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Importance of strains in semiconductors andEffect of strain on valence band
R. John Bosco BalaguruProfessor
School of Electrical & Electronics EngineeringSASTRA University
B. G. JeyaprakashAssistant Professor
School of Electrical & Electronics EngineeringSASTRA University
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Table of Content
1. IMPORTANCE OF STRAINS IN SEMICONDUCTORS..............................3
1.1 STRAINED LAYERS................................................................................................................3
1.2 EFFECT OF STRAIN ON VALENCE BANDS......................................................................41.3 ELASTICITY.............................................................................................................................4
2. EFFECT OF STRAIN ON VALENCE BAND................................................11
2.1 BAND STRUCTURE IN QUANTUM WELL AND EXCITON EFFECT...........................13
3. QUIZ AND ASSIGNMENT............................................................................15
3.1 SOLUTIONS...........................................................................................................................16
4. REFERENCES................................................................................................20
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1 Importance of strains in semiconductors
This lecture provides you about the strained layer and the mathematical
representation of it in low dimensional semiconductor
In the late 1980s, it was believed that laser devices could only be made reliablyfrom lattice-matched epitaxial materials. By 1999, low cost diode pumped laser werefabricated from the strained-layer. The presence of strains within atoms in a lattice willchanges the physical properties and the device obtained from those materials will haveenhanced performance. For e.g.strained silicon is a layer of silicon in which the siliconatoms are stretched beyond their normal interatomic distance. This can be done bydeposited thin film of silicon over a substrate of silicon germanium (SiGe). As the atomsin the silicon layer align with the atoms of the underlying silicon germanium layer, thebonds between the silicon atoms become stretched - thereby leading to strained silicon.
This reduces the atomic forces that interfere with the movement of electrons and canmove faster with better mobility. Also allowing strained based silicon transistors toswitch faster.
1.1 Strained Layers
In general, the quality of an interface between two materials depends greatly onthe relative size of the lattice constants. If the lattice constants are very similar, as in thecase of the AlxGa1xAs and GaAs heterojunctions, for which the lattice constant variesless than 0.2% for the whole range of x, and the thermal expansion coefficients aresimilar, no stresses are introduced at the interface. However, in other cases,
heterojunctions with differences in lattice constants up to 6% are fabricated (for instance,InxGa1xAs and GaAs). In this case strong stresses appear at the interface and only verythin films of a few monolayers can be grown on a given substrate.
These strained layers show new effects that are exploited in variousoptoelectronic applications, especially in quantum well lasers and electro-opticmodulators due to reduced or change in atomic force between atoms in the lattice.
Suppose a layer of lattice constant aL is grown on a substrate of lattice constantaS
. The strain of the layer is define as:
(1)
Fig. 1 show the case of InxGa1xAs grown on GaAs for which aL> aS
s
sL
a
aa =
. In Fig. 1, thesituation of the separate layer and substrate is depicted. If the epilayer is not too thick, theatoms of the layer match those of the substrate. Therefore, the layer is subjected to acompressive stress in the plane of the interface and the interplanar vertical (or on the
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growth direction) distance increases (Fig. 1(b)). As a consequence of the distortion of theInGaAs lattice, elastic energy is stored in the system, which increases with layerthickness. Therefore, if the thickness of thefilm is la rger than the so-called criticalthickness, the system relaxes and the appearance of dislocations in the plane of theinterface is energetically favourable (Fig. 1(c)).
Fig. 1 Growth of a layer of lattice constant aL>as
Electrons in a semiconductor experience the periodic potential of the crystallattice. This potential leads to the formation of energy bands. The electronic bandstructure of a semiconductor describes the energy states that an electron is
allowed or forbidden.
. (a) The layer is not yet deposited over the substrate; (b) the layer issubjected to a compressive stress; (c) when the layer is thicker than the critical thickness, dislocations are formed.
1.2 Effect of strain on valence bands
Band structure is altered by the application of stress and strain. Both are tensorquantities and are related through Hook's law. To know about the effect ofstress/strain on band structure, let we go through the fundamental theory ofelasticity of it.
1.3 Elasticity
The property of solid materials to deform under the application of an externalforce and to regain their original shape after the force is removed is referred to as itselasticity. The external force applied on a specified area is known as stress, while theamount of deformation is called the strain. Imagine an object oriented in the cartesiancoordinate system with a number of forces acting on it, such that the vector sum of all theforces is zero. Take a slice orthogonal to the -direction and define a small area on thisslice as Ax. Let the total force acting on this small area be
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kFjFiFF zyx... ++= )2(
We can define the following scalar quantities
The subscript I and j in T ij
refer to the plane and the force direction, respectively.Similarly considering slices orthogonal to the y and z- direction, we obtain
The scalar quantity can be arranged in a matrix form to yield the stress tensor and thevarious components are shown in Fig. 2.
