Frequency dependence of the photonic noise spectrum in an ...

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o o University of Utah Institutional Repository Author Manuscript Frequency dependence of the photonic noise spectrum in an absorbing or amplifying diffusive medium E. G. Mishchenko 1 ,2, M. Patra 1 , and C. W. J. Beenakker 1 l Instituut-Lorentz, Universiteit Leiden, P. O. Box 9506, 2300 RA Leiden, The Netherlands 2 L. D. Landau Institute for Theoretical Physics, Russian Academy of Sciences, Kosygin 2, Moscow 117334, Russia Abstract A theory is presented for the frequency dependence of the power spectrum of photon current fluctuations originating from a disordered medium. Both the cases of an absorbing medium ("grey body") and of an amplifying medium ("random laser") are considered in a waveguide geometry. The semiclassi- cal approach (based on a Boltzmann-Langevin equation) is shown to be in complete agreement with a fully quantum mechanical theory, provided that the effects of wave localization can be neglected. The width of the peak in the power spectrum around zero frequency is much smaller than the inverse coherence time, characteristic for black-body radiation. Simple expressions for the shape of this peak are obtained , in the absorbing case, for waveguide lengths large compared to the absorption length , and, in the amplifying case, close to the laser threshold. PACS: 42.50.Ar, 05.40.-a, 42.68.Ay, 78.45.+h I. INTRODUCTION The noise power spectrum of a black body is frequency independent for frequencies below the absorption band width. The inverse of the band width is the coherence time Tcoh of the radiation [1], which for a black body is the longest relevant time scale - hence the white noise spectrum P(O) for 0 :s l/T co h. In a weakly absorbing, strongly scattering medium there appear two longer time scales: The absorption time Ta and the time L2 / D it takes to diffuse (with diffusion constant D) through the medium (of length L). As a consequence, P(O) for such a weakly-absorbing medium (sometimes called a "grey body") starts to decay at much lower frequencies than for a black body having the same coherence time. Although there is by now a substantial literature on the theory of grey-body radiation [2- 7], the results have been limited to either the zero or high-frequency limits of the noise spectrum (or, equivalently, to short or long photodetection times). In the present work we remove this limitation, by computing P(O) for a diffusive medium for arbitrary ratios of 0, l/T a , and D / L2. We compare two different approaches in a waveguide geometry: One which is fully quantum mechanical (based on random-matrix theory [7,8]) and another which is semiclassical (based on a Boltzmann-Langevin equation [9]). Each method has 1

Transcript of Frequency dependence of the photonic noise spectrum in an ...

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University of Utah Institutional Repository Author Manuscript

Frequency dependence of the photonic noise spectrum in an absorbing or amplifying diffusive medium

E. G. Mishchenko1,2, M. Patra1

, and C. W. J. Beenakker1

l Instituut-Lorentz, Universiteit Leiden, P. O. Box 9506, 2300 RA Leiden, The Netherlands 2 L. D. Landau Institute for Theoretical Physics, Russian Academy of Sciences, Kosygin 2,

Moscow 117334, Russia

Abstract

A theory is presented for the frequency dependence of the power spectrum of photon current fluctuations originating from a disordered medium. Both the cases of an absorbing medium ("grey body") and of an amplifying medium ("random laser") are considered in a waveguide geometry. The semiclassiยญcal approach (based on a Boltzmann-Langevin equation) is shown to be in complete agreement with a fully quantum mechanical theory, provided that the effects of wave localization can be neglected. The width of the peak in the power spectrum around zero frequency is much smaller than the inverse coherence time, characteristic for black-body radiation. Simple expressions for the shape of this peak are obtained, in the absorbing case, for waveguide lengths large compared to the absorption length, and, in the amplifying case, close to the laser threshold.

PACS: 42.50.Ar , 05.40.-a, 42.68.Ay, 78.45.+h

I. INTRODUCTION

The noise power spectrum of a black body is frequency independent for frequencies below the absorption band width. The inverse of the band width is the coherence time Tcoh of the radiation [1], which for a black body is the longest relevant time scale - hence the white noise spectrum P(O) for 0 :s l/Tcoh. In a weakly absorbing, strongly scattering medium there appear two longer time scales: The absorption time Ta and the time L2 / D it takes to diffuse (with diffusion constant D) through the medium (of length L). As a consequence, P(O) for such a weakly-absorbing medium (sometimes called a "grey body") starts to decay at much lower frequencies than for a black body having the same coherence time.

Although there is by now a substantial literature on the theory of grey-body radiation [2- 7], the results have been limited to either the zero or high-frequency limits of the noise spectrum (or, equivalently, to short or long photodetection times). In the present work we remove this limitation, by computing P(O) for a diffusive medium for arbitrary ratios of 0, l/Ta , and D / L2. We compare two different approaches in a waveguide geometry: One which is fully quantum mechanical (based on random-matrix theory [7,8]) and another which is semiclassical (based on a Boltzmann-Langevin equation [9]). Each method has

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its advantages and disadvantages: The quantum theory includes interference effects , which are ignored in the semiclassical theory, but it is mathematically more involved. Complete agreement between the two approaches is obtained in the limit that the waveguide length L is much smaller than the localization length (equal to the mean free path times the number of propagating modes).

The results for absorbing media can be applied directly to linear amplifiers , by formally changing the sign of the temperature and the absorption time. Loudon and coworkers [10,11] used this relationship to calculate the noise power spectrum of a waveguide without disorder. The generalization to a diffusive medium presented here describes a random laser [12] below threshold.

