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Transcript of Engineering and Control of Cold Molecules N. P. Bigelow University of Rochester.
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Engineering and Control of Cold Molecules
N. P. BigelowUniversity of Rochester
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Why Cold (Polar) Molecules ?
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Why Cold (Polar) Molecules ?
Talks from:Shlyapnikov
PfauBurnett
Sengstock...
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Why Cold (Polar) Molecules ?
Talks from:Shlyapnikov
PfauBurnett
Sengstock...
More Reasons Later in Talk
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So what about cold molecules?
Hard to find cycling transitions
Laser cooling of molecules is hard if not impossible
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Doyle approach - Thermalizationwith cold helium gas &
magnetic trapping
Dilution Refrigerator
~mKParamagnetic molecules
Large samples
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Meijer - time and spatially varying E fields – decelerator –
(à la high-energy in reverse; H. Gould)
accelerate
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Meijer - decelerator (à la high-energy; H. Gould)
decelerate
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Here
“Build” the molecules
from a gas of
pre-cooled atoms
via photoassociation
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A Quick Review ofPhotoassociation
Starting with Homonuclears
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Molecular potentials
Ground state
Singly excited state
Homonuclear
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Photoassociation
Ground state
Singly excited state
photon
600-1000Å
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Ground state molecule formation?
Ground state
Excited state
photon
Sp. emission
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(transition rate) (collision rate& pair distribution)*
(excitation rate)*(survival rate)*(process probability)*
(density2)*(volume)
These factors determine molecular production rates
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Ground state molecule formation
photon
Sp. emission
i
f
Poor Franck-Condon factors are discouraging f i 0
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In 1997 Pierre Pillet and co-workers startled the community
by showing the Cs2 ground-state molecules were produced
in a conventional optical trap
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R-transfer methodFrank-Condon Matching
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Why not heteronuclear molecules?
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Molecular potentials
Ground state
Singly excited state
Far better Franck-Condon factors….
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We might be CLOBBERED by the pair distribution function
Rhomo/Rhetero = 950/76 ~ 13
(Rhomo/Rhetero = 950/76 ~ 1/10)2 ~ 100 !
The interaction time is also smaller by a factor of ~ 13!
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Nevertheless, several groups
built multi-species MOTs -
including Rochester and Sao Carlos and
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Kasevich
Arimondo
Ingusio
Weidemuller
Windholz
DeMille
Stwalley/Gould
Wang/Buell
Ruff
others
Bose-Fermi&Isotopic: Jin, Salamon, Ertmer, Ketterle, Hulet, Sengstock…
Sukenik
NaCsNaKNaRbRbCsKRbLiCsLiNa
?
Most “reactive”
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We started with Na + Cs
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Search for ground state molecules - the detection pathway
20-200 J 9ns 580-589 nm 2 mm2
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NaCs formation and detection
Traps
100J pulse @ 575-600nm
time (s)
-30 0 20 105
9ns
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Choice of pulsed laser wavelength
575-600 nm was chosen
To implement a resonant ionization pathway
It has enough energy to 2-photon ionize
NaCs
It will NOT resonantly ionize Cs
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0
500
1000
1500
2000
2500
0 5 10 15 20
Time (s)
Co
un
t Na+Cs
Cs
Na
Na+Cs Lin Scale Zoomphotons
cold Na
Thermal Na
Cold Cs
Cold NaCs
Cs2Na2
Time of Flight
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Is NaCs formed by the ionizing pulse ?
Traps
Ionizing Pulse
time (s)
-30 -15 0 20 105
9ns
Na-push beam
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Push –beam experiment
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How cold are the molecules?
We use time-of-flight from the interaction zone as our probe
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0
10
20
30
40
50
60
70
80
90
100
12.6 12.8 13 13.2 13.4 13.6
Time (s)
Co
un
t
21
100
500
1000
2000
3000
4000
4500
4980
NaCs Temp
TNaCs ~ 260 K0.2 m/s
(kinetic temp)
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KNaCs : The rate of formation
We detect 500 molecules in 10,000 pulses
Estimate ionization and detection efficiency ~ 10%
Kinetic model : 90% of NaCs drifts out of the
trapping region between pulses.
Production rate ~ 50 Hz
d [NaCs] / dt = KNaCs [Na][Cs]
KNaCs ~ 7.4 x 10-15 cm3 s-1
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Measured depth of the triplet is 137-247 cm-1
Neumann & Pauly Phys. Rev. Lett. 20, 357-359 (1968).
and J. Chem. Phys. 52, 2548-2555 (1970)
We have scanned 0 – 268 cm-1 and found strong ion signals
(includes 5% of singlet potential)
We have a mixture of singlets and triplets
C. Haimberger, J. Kleinert, npb PRA Rapid Comm.
70, 021402 (R) Aug 2004
NaCs has largest polarizability (measured) of all bi-alkalis
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Coherent Transfer - State Selective
Ro-vibrational ground state (lower dipole moment)or
Single excited ro-vibrational state
Incoherent transfer results already at Yale
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The most important partof this part of our work:
C. HaimbergerJ. Kleinert
(M. Bhattacharya, J. Shaffer & W. Chalupczak)
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KRb
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RbCs
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40,000 molecules/sec !!
KRb
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Franck-Condon Factors for hetero-pairs based on long range (dispersion) potentials
Wang & Stwalley, J. Chem Phys.
