Structure and Interactions of Nuclear Matter (99.95% of ...

46
Nuclear Science Objectives of Basic Science: • Structure and Interactions of Nuclear Matter (99.95% of visible) Æ complexity and synergy emerging from simplicity Applications: Æ complexity and synergy emerging from simplicity • Synthesis and Transformation of Elements 1 ations Life science (nuclear medicine, diagnostic imaging, pharmaceuticals, therapy) Materials science Applica Materials science Cosmology (chemistry & physics) Environmental studies Earth and planetary science Earth and planetary science Separation technology Hot-atom chemistry Nuclear forensics W. Udo Schröder, 2007 Nuclear forensics Advanced nuclear power generation/transmutation

Transcript of Structure and Interactions of Nuclear Matter (99.95% of ...

Page 1: Structure and Interactions of Nuclear Matter (99.95% of ...

Nuclear Science

Objectives of Basic Science:

• Structure and Interactions of Nuclear Matter (99.95% of visible)complexity and synergy emerging from simplicity

Applications:

complexity and synergy emerging from simplicity• Synthesis and Transformation of Elements

1at

ions

Life science (nuclear medicine, diagnostic imaging, pharmaceuticals, therapy)

Materials science

Applic

a Materials scienceCosmology (chemistry & physics)Environmental studiesEarth and planetary scienceEarth and planetary scienceSeparation technologyHot-atom chemistryNuclear forensics

W. Udo Schröder, 2007

Nuclear forensics Advanced nuclear power generation/transmutation

Page 2: Structure and Interactions of Nuclear Matter (99.95% of ...

Applications of Nuclear Instruments and Methods2

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 3: Structure and Interactions of Nuclear Matter (99.95% of ...

Nuclear Magnetic Resonance Imaging (MRI)

• 1.5T, MasterQ Body Coil

Magnetic Resonance Angiogram

• Q-Body Coil• 3D T1-FFE• Low-high profile order3

atio

ns

• 50 x 1.6 mm slices oc.• 512 x 196 matrix• FOV = 400 x 320 mm• TE / TR = 1.3 / 5.0 ms

Applic

a TE / TR 1.3 / 5.0 ms• WFS = 0.9 pix (± 62 kHz)• Flip = 35°

18 seconds Breathhold• 30 cc Gadolinium @ 2cc/sec• 30 cc Gadolinium @ 2cc/sec.

18 Second MRI image!!

W. Udo Schröder, 2007

Page 4: Structure and Interactions of Nuclear Matter (99.95% of ...

Radiation Detectors for Medical Imaging

P it i i t hi (PET) i t l li th h ti t’ b i

Positron e+ (anti-matter) annihilates with electron e-

Positron emission tomographic (PET) virtual slice through patient’s brain

annihilates with electron e(its matter equivalent of the same mass) to produce pure energy (photons,

rays) Energy and

4at

ions

γ-rays). Energy and momentum balance require back-to-back (1800) emission of 2 γ-rays

Applic

a

e e 2 (511 keV )γ+ −+ →

( ) γ yof equal energy

e e 2 (511 keV )γ+ →

W. Udo Schröder, 2007

γ detectors (NaI(Tl))

Page 5: Structure and Interactions of Nuclear Matter (99.95% of ...

Positron Emission Tomography

After

Positron emission tomographic image of the heart

After administration of radioactive water: H2

17O to

5at

ions

2blood flow, after infarct episode

blood flow

Applic

a blood flow

After administration of radioactive acetat: 11CH3COOX

W. Udo Schröder, 2007

metabolism

Loveland, Morrissey, Seaborg

Page 6: Structure and Interactions of Nuclear Matter (99.95% of ...

DNA Analysis

DNA sample decomposed into single strands into single strands, cut by enzymes into pieces, use electrophoresis to separate according to size,

6at

ions

p g ,React separated segments with radio-labeled probe protein sequences,identify by auto-radiography

Applic

a identify by auto-radiography

W. Udo Schröder, 2007

Page 7: Structure and Interactions of Nuclear Matter (99.95% of ...

Applications of Nuclear Instruments and Methods7

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 8: Structure and Interactions of Nuclear Matter (99.95% of ...