)3(
The condition of static equilibrium implies
)4(
Fig. 2. Component of the stress sensor
x
z
Axz
x
y
Axy
x
x
Axx
A
FT
A
FT
A
FT
xxx
=
=
=
000lim,lim,lim
z
z
Azz
z
y
Azy
z
x
Azx
AFT
AFT
AFT
zzz =
=
=
000lim,lim,lim
y
z
Ayz
y
y
Ayy
y
x
Ayx
A
FT
A
FT
A
FT
yyy
=
=
=
000lim,lim,lim
=
zzzyzx
yzyyyx
xzxyxx
TTT
TTT
TTT
T
jiij TT =
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A body under elastic deformation experiences an internal restoring force. The amount of
deformation caused is called strain Similar to stress; the tensor strain component can be
given as
=
zzzyzx
yzyyyx
xzxyxx
)5(
Such that
+
=
i
j
j
i
ijx
u
x
u
2
1 )6(
The sign convention adopted for stress is that tensile stress causes an expansion, whereascompressive stress causes a contraction.
The relation between stress and strain was given by Hook's law and it states that the
amount by which a material body is deformed (the strain) is linearly related to the force
causing the deformation (the stress). The most general relationship between stress andstrain can be mathematically written as
)9(
Here, Cijkl is a fourth order elastic stiffness tensor comprising 81 coefficients. However,
depending on the symmetry of the crystal the number of coefficients can be reduced. For
cubic crystals such as Si and Ge only three unique coefficients, C 11, C12 and C44
ijijklij TS=
, exist.These coefficients are known as the stiffness constants. The generalized Hooks law in
matrix form is given as
(10)
00000
00000
00000
000000
000
6
5
4
3
2
1
44
44
44
111212
121112
121211
6
5
4
3
2
1
=
x
c
c
c
cccccc
ccc
T
T
T
TT
T
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Of practical interest is the strain arising from a certain stress condition. The strain
components can be obtained by inverting Hook's law and utilizing the compliance
coefficients S
ijkl
)9(
The stiffness and compliance tensors are linked through the relation S = C-1
. Using thisrelation, the three independent compliance coefficients can be calculated as
(10)
It is often required to know the stress in the crystallographic coordinate system for astress applied along a general direction. Consider a generalized direction [x, y, z] in
which the stress is applied. The stress in the crystallographic coordinate system [x, y,z]
can be calculated using the transformation matrix U.
=
cossinsincossin
0cossinsinsincoscoscos
),(U )11(
Here denotes the polar and the azimuthal angle of the stress direction relative to thecrystallographic coordinate system, as shown in Fig.3. The stress in the crystallographic
coordinate system is then given by
Tcrys
UTUT ..=
44
44
2121211
211
1211
12
2
121211
2
11
121111
1
,2
,2
cs
cccc
cc
s
cccc
ccs
=
+
+=
+
+=
ijijklij TS=
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Fig. 3. Stress direction relative to crystallographic plane
Applying a non-zero stress of magnitude applied along the [100], [110] and [111]
directions, the stress tensors in the principal coordinate system read, respectively
[ ] [ ] [ ] ,
333
333
333
,
000
022
022
,
000
000
00
111110100
=
=
=
PPP
PPP
PPP
TPP
PP
T
P
T
The corresponding strain tensors are:
[ ]
[ ]
[ ]
+
+
+
=
+
+
=
=
)3).2(6.6.
6.)3).2(6.
6.6.)3).2(
.00
02).(4.
04.2).(
.00
0.0
00.
12114444
44121144
44441211
100
12
121144
441211
100
12
12
11
100
PssPsPs
PsPssPs
PsPsPss
Ps
PssPs
PsPss
Ps
Ps
Ps
)12(
For the case of epitaxially grown Si on SiGe, the in-plane strain
='
33
'
32
'
31
'
23
'
22
'
21
'
13
'
12
'
11
'
is given by Eqn. 1.