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Cold (Polar) Moleculesand Quantum Information
0
500
1000
1500
2000
2500
0 5 10 15 20
Time (s)
Co
un
t Na+Cs
Cs
Na
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Polar Molecules Allow Coupling Enabling Quantum Information Applications
• Heteronuclear molecules are highly polarizable
• The dipole-dipole coupling of the molecules can be harnessed for quantum information applications (see protocols for EDMs in Quantum Dots - e.g. Barenco, et al PRL 82 1060)
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Polar Molecules Allow Couplings Enabling Quantum Information Applications(based on scheme by Côté, Yellin [Lukin])
-6
-5
-4
-3
-2
-1
0
1
0 10 20 30 40
Internuclear Separation (Å)
En
erg
y (
10
3 c
m-1)
atoms
boundmolecularstates
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Polar Molecules Allow Coupling Enabling Quantum Information Applications
-6
-5
-4
-3
-2
-1
0
1
0 10 20 30 40
Internuclear Separation (Å)
En
erg
y (
10
3 c
m-1)
atoms
boundmolecularstates
v, j 0
v , j 1
v , j v
•Start with two molecules in same state
Ai 0
Bi 0
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Polar Molecules Allow Coupling Enabling Quantum Information Applications
-6
-5
-4
-3
-2
-1
0
1
0 10 20 30 40
Internuclear Separation (Å)
En
erg
y (
10
3 c
m-1)
atoms
boundmolecularstates
v, j 0
v , j 1
v , j v
•Start with two molecules in same state
•Use Raman pulses - create superposition
Ai 0
Bi 0
A a0 0 a1 1
B b0 0 b1 1
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Polar Molecules Allow Coupling Enabling Quantum Information Applications
-6
-5
-4
-3
-2
-1
0
1
0 10 20 30 40
Internuclear Separation (Å)
En
erg
y (
10
3 c
m-1)
atoms
boundmolecularstates
v, j 0
v , j 1
v , j v
AB c00 00 c11 11 c01 01 c10 10
Two-molecule state:
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Polar Molecules Allow Coupling Enabling Quantum Information Applications
v, j 0
v , j 1
v , j v
(large dipole moment)
Now excite to the state
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Polar Molecules Allow Coupling Enabling Quantum Information Applications
v, j 0
v , j 1
v , j v
(large dipole moment)
AB c00 00 e ic11 11 c01 01 c10 10
Now excite to the state , wait an Interaction time then de-excite back to 1
Phase gate, CNOT gates etc. possible
“Dipole blockade and quantum information processing using mesoscopicAtomic ensembles”, Lukin, Fleischhauer, Côté, Duan, Jaksch, Cirac and ZollerPRL 87 037901
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A specific qubit platform
Each atom sees a local field that couples it to its neighbors and permits selective addressing
The coupling cannot be switched off but instead can be compensated using echo-type refocussing techniques of NMR.
What is needed is a source of cold molecules
D. DeMille, PRL 88, 067901
E a
E ext (xa )
E int (xa )
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Molecules and “Chips”
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Atom Chip
Si(1mm)
SiO2(250nm)
Ag(50nm)Cu(1mm)
+-- polarization
IB~15-20 A
IS~1-3 A
Y
Z
x
B=B0y
z0
z
y
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Our 1st Generation Atom Chips
20 mm
5 mm
2 mm
1 mm10 mm
y
x
w=250 m
h=1-5 m
J~ 106 A/cm2
Cross-section:
Current density:
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Trap
Image of Trap
Atom chip surface
Cold AtomicMixtures-on-a-chip
Rb-Cs
Holmes, Tscherneck, Quinto-su and Bigelow
Imaging of sample
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2nd Generation Chips
P. Quinto-Su, M. Tschernek, M. Holmes and N. P. Bigelow, On-chip detection of laser-cooled atoms, Optics Express, 12, 5098 (2004).
•Collaboration with Corning, Inc.
•<100 atom sensitivity
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3rd Generation Chips: Molecule Chips
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WHY OPTICS and MOLECULES ON THE CHIP?
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Optical Fiber
Probe/readout/control laser
WHY OPTICS and MOLECULES ON THE CHIP?
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4th Generation Chips
3 cm
Higher currentCapability
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Heroines and Heroesof this part of the work:
Michaela TscherneckMichael HolmesPedro Quinto-SuC. Haimberger
J. Kleinert
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Vortex Lattice in a Coupled
Atom-Molecule Condensate
(non-polar molecules)
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Single component atomic BEC - Triangular vortex lattice
Ω is rotation frequency
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Mean-field model
• Three scattering constants ga, gm and gam
• Coherent constant • Two Gross-Pitaevskii equations
Atom-Molecule BEC (homo-nuclear)
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Atom-Molecule BEC – Energies
– Two key types of interaction between atoms and molecules
• Coherent coupling
• Interspecies scattering
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Atom-Molecule BEC - rotating
(nv)m = 2(nv)a
Vortex density of molecular condensate istwice that of the atomic condensate
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Vortex Lattice in a Coupled Atom-Molecule Condensate
(non-polar molecules)
Sungjong Woo
Department of Physics & Astronomy
University of Rochester
Q-Han Park
Department of Physics
Korea University
![Page 71: Engineering and Control of Cold Molecules N. P. Bigelow University of Rochester.](https://reader034.fdocuments.net/reader034/viewer/2022051316/56649e205503460f94b0b05e/html5/thumbnails/71.jpg)
Summary
We can create cold diatomic polar molecules
We can create them and manipulate them on “chips”
There are interesting new aspects ofdegenerate systems involving molecules
![Page 72: Engineering and Control of Cold Molecules N. P. Bigelow University of Rochester.](https://reader034.fdocuments.net/reader034/viewer/2022051316/56649e205503460f94b0b05e/html5/thumbnails/72.jpg)
Summary
We can create cold diatomic polar molecules
We can create them and manipulate them on “chips”
There are interesting new aspects ofdegenerate systems involving molecules
Can you calculate your Archimedes factor?