Nuclear Batteries with Really Long Lifetimes

Nuclear battery: a radioactive source placed inside a capacitor emits αpparticles, which build up an electric charge on the plates, or deliver an electric current

8at

ions

electric current. Such batteries can operate for long durations, a major fraction of a century (e.g.,

Applic

a

t1/2=86 a) and can be made small enough to be used in implant pace makersmakers.

W. Udo Schröder, 2007

Page 9: Structure and Interactions of Nuclear Matter (99.95% of ...

Cancer Treatment with Neutrons

Patient treatment station

9at

ions

Cyclotron accelerates protons, which generate a

Applic

awhich generate a well defined secondary beam of neutrons with variable energy and range in tissue.

W. Udo Schröder, 2007

Treatment success rates of neutron and gamma irradiation

Page 10: Structure and Interactions of Nuclear Matter (99.95% of ...

Radio Therapy

Heavy ions (here 12C) have a well-defined range in defined range in materials. They lose much of their kinetic energy sho tl befo e

10

atio

ns 12C Beam

12GeV

shortly before complete stopping, leading to a radiation dose

Applic

a 12GeVconcentrated at the end of their range. This provides a non intrusive non-intrusive surgical tool

W. Udo Schröder, 2007

Page 11: Structure and Interactions of Nuclear Matter (99.95% of ...

Applications of Nuclear Instruments and Methods11

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 12: Structure and Interactions of Nuclear Matter (99.95% of ...

Rutherford α Backscattering

Backscatter energy

m M

12

atio

ns

0 4m ME(180 ) E α

mα M

Applic

a

( )0

0 2

00

E(180 ) E1 m M

M m E(180 ) E

α

α

α

= ⋅+

→ ≈

W. Udo Schröder, 2007Target Material Mass Number A

Page 13: Structure and Interactions of Nuclear Matter (99.95% of ...

Thickness of Thin Films

Probe particle (α) loses energy ≤ ΔE in

0M 0E(180 ) k E= ⋅

gyelectronic interactions

13

atio

ns EΔ

Applic

a

0M 0E(180 ) k (E E)= ⋅ − Δ

W. Udo Schröder, 2007

Page 14: Structure and Interactions of Nuclear Matter (99.95% of ...

Sample Mass Analysis14

atio

ns

Abalone – Pacific shellfish

Applic

a

W. Udo Schröder, 2007

Blood sample

Page 15: Structure and Interactions of Nuclear Matter (99.95% of ...

Non-Destructive Material Depth Analysis

Ion Beam le

Different ions of a given energy test to different depths. Used most often: p.

Recoil mass Mr

Ion Beam

Elastic Scattering KinematicsSam

p

15

atio

ns

Depth Projectile

Applic

a

f Fli

gh

tTim

e o

f

W. Udo Schröder, 2007

Recoil Energy E2

Page 16: Structure and Interactions of Nuclear Matter (99.95% of ...

Applications of Nuclear Instruments and Methods16

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 17: Structure and Interactions of Nuclear Matter (99.95% of ...

Nuclear Space Technology

Nuclear radiation detectors are used inNuclear radiation detectors are used inexplorations of the sun and its planets. Spacevehicles use them to detect and identify directlyemitted or back-scattered radiation. Surfacematerials on Mars have been analyzed withactivation methods using radioactive sources.1

7at

ionsRadiation

detector

Applic

adetector

W. Udo Schröder, 2007

Sojourner Pathfinder Mars explorer

Page 18: Structure and Interactions of Nuclear Matter (99.95% of ...

Activation Radiation from Planetary Surface18

atio

ns

Applic

a

W. Udo Schröder, 2007Group project: N* Detector for Application in Nuclear Forensics

Page 19: Structure and Interactions of Nuclear Matter (99.95% of ...

Origin of Chemical Elements: Stellar Nucleosynthesis

r-p process (rapid-proton capture)produces heavy elements.

r process (rapid-neutron capture)

Strong T dependence19

atio

ns

Details of nuclear structure andstability and the conditions atformation (star, Big Bang) account forthe natural abundance of elements.reaction

Applic

a

Much of the information needed is notyet known

Task of future experiments.

path

W. Udo Schröder, 2007

Page 20: Structure and Interactions of Nuclear Matter (99.95% of ...