The outline of this paper is as follows. We start with the semiclassical approach, preยญsenting a general solution of the Boltzmann-Langevin equation in Sec. II and applying it to a waveguide geometry in Sec. III. The quantum mechanical approach is developed in Sec. IV. For the quantum theory we need the correlator of reflection and transmission matrices at different frequencies. These are calculated in the appendix, using the random-matrix method of Ref. [13]. We discuss our findings in Sec. V.

II. SEMICLASSICAL THEORY

Starting point of the semiclassical theory is the Boltzmann-Langevin equation for photons of Ref. [9]. We first consider an absorbing medium (in equilibrium at temperature T), leaving the amplifying case for the end of this section. We make the diffusion approximation, valid if the mean free path l is the shortest length scale in the system (but still large compared to the wavelength). The fluctuating number density n(w, r, t) and current density j(w, r, t) of photons at frequency w, position r, and time t are related by [9]

. Dan r J = - ar + -'-'1, (2.1)

an a. -2 - + - . J = D~ (pf - n) + Loยท at ar a (2.2)

Here D = ~cl is the diffusion constant, ~a = JDTa is the absorption length (with Ta the absorption time) , p = 47rw2 (27rc)-3 is the density of states (not counting polarizations) , and f = [exp (nwlkT) - 1]-1 is the Bose-Einstein function. We assume ~a ยป l. The fluctuating source terms Lo and ยฃ1 have zero mean and correlators

LO(W, r, t)Lo(W', r', t') = b(w - w')b(t - t')b(r - r')D~;;2(2fn + pf + n),

L1a(W, r, t)L1{3(W', r', t') = 2ba{3b(w - w')b(t - t')b(r - r')Dn(l + nip).

(2.3a)

(2.3b)

The cross-correlator of Lo and ยฃ1 is given in Ref. [9] , but will not be needed. Combining Eqs. (2.1) and (2.2) we find equations for the mean n and the fluctuations bn of the photon number density n = n + bn,

1 an a2n n pf - D at + ar2 - ~~ = - ~~ , (2.4)

_ ~ abn + a2bn _ bn = ~~ . ยฃ1 _ Lo

D at ar2 ~~ D ar D . (2.5)

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I ~ ___

i S2

FIG. 1. Thermal radiation (solid arrow) is incident through port So on an absorbing disordered medium (shaded). The outgoing radiation (dashed arrows) is absorbed by photodetectors.

We present a general solution for the multiport geometry of Fig. 1. Thermal radiation is incident through the port So and can leave the system via ports So, Sl, S2, ... , where it is absorbed by photodetectors. The corresponding boundary conditions are n(w, r, t)lrESp = nin(W, t)6po. We assume that the closed boundaries ~ of the system (with volume V) are perfectly reflecting. The separation of the ports is of order L ยป l. In what follows we assume detection of outgoing radiation in a narrow frequency interval 6w around w. We require that 6w is small both compared to wand to l/Tcoh. To minimize the notations in this section we omit the frequency argument wand use units in which 6w - 1. (We will reinsert 6w in the next section.)

The Green function of the differential equations (2.4) and (2.5) in the Fourier represenยญtation with respect to the time argument satisfies

( 82 -2 io') ( ') ( ') 8r2 - ~a + D G r, r ,0, = 6 r - r . (2.6)

C [Fourier transforms are defined as f (D,) = J~= dt eiOt f (t).] For frequency resolved detection C we require n ยซ 6w. We impose the boundary conditions

G(r, r', o')lrESp = 0, p = 0,1,2, ... ,

:E . 8G(r, r' , 0,) I = ยฐ 8r rE~ ,

(2.7a)

(2.7b)

~ b where :E denotes the outward normal direction to the surface ~. We consider separately the ~ mean and the fluctuations of the photon number and current densities. n H ~. rt

A. Mean solution

The average photon density satisfying Eq. (2.4) can be expressed in Fourier representation in terms of the Green function (2.6),

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- () - 2 -' ( ) J ' ( , ) - ( ) J ' ac ( r , r', 0) n r,O = -21[Pf~a u 0 dr C r,r ,0 +nin 0 dSยท ar' . v So

(2.8)

Substituting this formula into the expression for the current (2.1) and integrating over the area Sp one obtains the mean outgoing current lp through port p i= 0,

Ip(O) = 27rpD f~;;26(0) J dS . J dr' aC(~:" 0)

Sp v

- Dnin(ll) J dS" J dS~ a2~;:~~ Il). Sp So

(2.9)

(Summation over the repeating Greek indices is implied.) The first term ex 6(0) is the time-independent mean thermal radiation from the medium. The second term is that part of the mean radiation entering through port 0 that leaves the medium through one of the other ports. (The restriction to p i= 0 is not essential but simplifies the general formulas considerably, so we will make this restriction in what follows.)

