 1

z'7..................................-:.........S ............................................::V," " 1 1 li_'

(..J C .J l I I .I 1. ) (') I ',1 I. J 1.++1 L I I+ ) i_::l I. I L_.I I:::) I. I I++.1 {+.1 I,+;_.](+ I

r..J c: J c-.l l:.l l i r:.l (.-:i I::_ L'.J (:::_i 1::) _::.l '_-.l £ :l E:-] 1.:::] L:._ .c:..-_lL:;I r:J

Figure 20. Source layout for the enhanced variable source case in

a panel.

39-

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9

10,q

II ' H-

12 o

13

14

15

0

16

17

PANEL6 - 300 YEARS AFTER CLOSURE

Figure 21. Isotherms for the enhanced variable source case.

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lP

Figure 22. Fraction of boreholes below 97°C at various time_ afteremplacement for the enhanced variable source case.

-41 -

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5. Conclusions

To support the Yucca Mountain Project nuclear waste disposal package and

repository design efforts, LLNL has modeled conduction heat-transfer of the nuclear-

decay-heated volcanic tuff In the repository, These analyses extend the analyses

documented In the CDR by quantifying the thermal response for a finite, uniformly

loaded repository with each panel containing a distribution of the same heat sources;

the response for a realistic panel-by-panel distribution of heat sources (where the

sources in a given panel have been averaged to some uniform value) to show the

effect of inter-panel variations; and the Intra-panel change In response for various

realistic distributions of sources within the panel,

For this study, the tuff's response to the heat sources In the repository Is

modeled by linearly superimposing, In time and in space, individual contributions of an

analytically defined series of constant output point sources located In an Infinite,

uniform, and constant property medium. No voids, such as drifts or emptty boreholes,

are modeled. However, the "constant temperature" surface 1000 ft above the

repository is modeled. Heat transfer is only by conduction.

Calculational results show that the effect of using an infinite array model to

predict the local temperature rise in the center of finite-size panels In the repository is

barely perceptible during the first 150 years and only 10% high after 1000 years. Thisq

error would increase substantially near the ends of drifts and edges of panels.

For the case of a finite repository model with uniform power density, age and

burn-up, the following conditions are observed at 300 years after emplacement.

Although the borehole wall temperatures near the center of most "full-sized" panels

are greater than 97°C, most of the boreholes in Panels 1 and 2 drop to below the 97°C

limit. In an "average" panel, the borehole wall temperature can vary by as much as

60°C between the coolest and the hottest borehole. At the time of peak borehole wall

temperature (,..20 years after emplacement), there is up to 100°C variation in the peak

borehole wall temperature in a panel. At this time, about 70% of a borehole wall's ,_

temperature rise is due to the source in its hole. After 1000 years, only 10% of this

temperature rise is due to the output from the source in its borehole.

Assuming an emplacement schedule where the oldest SF from the actual

expected waste inventory is emplaced in the repos{tory first, the following thermal

-42-

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response is noted at 300 years after emplacement, The hottest borehole wall for this

emplacement scheme has Increased by 11°C while the coolest has decreased by

19°L,, which Is an Increase of 47% In the borehole wall temperature range. A

representative panel has a 53°C variation In borehole wall temperature° Many more

boreholes than the uniform source model have predicted temperatures less than 97°C

at 300 years, Thus, although only the load of an isolated borehole need be used to

predict Its peak borehole wall temperature, the actual emplaced Inventory In the, repository should be used to predict whether a given borehole will remain above the

unconfined boiling point at 300 years.W

Finally, calculations for a representative panel Involved determining

characteristic intra-panel borehoi_'_temperature distributions at 300 years after

repository closure to detail the local effects of finite panels, non-uniform source

distributions, and heat-tailored emplacement layout. The model includes detailed

descriptions of drifts with commingled consolidated SF and DHLW and drifts with intact

SF only, The containers near the ends of a large number of drifts In the middle of thepanel fall below the 97°C limit, especially near the "intact SF" drifts. Also, a high

percentage of DHLW packages have borehole wall temperatures below 97°C. At 200

years after emplacement, greater 'than 10% of ali the boreholes are cooler than 97°C.

At 300 years, this percentage has risen to 15%. At 1000 years, nearly the whole panelIs less than 97°C.

Altering the source distribution to keep as many boreholes as hot as possible as

long as possible (heat-tailored emplacement) results In a marked reduction in the

number of containers occupying boreholes with wall temperature below 97°C. The

fraction below 97°C, for this heat-tailored configuration, is one-half that for the

untailored layout up to about 400 years after emplacement. A relative variation of 10%

in the thermal conductivity of the tuff can vary these fractions by a factor of two or more.

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ReferencesJ

1, Site Characteristic Plan, Yuoca Mountain Site, Nevada Research

and Development Area, Nevada, Volume III, U, S, Department of Energy,

Office of Civilian Radioactive Waste Management, DOE/RW-0199, 1988,HQ0,881201,0002

2, SNL (Sandia National Laboratories), Site Characterization Plan

Conceptual Design Report, SAND84-2641, Sandia National Laboratories,

Albuquerque, NM, 1987, NNA.880902,0014, NNA,880902,0015, V

NNA,880902.0016, NNA,880902.0017, NNA,880902,0018, NNA.880902.0019

/

3. U.S. Department of Energy, Integrated Data Base for 1987: Spent Fuel

end Radioactive Waste Inventories, Projections, and Characterlcts,

DOE/RW-0006, Rev, 3, Oak Ridge National Laboratory, Oak Ridge, Tennessee

(September 1987), NNA,900403,0377

4, DOE (U.S. Dept. of Energy), Mission Plan, Office of Civilian Radioactive

Waste Management, Washington, D,C., 1985, DOE/RW-0005 (Table 2-2).NNA.870519.0050 "

5. Baxter, R.G., Defense Waste Processing Facility Wasteform and

Canister Description, Savannah River Plant, SC, 1988, DP-1606, Rev, 2

(Table 19). NIVA.890327.0057

6. F.C. NImic, S. J. Bauer, J. R. Tillerson, Recommended Matrix and Rock

Mass Bulk, Mechanical, and Thermal Properties for Thermal,.

Mechanical Stratigraphy of Yucca Mountain, Sandia National

Laboratory- Albuquerque, NM, Keystone Document 6310-85-1, 1985.NNA.891129.0284

7. D.N. Montan, The Plus Family . A Set of Computer Programs to _'

Evaluate Analytical Solutions of the Diffusion Equation, Lawrence

Livermore National Laboratory (University of California), Livermore, CA, UCID-

, 20680, February 1986. NNA,900430.0044

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8, J,J, NItao, Numerloal Modeling of the Thermal and HydrologloalEnvironment around a NuolAar Waste Paokage using the EquivalentContinuum Approximation: Horizontal Emplaoement, Lawrenoe

LivermoreNationalLaboratory(Universityof California),Livermore,CA, UCID.21444, 1990, NNA,890317,0021

W

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Appendix A

This report does not use any Information from the Referenoe Information Base nor

contain any c,andldate Information for the Reference Inforrnatlon Base or tile Site and

Engineering Properties Data Base (SEPDB),

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i

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