Consider an interface (primed) coordinate system, the -axis of which is perpendicular to
the Si/SiGe interface. The strain tensor in this coordinate system can be written as
with 1'
22
'
11 == . Since epitaxial growth does not produce any in-plane shear strain inthe interface coordinate system, we have 0'21
'
12 ==
Other strain components can be determined by considering all the external stress
components in the vertical direction vanish i.e. T13=T23=T33=0 and using Hookes law
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)3,3(),3,2(),3,1(),(0'' == ijijC )13(
Expanding above equation,
''
22
''
11
'
31
'
31
'
23
'
23
'
33
'
33 )(222 ICCCCC +=++
This can be expressed in matrix form as
+
+
+
=
'
3122
'
3111
'
2322
'
2311
'
3311
'
3311
'
31
'
23
'
33
'
3131
'
3123
'
3133
'
2331
'
2323
'
2333
'
3331
'
3323
'
3333
2
2
CC
CC
CC
CCC
CCC
CCCI
)14(
The ' klC matrix element can be determined from the elastic stiffness tensor klC through
the relation,
ijjlikkl CUUUUC =' )15(
where U denotes the transformation matrix. Once the matrix elements are known, the
matrix can be inverted to determine the ),,( '33'
23
'
13 . Having determined the strain tensor
in the interface coordinate system, the tensor can be transformed to the principalcoordinate system using
ijjiUU = (16)
Equation A and B can be solved to obtain the strain tensor. Above table lists theexpressions for the strain tensor components for the high-symmetry (100), (110) and
(111) oriented SiGe substrates.Table 1 summarizes these symmetry points and directions.
These points and directions are of importance for interpreting the band structure plots.
Substrate orientation
[ ]100 [ ]110 [ ]111
11
I
441211
1244
2
2
ccc
ccI
++
441211
44
42
4
ccc
cI
++
22 I
441211
1244
2
2
ccc
ccI
++
441211
44
42
4
ccc
cI
++
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33
11
122
c
cI
I
441211
44
42
4
ccc
cI
++
12 0
441211
1211
2
2
ccc
ccI
++
+
441211
1211
2
2
ccc
ccI
++
+
13 0 0
441211
1211
2
2
ccc
ccI
++
+
23 0 0
441211
1211
2
2
ccc
ccI
++
+
Fig. 4. (a) Structure of Si crystal lattice (b) Brillioun zone
Symmetric pointsDirection Coordinate Remark ( )0,0,0 Origin of k space
( )0,0,1 Middle of square faces
L
21,
21,
21 Middle of hexagonal faces
K
4
3,
4
3,
4
3
Middle of edge shared by twohexagons
U Middle of edge shared by
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hexagons and squareW Middle of edge shared by two
hexagons and square 0,0,1 Directed from and
1,1,1 Directed from and L
0,1,1 Directed from and K
2 Effect of strain on valence band
This lecture deals about the change in band structure in strained layers of
semiconducting materials
Several symmetry operations can be performed on the diamond structure which
leave the structure unchanged. Apart from translation, such operations can be categorized
as rotation or inversion, or a combination, and are collectively known as symmetry
operations. Due to the fcc lattice of the diamond structure there exist a total of 48 such
independent symmetry operations. This symmetry of the lattice in real space is also
reflected in the first Brillouin zone. The lowering of symmetry of the fcc structure due to
strain can distort it to some of the 14 Bravais lattice forms, such as the tetragonal,
orthorhombic or trigonal lattice. The new lattice structure formed has different symmetry
properties which can have pronounced consequences on the band structure. Numerical
methods for calculating the band structure allow the prediction of several important
electronic and optical properties.
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Fig. 5. (a) Band structure of silicon (b) Splitting of valence band
At T=0K, the highest energy band that is completely filled is denoted as the
valence band. The next higher band is completely empty at and called the conduction
band. The two bands are separated by a forbidden energy gap, known as the bandgap Eg
++=
t
z
t
y
l
x
m
k
m
k
m
kk
2222
2)(
.
The principal conduction band minima of Si are located along the [100], [010]
and [001] directions at a distance of about 85% from the -point to the X-points. The
minima of the second conduction band touch the first conduction band at the X-points.
This degeneracy of the two conduction bands can produce interesting effects on applying
shear strain we discussed earlier. Close to the principal minima the band structure can be
represented by ellipsoidal constant energy surfaces by assuming a parabolic energy
dispersion relation. For valleys located along the [100] direction, the energy dispersion
reads
)17(
where the wave vector )zyx kkkk ,,= .The constant energy surfaces are described by a
longitudinal mass,ol mm = 91.0 , and a transversal mass 019.0 mmt = . This anisotropy
in the masses makes the transport in each valley anisotropic. The 6-fold degeneracy of
the valleys arise due to the symmetry of the lattice along the [100], [010] and [001]
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directions. At low values of the electric field, the electrons occupy all the 6 valleys
equally and thus the transport is isotropic.