B. Fluctuations

The fluctuations in the number density follow in a similar way from the Green function and Eq. (2.5),

( ) 1 J ' ( , ) ( a (') (')) ( ) J ' ac (r , r', 0) 6n r, 0 = D dr C r, r , 0 ar'ยท .L1 r , 0 - Lo r , 0 + 6nin 0 dSยท ar' . v ~

(2.10)

The fluctuation of the current density is then given by Eq. (2.1),

. ( ) J '( ( , ) (' ) ac ( r, r', 0) (' )) 6 J ex r , 0 = dr C ex(3 r , r ,0 L 1(3 r ,0 + ar ex Lo r , 0 v

- D6nin(0) J dS~ C ex(3(r , r', 0). (2.11) So

We have defined

( , ) a2C(r, r', 0) ( ') C ex(3 r, r ,0 = a a ' + 6ex(36 r - r .

rex r(3 (2.12)

We seek the correlator of the current fluctuations

C ex(3 ( r, 0; r', 0') = 6 j ex ( r, 0) 6 j (3 ( r', 0) (2.13)

for r ESp, r' E Sq with p, q i= O. With the help of Eqs. (2.3) and (2.11) it can be expressed as

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C ( n. , n') = DJd "aC(r ,r", 0) aC(r',r", 0') [(2f )-(" n n') f] af3 r , ~ {" r , ~ (, C2 r a a ' + 1 n r ,H + H + P ~a V r a r f3

[ 1 dO" ] +2D J dr"Cary (r, r", O)Cf3ry (r', r", 0') n(r",O + 0') + p J 21f n(r",O + O")n(r", 0' - 0") .

V

(2.14)

Following Ref. [9], we have neglected the term ex: 6nin in Eq. (2.11) (smaller by a factor ilL) and the cross-correlator LoLl (smaller by a factor i/~a).

We now integrate rand r' over Sp and Sq to obtain the correlator of the total currents through ports p and q,

Cpq(O , 0') = J dSa J dS~ Caf3 (r, 0; r', 0') = C~~)(O , 0') + C~~)(O , 0'). (2.15) Sp Sq

The first term C~~) contains the contribution from the terms linear in the number density n in Eq. (2.14). Performing integration by parts and using Eqs. (2.6)-(2.8) we find that this term vanishes for p -# q. For p = q it contains the mean current,

(2.16)

For a time-independent mean current Jp one has a white-noise spectrum C~~) (0,0') =

21f6pq6(0 + O')Jp- This is the usual shot noise, corresponding to Poissonian statistics of the current fluctuations. The second term C~~) describes the deviations from Poissonian statistics. It arises from terms in Eq. (2.14) that are quadratic in n. Performing again an integration by parts, one finds

C(2)(0 0') = 2D J dSa J dS' J dr" J dO" an(r", 0 + 0") an(r" , 0' - 0") pq' P f3 21f ar" ar"

Sp Sq V ry ry

ac ( r , r", 0) ac ( r' , r", 0') x a a ' . (2 .17) ra rf3

Equation (2.17) together with Eq. (2.8) is the result that we need for our analysis of the frequency dependence of the noise spectrum.

c. Amplifying medium

The extension of our general formulas to an amplifying medium (in the linear regime below the laser threshold) is straightforward [9]: We assume that the frequency w at which we are detecting the radiation is close to the frequency of an atomic transition with (on average) Nupper and Nlower atoms in the upper and lower state. Then the Bose-Einstein function can be replaced by the population inversion factor f = Nupper(Nlower - Nupper )-1. This factor is negative in the amplifying case (when Nupper > Nlower) , with f = -1 for a complete population inversion. (Equivalently, one can evaluate f at a negative temperature [11], with T ---+ 0- for complete inversion.) An amplifying medium has a negative absorption time Ta = ~;I D. We can account for this by taking ~a imaginary. With these two substitutions for f and ~a our formulas for an absorbing medium carryover to the amplifying case.

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x = 0 L-' ________ ---', X = L

FIG. 2. Thermal radiation (solid arrows) is incident on a waveguide containing an absorbing or amplifying disordered medium. The transmitted radiation (dashed arrows) is absorbed by a photo detector .

III. WAVEGUIDE GEOMETRY

For the application of our general formulas we consider a waveguide geometry (see Fig. 2). The waveguide has length L and cross-sectional area A, corresponding to N = w2 A/41fc2

propagating modes (not counting polarizations) at frequency w. We abbreviate 8 = L/~a. We consider a stationary incident current 10 = icAbwnin = (N bw /21f p )nin, and calculate the noise power spectrum of the transmitted current ,

00

P(O) = J dt eiDt bI(t)bI(O). (3.1) -00

In terms of the correlator of the previous section, one has Cl1 (O, 0') = 21fP(0)b(0 + 0').

A. Absorbing medium

We calculate the noise power from Eqs. (2.8) and (2.17), using the Green function

where x< and x> are the smallest and largest of x, x', respectively. The mean photon density is time independent. In Fourier representation one has, from Eq. (2.8) ,

n(x,O) = 21fb(0) .pfh

(sinh 8 - sinh (x/~a) - sinh (8 - X/~a)) sm 8

5:(n)- sinh (8 - x/~a) + 21fU H nin . h . sm 8

(3.3)

The mean current I = Ith + Itrans is the sum of the thermal radiation from the medium

- 4Df Ith = -(Nbw/21f) tanh (8/2)

c~a

and the transmitted incident current

- 4DIo Itrans = ~ . h .

c a SIn 8

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(3.4)

(3.5)

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Substitution of Eqs. (3.2) and (3.3) into Eq. (2.17) yields the super-Poissonian noise P - 1 as a sum of three terms, P - 1 = Pth + Ptrans + Pex , with

Pth(O) = 8~12 (Nflw/27r) JS ds' (COSh (s ~ s; - COShS,)2 K(s', s) , C"'a sm s o

(3.6)

8D12 JS cosh2 (s - s') Ptrans(O) = T(27r/Nflw) ds' . 2 K(s', s),

C"'a smh s o (3.7)

Pex(!1) = 16~f 10 JS ds' [cosh s' - cosh ~s ~ s')] cosh (s - s') K(s' , s). C a smh s o

(3.8)

We have defined

K(s' s) = ISinh(s'Jl- iOTa) 12 , sinh(sJl - iOTa)

(3.9)

The two terms Ptrans and Pth describe separately the noise power of the transmitted incident current and of the thermal current from the medium. The term Pex is the excess noise due to the beating of the incident radiation with the thermal fluctuations from the medium.

