ICE - Laboratory experiment goals
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Transcript of ICE - Laboratory experiment goals
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ICE - Laboratory experiment goals
• Basic scientific understanding• Check performance of airborne instruments• Develop new measurement techniques & combining
methods (CVI -> CFDC)
STRENGTHS:
Environment control
Repeatability
Mechanistic studies
Test specific aerosol types (dust, bacteria, ..)
Crystal growth habits & rates
Effects of organic coatings, electric charge, ..
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Laboratory Experiments A. Cloud types
Layer• upslope
• stratus
Wave
Cumulus• warm base
• cold base
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Laboratory Experiments B. Discussion Topics-AIDA
desert dustPaulF summarized yesterday
Sulfuric acid coated soot aerosolsnew JGR paper, in press
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AIDA (Aerosol Interactions and Dynamics in the Atmosphere)
84 m3
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AIDA - Sulfuric acid coated soot aerosolsice nucleating threshold
Koop, T., B. P. Luo, A. Tsias, and T. Peter (2000), Water activity as the determinantfor homogeneous ice nucleation in aqueous solutions, Nature, 406 (6796), 611–614.
Koop
w. sat
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Lab (& modeling) studies
Description Measurements Variables
water cloud formation rh > 100%
CCN spectra, haze & cloud drop conc, particle sizes
(1) CCN chemistry, sizes & conc, LCL, updraft (2) internally mixed or externally mixed
aerosol; organic films
Homog. freezingrh < 100%
same, plus ice crystals
artificial CCN properties (ammonium sulfate, sulfuric acid, sodium chloride, ..)
Heterog. freezing rh < 100%
same, + IN activation spectra (T, rh)
(1) Externally mixed aerosol: artificial CCN & IN; aerosol chemistry
(2) Internally mixed aerosol
Heterog. freezing rh > 100%
same same - (how important is the presence of the liquid phase?)
laboratory-generated surrogates of naturally particles: sea-salt; mineral dust; soot
natural airrh < 100% rh > 100%
same natural air
entrainment-mixing same Aerosol size, chem, elec charge, ..
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Measurement challenges
Ice nucleation modes:
• deposition ………………………….X
• condensation-freezing…………..X
• contact-freezing…………………X
• evaporation-freezing ……………?
• electro-freezing…………………?
Discriminating liquid from ice at small sizes (~1 µm)
Development of new techniques to measure ice nuclei
Aerosol concentrator (to improve statistics)
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Lab studies – possible participants
NCAR– EOL, ACD
NOAA– Aeronomy Lab, ..
International collaborations:– Germany, Japan, UK,
Switzerland
U.S. universities– CSU– DRI– Michigan Tech.– South Dakota SMT– PennState– Washington– Colorado– Wyoming
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Fluid dynamics modeling of instruments
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Computational mesh at inlet
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Compare FLUENT vs approx.thermodynamic trajectories
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Compare FLUENT vs approx.velocity profile