Unlike the conduction band, the valence band structure looks highly anisotropic even in
the unstrained case. The valence band maximum in Si is located at the point. Due to
the degeneracy of the bands at the point, the energy surfaces develop into quadratic
surfaces of the form
)()(
)()(
2222222422
2222222422
xzzyyxlh
xzzyyxhh
kkkkkkCkBAkk
kkkkkkCkBAkk
++++=
+++=
Here )(khh and )(klh denote the energies of the two degenerate bands and the
parameters A, B and C denote the inverse band parameters. Due to the smaller energy
values of the )(khh bands in comparison to the )(klh , the effective masses for the
)(khh band is larger. Therefore, this band is referred to as the heavy hole (HH) band and
the )(klh band as the light hole (LH) band. The shape of the constant energy surface for
the LH and HH bands is warped or fluted. There is also a third band, the so called split-
off band located about 44 meV below the HH/LH bands. A schematic plot of the constant
energy surface for the HH band is shown in Fig. 4(b)
2.1 Band structure in quantum well and exciton effect
Quantum wells are formed in semiconductors by having a material, like gallium
arsenide sandwiched between two layers of a material with a wider bandgap, like
aluminium arsenide. Because of their quasi-two dimensional nature, electrons in quantum
wells have a density of states as a function of energy that has distinct steps, versus a
smooth square root dependence that is found in bulk materials. Additionally, the effective
mass of holes in the valence band is changed to more closely match that of electrons inthe conduction band. The optical properties of quantum well strongly depend upon band
structure. For example, in multiple quantum well of GaAs-AlGaAs, the optical spectrum
follows in general the steps of the density of state curve in two dimensional
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semiconductors. At the edge of each step there will be a sharp maximum and is attributed
to excitonic effects.
In the case of confined systems for electrons and holes, such as quantum wells,
wires, and dots, the excitonic effects are much more important than in bulk solids. In
effect, the binding energy of the electronhole system forming an exciton is much higher
in quantum confined systems than in the
case of solids, and, therefore, the excitonic
transitions can be observed even at
temperatures close to room temperature, as
opposed to the bulk case for which low
temperatures are needed. This makes the
role played by excitons in many modern
optoelectronic devices very important.
Qualitatively, it is easy to understand the
reason by which the binding energies of
excitons EB in quantum confined systems are much higher than in the bulk. For instance,
in the case of bulk GaAs the binding energy of excitons is only E B=.2meV and the Bohr
radius has a fairly large value of about aB = 150. In the figure, the exciton is
represented in two situations, the one in (a), in which the Bohr radius of the exciton ismuch smaller than the quantum well width, and the one in (b), for which the width of the
well is smaller than aB. In this case, the separation between the electron and the hole is
limited by the width of the well and therefore the exciton becomes squeezed, thus
increasing the Coulomb attractive force. For a two-dimensional hydrogenic atom, a
simple calculation shows that EB is about four times larger in the 2D case than for 3D
solid. Another consequence of their high value of E B is that excitons can survive very
high electric fields in quantum wells which will find many applications in electro -optic
modulators
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3 Quiz and Assignment
1. For an isotropic material with GPaE 100= and 25.0= . Find the stress tensor
and strain energy density at a point in a body if the components of the straintensor are given by
2. A solid is subjected to stresses as shown by the arrows in the figure below.Indicate the indices for each of the stress components, and whether the stressesshould be positive or negative.
3. Suppose that the stress tensor field in a body is given by
Find the body force distribution required to maintain equilibrium. (x1,x2,and x3
4. Find the surface tractions at the internal point r=(1,-1,2) in the body on an internalsurface with a surface normal
are in meters). Show units.