The three contributions are plotted separately in Fig. 3. For L ยป ~a the frequency dependence simplifies to

R (0) = 11th th 1 + x'

R (0) = C"'a trans (2 /N fl) - e x C 12 (1 -2s(x-1) 3 +2) trans 16D 7r w x-I + -X-'--2 -+-x '

- 1 + 2x Pex(O) = I1trans + 2 '

X X

w here we have defined

X = Re VI - iOTa = [~(1 + 02T;)1/2 + ~P/2.

(3.10)

(3.11)

(3.12)

(3.13)

As discussed in Ref. [9] (for the zero-frequency case) the result for Ptrans requires that the incident radiation is in a thermal state, at some temperature To. (The quantity l(w, To) = 10 (27r/Nflw) is the corresponding value of the Bose-Einstein function.) There is no such requirement for Pth and Pex , which are independent of the incident state. For To ยป T we may generally neglect Pth and Pex relative to Ptrans , so that P = Itrans + Ptrans. However, if the incident radiation is in a coherent state, then Ptrans - 0 and since for sufficiently large 10

we may neglect Pth , we have in this case P = Itrans + Pex . The contribution Pth is important mainly in the absence of external illumination, when P = Ith + Pth .

B. Amplifying medium

The results for an amplifying medium are obtained by the substitution ~a ---+ i~a, 1 ---+

Nupper(Nlower - Nupper )-1, d. Sec. IIC. The frequency dependence of Pth , Ptrans, and Pex following from Eqs. (3.6)-(3.8) is plotted in Fig. 4 for lengths L below the laser threshold at L = 7r~a.

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213s = 1 ๏ฟฝaP th=f๏ฟฝ I th

0 1 2 3 4 50

0.2

0.4

s = 21510P trans=Z๏ฟฝ I2 trans

0

1

2

s = 1123P ex=f๏ฟฝ I trans

0

0.5

1

1.5

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โˆโœ’ โˆโœ“โœ”โœ•โœ•โœ—โœšโœ”โœ“โœ“โœ›โœœโœขโœฃโœ”โœ“

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โโฏโฑโฒโณโจ โƒโปโผโฝโฑ

โพโฟโœโฒโž€โ‘คโžโž‚โนโžƒโจ

โž„โญ

โž…

โซโž†โž‡

โžˆโœฏโœดโœฌโ˜… โฒโž† โž‰ โž†โž‡โจ โž‰ โœฏโœดโœฌโ˜… โž†โž‡

โœฌโœผโœฅโ˜… โž†

โžŠโฑ

โป

22:5

s = 1:5 ๏ฟฝaP th=jfj๏ฟฝ I th

0 1 2 3 4 50

2

4

6

s = 1:52 2:5P trans=Z๏ฟฝ I2 trans0

0.5

1

1.5

s = 1:522:5P ex=jfj๏ฟฝ I trans

0

5

10

โ‹โ– โ—โœณ โœนโœณ โ™โ›โ™ โก โ›s โ‹โœโฃโœณ โœธโœฑ โขโ™ฆr tโคโก โโ›sโก โ™ฆโข โ›โ™ฅ โ›โ™ โ™ฃโงโœโขโ‘กโœโ™ฅโฃ โœ‡โ›โœˆโกโฃโœ‰โœโžโกโœณ โšโคโก โงโ›sโกr tโคrโกsโคโ™ฆโงโž โ™ฆโโโœ‰rs โ›t

๏ฟฝ โ‚ โœ™โœณ

โœ‚โœโœ„โ˜Žโœ†โฌโœโœต

โœžโœถ โœŸ โœ โœกโœœโ˜›โช โœโœ„โ˜Žโœ†โฌโœญโœ โœŸ โœ

โœตโœฎโœžโœถ โœฐ โœ โœกโœœโ˜›โช

โฅ โœโœ„โ˜Žโœ†โฌโœโœžโœถ โœŸ โœ โœกโœœโ˜›โชโฅ

โœทโœฟ โœญโ˜žโœŒโœถโœบโœฎ

โœโœ†โœŽ โœโœ‘โœ’โœโœโœฒโœโœ’โœ‘โœ‘โœŽโœ“โœ”โœ•โœ’โœ‘ โœ„โœ โœ–โœ“โœ’โœ•โœ•โœŽโœ— โœ„โ˜Ž โœ˜โœ„โœšโœŒ โœบ โœ›โœ’โœ‘ โœโœ’โœ•โœ† โœ•โœ†โœŽ โœ”โœโœโœ’โœ‘โœโœ„โ˜Žโœš โœ”โ˜Žโœ— โœ”โœขโœ–โœ“โœ„โœ›โœฃโœ„โ˜Žโœš โœโœ”โœโœŽโœโœŒ โœโœ†โœŽ

โœ’โœคโœ•โœšโœ’โœ„โ˜Žโœš โœโœคโœ‘โœ‘โœŽโ˜Žโœ•โœ โœ”โœ• โœ•โœ†โœŽ โœ•โœฅโœ’ โœŽโ˜Žโœ—โœ โœ’โœ› โœ•โœ†โœŽ โœฅโœ”โœฆโœŽโœšโœคโœ„โœ—โœŽ โœ”โœ‘โœŽ โœ”โ˜Žโœ•โœ„โœฒโœโœ’โœ‘โœ‘โœŽโœ“โœ”โœ•โœŽโœ— โœ›โœ’โœ‘ โœกโœœโ˜› โœง โœถโœŒ