Abundance of Solar Elements

Too many heavy elements for production in solar burning processes. solar burning processes. Temperature is too low in solar interior(T9 = 0.015 K, ρ = 158 g/cm3).Sun is result of evolution through several

20

atio

ns

stellar life cycles (accretion of interstellar dust, ignition, burning, collapse and explosion)

Applic

a

W. Udo Schröder, 2007

Page 21: Structure and Interactions of Nuclear Matter (99.95% of ...

Supernovae

Large Magellanic Cloud

Kamiokande II

Time-of-flight spectrumof neutrinos, measuredrelative to γ -rays.

21

atio

ns

Applic

a

0.85 MeV and 1.24 MeV γ -rays from 56Co synthesized in the SN.

W. Udo Schröder, 2007

Page 22: Structure and Interactions of Nuclear Matter (99.95% of ...

Supernova Explosion Imaged by Hubble Space Telescope22

atio

ns

Applic

a

W. Udo Schröder, 2007

Supernova 1994D in Galaxy NGC 4526 (108 M ly). It is brighter than the galaxy. (Hubble Space Telescope, NASA)

Page 23: Structure and Interactions of Nuclear Matter (99.95% of ...

Supernova: Collapse and Explosion of a Star

(Simulation:NASA)

23

Page 24: Structure and Interactions of Nuclear Matter (99.95% of ...

Binary X-Ray System: Neutron Star/Companion Star

Neutron star and companion in a binary

t A ti di k i

Image:NASA

system. Accretion disk is created from matter pulled out of the companion. 2

4at

ions

Applic

a

h ’ f l

W. Udo Schröder, 2007

Matter impinging on the neutron star’s surface creates nuclear reactions.sp and rp processes proceed rapidly along drip lines and drive X-ray bursts that can be observed on earth.

Page 25: Structure and Interactions of Nuclear Matter (99.95% of ...

Structure of a Neutron StarNSCL-ISF Proposal, 2006

25

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 26: Structure and Interactions of Nuclear Matter (99.95% of ...

rp Reactions flow during X-Ray Burst

rp reaction flow (red line) during X-(red line) during Xray burst.

The series ends at the Sn-Sb-Te cycle.

26

atio

ns

y

Applic

a

W. Udo Schröder, 2007

Page 27: Structure and Interactions of Nuclear Matter (99.95% of ...

Applications of Nuclear Instruments and Methods27

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 28: Structure and Interactions of Nuclear Matter (99.95% of ...

Halflives of Radio-Isotopes for Dating

years Age of Earth Nucl. Synth.

28

atio

ns

Applic

a

α, β, β− : particles measured to identify fractional abundance of radioactive isotope, K: K electron capture pR : measure series of several decay products

W. Udo Schröder, 2007

Page 29: Structure and Interactions of Nuclear Matter (99.95% of ...

Carbon Dating of Organic Objects0 6931 0 6931 4 1

1 / 2

0.6931 0.69311.21

5730a10 a

tλ − −= = ×=

12C 12CN (t ) N (t 0)= = t 0 :=

12

t14C 14C

t14C

12C 1 3 10

N (t ) N (t 0) e

N (t )R(t ) R(t 0) e

N (t )

λ

λ

− ⋅

− ⋅

= = ⋅

= = = ⋅

n

14

time of deathNo further

C intake

29

atio

ns

12C 1.3 10

" ag1 R(0)

t nR(

e"t )λ

≈ ⋅

⎡ ⎤= ⎢ ⎥

⎣ ⎦→ =

Measure 14C/12C ratio of sample at t

Applic

a

Conventional method: β counting

14 2 1

Now :

N( C ) 2 5 − −

W. Udo Schröder, 2007

14 2 1

14 12 12

1 2

N( C ) 2.5 cm s

C C 1.5 10t 5730 a

= ⋅=

Direct 14C counting method: Accelerator Mass Spectroscopy R á 10 -16 (10 5 a)

Page 30: Structure and Interactions of Nuclear Matter (99.95% of ...

Calibration of 14C Dating Methods

t-dependent flux of cosmic rays (solar cycles)

t dependent 14C

Variation in 14C Production

t-dependent 14C production and intake

Calibration:30

atio

ns

14C-analyze yearly rings in trees of different ages (number and widths of rings) connect to fossils

Applic

a rings), connect to fossils

Errors in very old samples lead to underestimation of age (few hundred years)

(a) CE age (few hundred years).