( )1,1,1=n .5. Find the hydrostatic and deviatoric stress at the point ( )2,1,1=r . Find the
principal stresses at this point.6. Diamond structure has the ___________ lattice and exist a ____ Symmetry
operations.7. The principal conduction band minima of Si are located along the __________
directions.8. The band present in between the light and heavy hole band is called as _______9. How Quantum well is formed?10.The optical properties of quantum well strongly depend upon __________
610
01000
100200100
0100200
=ij
MPa
xxxxxx
xxxxx
xxxxx
ij
+++
++
++
=
2
2
12
2
32
2
1
2
2
331
2
3
2
2
1
2
32
2
1
2
2
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3.1 Solutions
1. The shear modulus ( ) is given by,
KPaGPaE 6104040
5.2
100
)1(2===
+=
The Lam modulus ( ) is given by
( )( )KPaGPa
E 6104040)5.0)(25.1(
25
211===
+=
The stress-strain relation for isotropic materials is
( )ijkkijijkkijij
+=
+=
240
2
Therefore, (after converting and into KPa so that the 10 -6
[ ]( )( )[ ] ( )( )[ ]( )( )[ ] ( )( )
[ ]( )( )[ ] ( )( )[ ] ( )( )[ ] ( )( )[ ] ( )( ) 800020040240
0040240
800020040240
16000400402002000340
240
32000800400200200340
240
32000800400200200340
240
1212
3131
2323
3322113333
3322112222
3322111111
===
===
===
==++=
+++=
==++=
+++=
==++=
+++=
term in the strain cancels
out),
In 3 x 3 matrix form (after converting into MPa from KPa)
MPaij
=
1680
8328
0832
The strain energy density is given by
( ) ijijU 2
1=
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Therefore,
( ) [ ]
( )( ) ( )( ) ( )( ) ( )( )( ) ( )( )( ) ( )( )( )[ ]
[ ]
KPPa
Pa
Pa
U
88000
16001600640064002
1
1008200208201620032200322
1
2
11212311312323333322221111
==
+++=
+++++=
+++++=
The strain energy density is KPaU 8=
2.
3. The equation of equilibrium is
0,0 , =+=+ jiij borb
Therefore,
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( ) ( ) ( )
( ) ( ) ( )
( ) ( ) ( ) 0
02
02
3
3
221
2
223
1
221
2
3
2
2
3
2
31
1
2
3
1
3
2
2
1
2
2
3
1
2
2
1
=+
++
++
+
=+
++
++
=+
++
+
+
bx
xx
x
xx
x
xx
bx
xx
x
xx
x
x
bx
xx
x
x
x
xx
(or)
0012
0200
0002
31
23
11
=+++
=++
=+++
bx
bx
bx
The required body forces are (in MN/m3
( )133211 21;2;2 xbxbxb +===
)
4. The surface traction is given by
ijij ntornt ==
The stress at point r is
[ ] MPa
=
050
538
080
Therefore
MPa
nnnt
MPa
nnnt
MPa
nnnt
5)0)(1()5)(1()0)(1(
0)5)(1()3)(1()8)(1(
8)0)(1()8)(1()0)(1(
3332321311
3232221211
3132121111
=++=
++=
=++=
++=
=++=++=
The traction vector is (after converting n^ into a unit normal)
( )( )MPat 5,0,831=
5. The hydrostatic stress is given by
Irt
h3
=
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In this case
3330332211 =++=++= rt
Therefore,
MPah
=
100
010001
The deviatoric stress is given by
hd =
Therefore,
MPad
=
150
528
081
The principal stresses can be found using the equation
( ) 0det = I where is a principal stress. In expanded form,
0det
332313
232212
131211
=
Substituting the values of stress into the above equation,
0
50
538
08
det =
Expanding out,
( )( ) ( )( )[ ] ( ) ( )( ) ( )( )[ ]
( ) ( )
0893064253
088253
00588553
23
32
2
=
=++
=++
=
Thus, the first possible value of =0 MPa.
Also
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08932 =
Therefore,
( )MPa05.8,05.112
35693=
+=
The principal stresses are (in MPa);05.8;0;05.11 321 ===
6. fcc, 487. [100], [010] and [001]8. Split off band.9. Quantum wells are formed as low band gap semiconductors material is
sandwiched between two layers of a wider band gap material.10.Band structure
5 References
[1] L.O.Lokot, Strain effect on the valence band structure, optical transitions, and
light gain spectra in zinc-blende GaN quantum wells, Semiconductor Physics,
Quantum Electronics & Optoelectronics, 11 (2008) 364-369.
[2] John C. Bean, Strained-Layer Epitaxy of Germanium Silicon Alloys, Science,
230 (1985) 127-131.
[3] X-H Peng, A.Alizadeh, N. Bhate, K K Varanasi, S K Kumar and S K Nayak,
First- principles investigation of strain effect on the energy gaps in silicon
nanoclusters, J.Phys.: Condens. Matter 19 (2007) 266212 (9pp).
[4] J.M. Martinez- Duart, R.J.Martin-Palma, F. Agullo-Rueda, Nanotechnology for
Microelectronics and Optoelectronics, Elsevier, 2006.