โ˜…โฑโœฉ โˆโ–โ–ผPโ†โœชโ˜…โœซโ–โ—† โฒโ˜…โœฌโ โ——โฏโ†โ—†โœฌโฏโ–ผ โœฌโโŠโ–โœชโจ

โœฏ โœ›โœคโœ“โœ“โœฃ qโœคโœ”โ˜Žโœ•โœคโœข โœขโœŽโœโœ†โœ”โ˜Žโœ„โœโœ”โœ“ โœ•โœ†โœŽโœ’โœ‘โœฃ โœ›โœ’โœ‘ โœ•โœ†โœŽ โœ–โœ†โœ’โœ•โœ’โœโœ’โœคโ˜Žโœ• โœ—โœ„โœโœ•โœ‘โœ„โœโœคโœ•โœ„โœ’โ˜Ž โœ’โœ› โœ” โœ—โœ„โœโœ’โœ‘โœ—โœŽโœ‘โœŽโœ—

โœขโœŽโœ—โœ„โœคโœข โœฅโœ”โœ โœ—โœŽโœฆโœŽโœ“โœ’โœ–โœŽโœ— โœ„โ˜Ž โ˜โœŽโœ›โœโœŒ โฌโœผโœดโœฝโชโœŒ โœปโ˜Ž โœ•โœ†โœ„โœ โœโœŽโœโœ•โœ„โœ’โ˜Ž โœฅโœŽ โœฆโœŽโœ‘โœ„โœ›โœฃ โœ•โœ†โœ”โœ• โœ„โœ• โœ”โœšโœ‘โœŽโœŽโœ โœฅโœ„โœ•โœ† โœ•โœ†โœŽ

โœโœŽโœขโœ„โœโœ“โœ”โœโœโœ„โœโœ”โœ“ โœ‘โœŽโœโœคโœ“โœ•โœ โœ’โœ› โœ•โœ†โœŽ โœ–โœ‘โœŽโœฆโœ„โœ’โœคโœ โœโœŽโœโœ•โœ„โœ’โ˜ŽโœŒ โœพโœŽ โœโœ’โ˜Žโœโœ„โœ—โœŽโœ‘ โœ•โœ†โœŽ โœโœ”โœขโœŽ โœโœฃโœโœ•โœŽโœข โœ’โœ› โœ˜โœ„โœšโœŒ โ€โœด โœ” โœ—โœ„โœโœฒ

โœ’โœ‘โœ—โœŽโœ‘โœŽโœ— โœฅโœ”โœฆโœŽโœšโœคโœ„โœ—โœŽ โœฅโœ„โœ•โœ† โœ” โœ–โœ†โœ’โœ•โœ’โœ—โœŽโœ•โœŽโœโœ•โœ’โœ‘ โœ”โœ• โœ’โ˜ŽโœŽ โœŽโ˜Žโœ— โœ”โ˜Žโœ— โœ” โœโœ•โœ”โœ•โœ„โœ’โ˜Žโœ”โœ‘โœฃ โœโœคโœ‘โœ‘โœŽโ˜Žโœ• โœ„โ˜Žโœโœ„โœ—โœŽโ˜Žโœ• โœ”โœ• โœ•โœ†โœŽ

โœ’โœ•โœ†โœŽโœ‘ โœŽโ˜Žโœ—โœŒ โœพโœŽ โœ”โœโœโœคโœขโœŽ โœ•โœ†โœ”โœ• โœ•โœ†โœŽ โœ„โ˜Žโœโœ„โœ—โœŽโ˜Žโœ• โœโœคโœ‘โœ‘โœŽโ˜Žโœ• โœ’โœ‘โœ„โœšโœ„โ˜Žโœ”โœ•โœŽโœ โœ›โœ‘โœ’โœข โœ” โœ•โœ†โœŽโœ‘โœขโœ”โœ“ โœโœ’โœคโœ‘โœโœŽ โœ”โœ• โœ•โœŽโœขโœฒ

โœ–โœŽโœ‘โœ”โœ•โœคโœ‘โœŽ โโƒโœŒ โœโœ†โœŽ โœ–โœ†โœ’โœ•โœ’โœโœ’โœคโ˜Žโœ• โœ—โœ„โœโœ•โœ‘โœ„โœโœคโœ•โœ„โœ’โ˜Ž โœ„โœ โœ•โœ†โœŽ โœ—โœ„โœโœ•โœ‘โœ„โœโœคโœ•โœ„โœ’โ˜Ž โœ’โœ› โœ•โœ†โœŽ โ˜ŽโœคโœขโœโœŽโœ‘ โœ’โœ› โœ–โœ†โœ’โœ•โœ’โ˜Žโœ โ„โœญโ…โœฎ

โ‡

C C H

~ :> c rt :::J 0 H

~ ~ ~ c (fJ

n H ...... ~ rt

c c

University of Utah Institutional Repository Author Manuscript

0.8

0.6

r:( 0.4

----N

~ 0.2

0

-0.2

0.2

~

~ ~ 0.1 ~

0

0

s=l

2

2.5

4 nTa

6 8

FIG. 5. Frequency dependence of the cross-correlator of the outgoing current at the two ends of the waveguide, in the absence of any external illumination. Computed from Eq. (3.15) for the absorbing case (lower panel) and amplifying case (upper panel).