W. Udo Schröder, 2007

Page 31: Structure and Interactions of Nuclear Matter (99.95% of ...

Rb/Sr Dating of Rocks/Age of the Earth

All rocky objects (planets, asteroids, meteorites) of solar system crystallized ≈ simultaneously (t=0) out of interstellar dust/nebula (supernova remnants).

87 87

87

P P D

Parent P Rb, daughter D Sr

Re ference R Rb (stable)N (0) N (t ) N (t ) but unknown!

= =

== +

1 2

9

t

4.7 10 a

=

⋅31

atio

ns

Undisturbed by erosion/transmutation

tP P R R

D P P D

P P D

N (t ) N (

N (0) N (t )

0) e N (t ) N (0)

N (t ) N (0) N (t ) N (0)

N (t ) but unknown!λ− ⋅= ⋅ =

= − +

+

R

Applic

a

tD P D

tPD

N

N (t )N

(t ) N (t ) e 1 N (0)

N (t )e 1

N (t )(t )

λ

λ

+ ⋅

+ ⋅

⎡ ⎤= ⋅ − +⎣ ⎦

⎡ ⎤= ⋅ −⎣ ⎦DN (0)

N (0)+

Different minerals in meteorite containing different amounts of R

mx

R

y

N N (t )(t )0

R

y

N (0)different amounts of NP different x

Construct isochron1

W. Udo Schröder, 2007

0 m( ) xy y t= + ⋅ 1t n m 1

λ→ = ⋅ +⎡ ⎤⎣ ⎦ Age of rock (since formation)

Page 32: Structure and Interactions of Nuclear Matter (99.95% of ...

Age of Earth

Age of Earth = 4.5·109 aMoon has similar age

32

atio

ns

Applic

a

Terrestrial volcanic activity dated:

W. Udo Schröder, 2007

produces younger rocks

Page 33: Structure and Interactions of Nuclear Matter (99.95% of ...

Applications of Nuclear Instruments and Methods33

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 34: Structure and Interactions of Nuclear Matter (99.95% of ...

Energy from Nuclear Fission

235 236 * 2 2(3) 200U U FF M V

converts 0.1% of the mass into energy1g 235U/day = 1MW108 h i l i

1938: Otto HahnFritz Straβmann Lise Meitner, Otto FrischHahn Straβmann

235 236

235 236 * 147 87

2 2(3) 200

: 2

th

th

U n U FF n MeV

Ex U n U La Br n

+ → → + +

+ → → + +

108 x chemical energies

Eff = 168 MeVEn tot = 5 MeVE 7 MeV

34

sion

Pow

er

Eγ = 7 MeVFF β-decay = 27 MeV

Qtotal = 207 MeV

<En>th = 0.025eVfission

fragment

Nucl

ear

Fiss

Neutrons:<mn> =2.5 ±0.1 nt

235U

n

neutron energies <En>≈2MeV

h

n

W. Udo Schröder, 2004

fission fragment

Page 35: Structure and Interactions of Nuclear Matter (99.95% of ...

The “Atomic Bomb”

July 16, 1945July 16, 1945

First explosion of a nuclear device.First explosion of a nuclear device.North of Alamogordo/NMNorth of Alamogordo/NMNorth of Alamogordo/NMNorth of Alamogordo/NM

35

Wea

pons

Nucl

ear

W

W. Udo Schröder, 2004

Page 36: Structure and Interactions of Nuclear Matter (99.95% of ...

Nuclear Power in Space

Nuclear energy is used to powersubmarines, ice-breakers, aircraftcarriers, extra-terrestrial craft,deep space probes, i.e.,everywhere where power has to becreated very reliably andefficiently, in order to maintainautonomous operations for long

36

atio

ns

time periods.

Applic

a

Galileo spacecraft

W. Udo Schröder, 2007Voyager spacecraft

Page 37: Structure and Interactions of Nuclear Matter (99.95% of ...

Global Problem: Finite Conventional Energy Sources

Most existing oil and gas fields have already been discovered.

X 4Major new discoveries not expected (world-wide)

Oil companies have not

37

atio

ns

productionbuilt any new refineries in > 30 years.

Applic

a

World will run out of oil,

time

gas, and coal within a few human generations

W. Udo Schröder, 2007

Page 38: Structure and Interactions of Nuclear Matter (99.95% of ...

The Need for Nuclear Power

Page 39: Structure and Interactions of Nuclear Matter (99.95% of ...

Conventional and Advanced Nuclear Energy Generation

Conventional power generation:Fission of 236U (5%-6% enriched)

Open fuel cycle produces long-lived

Fission induced by thermal neutronsFission chain reaction

Fi i i d d Open fuel cycle produces long lived radioactive fission fragments and weapons Pu

N th d Th/U l

Fission induced by thermal neutrons stops neutronsFission chain

39

atio

ns

Neutron multipliers:

New methods: Th/U cycle:

• Fission of 233Th (no Pu generation)closed fuel cycle

reaction

Applic

a

New methods:

•Spallation of heavy materials (Hg Pb Bi neutron multipliers

Neutron multipliers:p-induced spallation produces fast neutrons

fission of actinides and breedingU, actin. mix fuel

(Hg, Pb, Bi… neutron multipliersfast n fission Th, U, spent nucl. fuel)

• Sub-critical reactors ( k < 1)238U

W. Udo Schröder, 2007

• D - T fusion

Transmutation of nuclear wasteU, Cm, Np, Am

Page 40: Structure and Interactions of Nuclear Matter (99.95% of ...

Transmutation of Spent Nuclear Fuel

Spallation of heavy materials generates net energy: Powerout≈50xPowerin

40

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 41: Structure and Interactions of Nuclear Matter (99.95% of ...

Transmutation / Incineration

Fission P d t

Fission + + 180 MeV (32 pJ)

Incineration of TransUnnn

Product Product+84%

+ 180 MeV (32 pJ)

Pu-239n Pu-24024 000

41

atio

ns

Pu-240 U-2366535 a

α+16%

24.000 a

R l

Applic

a

Transmutation of Fission Fragments

Recycle, irradiate again

I-129n I-130 Xe-13012 h + β-

Transmutation of Fission Fragments

16 Ma

W. Udo Schröder, 2007

Xe-130 not radioactive

Page 42: Structure and Interactions of Nuclear Matter (99.95% of ...

Energy Source of the Future: Hydrogen Fusion

3 3 27M Vd d H

Deuterium and tritium in oceanic water (d: 0.015% in natH2O)

3

4

3 4

3.27

17.59

18 35

MeV

M

d d He n

d t He n

d He He

eV

p MeV

+ → +

+ → +

+ → +

+

+

+

42

atio

ns

18.35d He He p MeV+ → + +131 1.6 10MeV J−= ×

Applic

a

Laser Beams

W. Udo Schröder, 2007

Target UR-LLEOmega laser system

Page 43: Structure and Interactions of Nuclear Matter (99.95% of ...

Z-Pinch:

D-T Fusion Energy Generation in a Plasma Z-Pinch:In a z-pinch, a plasma is generated by passing a fast current pulse through many thin metal wires. These wires are usually initially arranged in a cylindrical shell geometry. After the current pulse ablates the wire material, the strong magnetic forces resulting from the current tend to crush the plasma toward the central z axis of the shell, hence the name "z-pinch."

Sandia National Lab is currently investigating the z-pinch as a possible ignition source for inertial confinement fusion. On its "Z-machine," Sandia can achieve dense, high temperature plasmas by firing fast, 100

(Ronald M. Gilgenbach, Yue Ying Lau)

43

atio

ns

temperature plasmas by firing fast, 100

Applic

a

zB

W. Udo Schröder, 2007

Page 44: Structure and Interactions of Nuclear Matter (99.95% of ...

Inertial Confinement Fusion by Electromagnetic Constriction

Sandia Laboratories, “Z machine”. 36 bus bars concentrate electrical energy in an intense current pulse (∼100 TW, 20 ns) focused on target chamber. Electric energy stored in capacitor banks.

44

atio

ns

Applic

a

Collapse of DT pellet

W. Udo Schröder, 2007

Converging currents

Page 45: Structure and Interactions of Nuclear Matter (99.95% of ...

Inertial Confinement Fusion by High Electric Currents

Shot of the Z-Machine

45

atio

ns

Applic

a

W. Udo Schröder, 2007

Page 46: Structure and Interactions of Nuclear Matter (99.95% of ...

46

atio

ns

Applic

a

W. Udo Schröder, 2007