counted (with unit quantum efficiency) in the time interval (0, t). Substitution of I = dn/dt in the definition (3.1) of the noise power p(n) leads to a relation with the variance Varn(t) of the photocount ,

00

p(n) = _n2 J dtVarn(t) cos nt, o

2 00

Var n(t) = -; J dn n-2 p(n) (cos nt - 1). o

(4.1a)

(4.1 b)

The variance can be separated into two terms, Varn(t) = n(t) + K,(t) = tl + K,(t), with K,(t) the second factorial cumulant. The term tI, substituted into Eq. (4.1a) , gives the frequency-independent shot noise contribution I to the power spectrum,

00

p(n) = I - n2 J dt K,(t) cos nt. o

( 4.2)

The cumulant K, = K,trans + K,th + K,ex contains separate contributions from the transmitted incident radiation and thermal fluctuations in the medium, plus an excess contribution from the beating of the two. These contributions have an exact representation in terms of the N x N reflection and transmission matrices r(w), t(w) of the waveguide [7,8],

10

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ood ood I

K;trans(t) = 1 ~ 1 ~L(w - w', t) f(w, To)f(w' , To)TrT(w)T(w/), 27r 27r o 0

K;th(t) = 100

dw roo dw' L(w - w', t) f(w, T)f(w', T)TrQ(w)Q(w/),

27r Jo 27r o 00 00 I

K;ex(t) = 1 dw 1 dw L(w - w', t) 2f(w, To)f(w' , T)TrT(w)Q(w/), 27r 27r o 0

w here we have defined

t t

L(w, t) = 1 dt' 1 dt" exp[iw(t' - til)] = 2w-2(1 - coswt) , o 0

Q(w) = n - r(w)rt(w) - t(w)tt(w) ,

T(w) = t(w)tt(w).

(4.3)

( 4.4)

( 4.5)

(4.6)

(4.7) (4.8)

Substitution into Eq. (4.2) gives the corresponding contributions to the noise power P = J + Ptrans + Pth + Pex ,

1 00 dw Ptrans(O) = "21 27r f (w, To)f(w + 0, To)TrT(w)T(w + 0) + {O --+ -O} ,

o 00

Pth(D) = ~ 1 dw f(w , T)f(w + D, T)TrQ(w)Q(w + D) + {O --+ -O} , 2 27r

o 1 00 dw

Pex(O) = "21 27r 2f(w , To)f(w + 0 , T)TrT(w)Q(w + 0) + {O --+ -O}. o

(4.9)

(4.10)

(4.11 )

As in the previous section, we assume a frequency-resolved measurement in an interval 6w ยซ w, I/Tcoh with 0 ยซ 6w. We may then omit the integral over wand approximate the argument w ยฑ 0 in the functions f by w. We take the ensemble average ( ... ) of the noise power, in which case the contributions from ยฑO are the same. Finally, we insert the incident current 10 = f(w , To)N 6w /27r , to arrive at

Ptrans(O) = (27r/N6w)15(N- 1TrT(w)T(w + 0)),

Pth(O) = (N6w/27r)f2(W , T)(N-1TrQ(w)Q(w + 0)) , Pex(O) = 210f(w, T)(N-1TrT(w)Q(w + 0)).

(4.12)

(4.13)

(4.14)

It remains to evaluate the ensemble averages. This is done in the appendix, by extending the approach of Ref. [13] to correlators of reflection and transmission matrices at different frequencies. The calculation applies to the diffusive regime that the length L of the waveguide is large compared to the mean free path l, but still small compared to the localization length Nl. (The absorption length ~a is also assumed to be ยป l.) The results are

11

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University of Utah Institutional Repository Author Manuscript

(N-1TrT(w)T(w + 0)) = 8~ J8 ds' K(s', s) cosh.2(s2- s'),

C<."a smh s o

(N-1Tr Q(w)Q(w + 0)) = 8~ J8 ds' K(s' , s) [cosh s' -.co~h(s - S')]2, C<."a smh s o

(N-1TrT(w)Q(w + 0)) = 8~ J8 ds' K(s' , s) cosh(s - s') co~hs~ - cosh2(s - s'), C<."a smh s o

(4.15)

( 4.16)

( 4.17)

where s = L/~a and the kernel K(s' , s) is defined in Eq. (A29). The combination of Eqs. (4.12)- ( 4.17) agrees precisely with the results (3.6)- (3.8) of the semiclassical theory. The quantum theory is more general than the semiclassical theory, because it can describe the effects of wave localization. The method of Ref. [13] gives corrections to the above results in a power series in LI Nl. We will not pursue this investigation here.

v. DISCUSSION

We have presented a theory for the frequency dependence of the noise power spectrum P(O) in an absorbing or amplifying disordered waveguide. The frequency dependence is governed by two time scales, the absorption or amplification time Ta and the diffusion time L2 I D , both of which are assumed to be much greater than the coherence time Tcoh. A simplified description is obtained, in the absorbing case, for lengths L much greater than the absorption length ~a = V DTa , and, in the amplifying case, close to the laser threshold at L = 7r~a. We will discuss these two cases separately.

A. Absorbing medium

The general formulas (3.6)- (3.8) for P = 1 + Pth + Ptrans + Pex simplify for L ยป ~a to Eqs. (3.10)- (3.12). To characterize the frequency dependence we define the characteristic

C frequency Oc as the frequency at which the super-Poissonian noise has dropped by a factor C of two:

In the absence of any external illumination (10 = 0) we have, from Eq. (3.10),

P = Ith (1 + _1_) , l+x

- 4D1 Ith = -(NfJw/27r) ,

c~a

(5.1)

(5.2)

with x = Re VI - iOTa, hence Oc = 17 ITa. If the illumination is in the coherent state from a laser, then we have, from Eq. (3.12),

- ( 1 + 2X) P = Itrans 1 + 1 2' X+X

12

- 8DIo -8

Itrans = -c-e , C<."a

(5.3)

c c

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University of Utah Institutional Repository Author Manuscript

o 0.9 0.95

L/7r~a

FIG. 6. Ratio of l;h and Pth in an amplifying waveguide as a function of its length for different frequencies, computed from Eqs. (3.4) and (3.6). The approximation (5.5) valid near threshold for small frequencies is shown dashed.

here Oc = 9/Ta . In both these cases the diffusion time does not enter in the frequency dependence. This is different for illumination by a thermal source at temperature To much greater than the temperature of the medium. From Eq. (3.11), with fo = f(w, To), we then have

- ( fi [1 - e-2s(x-1) 3x + 2])

Ptrans(O) = Itrans 1 + 20 e-

s x-I + x 2 + X . (5.4)

The characteristic frequency Oc = (64D / L2T:) 1/4 now contains both the diffusion time and the absorption time.

B. Amplifying medium

In the amplifying case the noise power becomes more and more strongly peaked near zero frequency with increasing amplification. Close to the laser threshold at s = 7r the frequency dependence of Pth for small frequencies OTa ยซ 1 has the form

zI;h Pth = ---------27r[02T~ + 4(1 - S/7r)2] ,

- 4f Ith = Z (7r - s)" (5.5)

Here again Z = (c~a/2D) (27r / N bw ). Close to threshold the peak in the noise power spectrum has a Lorentzian lineshape with half-width Oc = (2/Ta)(1 - L/7r~a). At the laser threshold both Pth and Ith diverge, but the ratio I;h/ Pth remains finite (see Fig. 6).

Finally, we note the fundamental difference between the time scales appearing in the noise spectrum for photons, on the one hand, and electrons, on the other hand. The absorption or amplification time Ta obviously has no electronic analogue. The diffusion time L2 / D appears in both contexts, however, the electronic noise spectrum remains frequency independent for o > D / L2 [14]. The reason for the difference is screening of electronic charge. As a result the characteristic frequency scale for electronic current fluctuations is the inverse scattering time D /l2, which is much greater than the inverse diffusion time D / L2.

13

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University of Utah Institutional Repository Author Manuscript

ACKNOWLEDGMENTS

We thank P. W. Brouwer for advice concerning the calculation in the appendix and Yu. V. Nazarov and M. P. van Exter for useful discussions. This research was supported by the "Nederlandse organisatie voor Wetenschappelijk Onderzoek" (NWO) and by the "Stichยญting voor Fundamenteel Onderzoek der Materie" (FOM). E. G. M. also thanks the Russian Foundation for Basic Research.

APPENDIX A: CORRELATORS OF REFLECTION AND TRANSMISSION MATRICES

To compute the noise power spectrum in the quantum mechanical approach of Sec. V, we need the correlators of reflection and transmission matrices t(wยฑ) and r(wยฑ) at two different frequencies wยฑ = w ยฑ D/2. (For D ยซ w this is the same as the correlator at frequencies w and w + D.) We calculate these correlators for a waveguide geometry in the diffusive regime, by extending the equal-frequency (D = 0) theory of Brouwer [13].

Upon attachment of a short segment of length <5 L to one end of the waveguide of length L , the transmission and reflection matrices change according to

t ---+ tOL(l + rrOL)t,

r ---+ r~L + toL (l + rrOL)rtgL'

(Ala)

(Alb)

where the superscript T indicates the transpose of a matrix. (Because of reciprocity the transmission matrix from left to right equals the transpose of the transmission matrix from right to left.) The transmission matrix toL of the short segment at frequency wยฑ may be chosen proportional to the unit matrix,

toL = 1-----ยฑ-- n. (

<5L <5L iD<5L) 2l' 2c'Ta 2c'

(A2)

C The mean free path l' = 4l/3 and the velocity c' = c/2 represent a weighted average over C the N transverse modes in the waveguide. ~ U nitarity of the scattering matrix dictates that the reflection matrix from the left of :> the short segment is related to the reflection matrix from the right by rh = -r JL. We g abbreviate roL = <5r. The matrix <5r is symmetric (because of reciprocity), with zero mean ::r-' o and variance H

~ ~ ~ C (fJ

n H The resulting change in the matrix products ttt and rrt is ~. rt

ttt ---+ (1 - <5L/l' - <5L/C'Ta)ttt + (r<5rt)(r<5rt)t

+ r<5rttt + (r<5rttt) t,

rrt ---+ (1 - 2<5L/l' - 2<5L/c'Ta)rrt + (r<5rr) (r<5rr)t + <5rt<5r

+ r<5rrrt + (r<5rrrt)t - r<5r - (r<5r)t.

14

(A3)

(A4a)

(A4b)

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University of Utah Institutional Repository Author Manuscript

The frequency 0 does not appear explicitly in these increments. We define the following ensemble averages

R = (N-1Tr (n - rrt)),

C = (N-1Tr (n - r _r~)), T = (N-1Tr ttt),

(A5)

(A6)

(A7)

where r, t are evaluated at frequency wand r ยฑ, tยฑ at frequency w ยฑ 0/2. Similarly, we define the correlators

Crr = (N-1Tr (n - r _r~)(n - r +r~)),

Crt = (N-1Tr (n - r _r~)t+t~) , Ctt = (N-1Tr t_t~t+t~).

(AS)

(A9) (A10)

We will see that , in the diffusive regime, these 6 quantities satisfy a coupled set of ordinary differential equations in L.

The diffusive regime corresponds to the large-N limit, in which the length L of the waveguide is much less than the localization length Nl. In this limit we may replace Eq. (A3) by (6rkl6r":nn) = (6L/Nl')6km6ln. In the large-N limit we may also replace averages of products of traces by products of averages of traces. From Eq. (A4) we thus obtain the diffential equations

,dR ( ) 2 l dL = 2, 1 - R - R ,

l':~ = 2,(1 + iOTa)(l- C) - C2,

,dT T T l- = -'\I - R dL I ,

de l' d{r = -(4, + C + C* + 2R)Crr + 2R(R + 2,),

,dCrt ( *) () l dL =- 3,+C+C +RCrt -TCrr +2 R+,T,

, dCtt ( *) T T2 l dL = - 2, + C + C Ctt - 2 Crt + 2 ,

(All)

(A12)

(A13)

(A14)

(A15)

(A16)

with the definition, = l' / e' Ta. The initial conditions are that each of these 6 quantities ---+ 1 for L ---+ o.

This set of differential equations may be simplified further if we assume, as we did in the semiclassical theory, that the mean free path is small compared to both the absorption length and the length of the waveguide. All 6 quantities (A5)-(A10) are of order .;1, which is ยซ 1 if l' ยซ e'Ta , so that we obtain in leading order

,dR 2 l dL = 2, - R ,

l' :~ = 2,(1 + iOTa) - c2,

15

(A17)

(A1S)

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University of Utah Institutional Repository Author Manuscript

l,dT = -RT dL '

l,dCrr = -(C + C* + 2R)C + 2R2 dL IT,

, dCrt ( * ) l dL = - C + C + R Crt - TCrr + 2RT,

l,d~t = -(C + C*)Ctt - 2TCrt + 2T2.

(A19)

(A20)

(A21)

(A22)

As initial condition we should now take that the product of each quantity with L remains finite when L ---+ O.

Although the differential equations are coupled, they may be solved separately for R, C, T, Crr, Crt, Ctt, in that order. In terms of the rescaled length s = (21)1/2 LIl' = L/~a, the results are

(21 )1/2 R=--'--------'-------

tanh s ' C = (21 ) 1/2 y''-'"""1 -+----:-iO=-T.-a

tanh SV1 + iOTa' (21 )1/2

T = --'--------'---sinh s '

( )1/2 s

C 81 J d ' K(') h2 , rr = . 2 S S ,S cos s, smh s o ( )1/2 s

Crt = ~1 2 J ds' K (S' , S) cosh( s - s') cosh s', smh s

o ( )1/2 s

Ctt = ~1 2 J ds' K(s' , S) cosh2(s - S'), smh s

o

where the kernel K is defined by

(A23)

(A24)

(A25)

(A26)

(A27)

(A28)

(A29)

These are the expressions used in Sec. 4 (where we have also substituted v'21 = 4Dlc~a).

The remaining integrals over s' may be done analytically, but the resulting expressions are rather lengthy so we do not record them here. For 0 = 0 our results reduce to those of Brouwer [13] (up to a misprint in Eq. (13c) of that paper, where the plus and minus signs in the expression between brackets should be interchanged).

16

c c

c c

University of Utah Institutional Repository Author Manuscript

REFERENCES

[1] R. Loudon, The Quantum Theory of Light (Clarendon, Oxford, 1983). [2] J. D. Bekenstein and M. Schiffer, Phys. Rev. Lett. 72 , 2512 (1994). [3] M. Schiffer, Gen. ReI. Grav. 27, 1 (1995). [4] C. T. Lee, Phys. Rev. A 52, 1594 (1995) . [5] F. Egbe, K. 1. Seo, and C. T. Lee, Quantum Semiclass. Opt. 7, 943 (1995). [6] V . Buzek, D. S. Krahmer, M. T. Fontenelle, and W . P. Schleich, Phys. Lett . A 239, 1

(1998) . [7] C. W. J. Beenakker, Phys. Rev. Lett. 81 , 1829 (1998); reviewed in: Diffuse Waves

in Complex Media, J.-P. Fouque, ed., NATO Science Series C531 (Kluwer, Dordrecht, 1999).

[8] M. Patra and C. W. J. Beenakker, Phys. Rev. A 60 , 4059 (1999); Phys. Rev. A (to be published).

[9] E. G. Mishchenko and C. W. J. Beenakker, Phys. Rev. Lett. 83, 5475 (1999). [10] J. R. Jeffers , N. Imoto, and R. Loudon, Phys. Rev. A 47, 3346 (1993). [11] R. Matloob, R. Loudon, M. Artoni , S. M. Barnett , and J. Jeffers, Phys. Rev. A 55,

1623 (1997). [12] H. Cao, Y. G. Zhao, S. T. Ho, E. W. Seelig, Q. H. Wang, and R. P. H. Chang, Phys.

Rev. Lett. 82, 2278 (1999). [13] P. W . Brouwer, Phys. Rev. B 57, 10526 (1998). [14] Ya. M. Blanter and M. Biittiker, Phys. Rep. (to be published).

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