A Kinetic Study of Hot Metal Desulphurization by Calcium ... · Calcium carbide Is one of the...
Transcript of A Kinetic Study of Hot Metal Desulphurization by Calcium ... · Calcium carbide Is one of the...
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A KIIETIC STUDY OF HOT ttETAL DESULPHURl-ZATION
BY CALCIU" CARBIDE PONDER INJECTION
by
(f) L. K. ChIang, B.Sc
A ThesIs
SubmItted to the School of Graduate StudIes
In PartIal FulFI I.lment .oF· the RequIrements
For the Degree
Doctor of PhIlosophy
~ McMaster UnIversIty
September, 1986
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P!3rmission has been granted to the National Library of Canada to microfilm this thesis' and to lend or sell copies of the film.
The a~or (copyright owner) has reserved other publication rights, and neither the thesis nor extensive extrac'ts from it may be printed or otherwise reproduced without his/her written permission.
ISBN
L'autorisation a ete accordee a la Bibliotheque nationale du Canada de microfilmer cette these et de prater, ou de vendre des exemplaires du film.
L' auteur (titulaire du droit d"auteur) se reserve les autres droits de publication; n1 la these, ni' de longs extra its de cel1e-ci ne doi vent atre ~mprJ.mes ou autrement reprod~its sans son autorisation ecrite.
0-315-35872_6
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A KINETIC STUDY OF HOT METAL DESULPHURIZATION
BY CALCIUM CARBIDE· POWDER INJECTION
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'Doctor or Ph I 10sdphy, (1986) j McMaster Un'iversity
HamIlton, Ontario
TITLE: A Kinetic Study of Hot Metal De~wlphurlzatlon
by Calcium Carbide Powder InJection. ,":, .
. ,-,' . ' \ AUTHOR: L I u-'Kyen Ch lang
B.Sc. National Cheng Kuhg University
Taiwan,' Republic of China
SUPERVISORS: Proressor G.A. Irons ,and Proressor W -K. Lu • \
NUMBER OF PAGES: xxx,327
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" ABsTRACT
curreritly, 'sulphur ~s the most problematic
Impurity which aFFects the physical and mechanical
propert I'es 0.'1" stee I. ThereFore a I I the I ntegrated s~E!e I
producers desulphurlze Iron beFore steelmaking. Calcium
carbide Is one of the reagents used to desulphurlze~ot
metal from the blast furnace, yet the kinetic reaction
phenomena are not c I ear. The present work was ! n,ft ! ated to
study the k. I n~t I cs of hot meta I desu I phur. I zat I on by "~ . calcium carbide powder Injection at the 3 Tonne scale.
The most Important variables which 'aFFect the rate
and eFFiciency of calcium carbide desulphu':"t.zatlon are the
type of top slag, the Injection conditions and the oxygen
activity In the hot metal •
. The present resu Its quant I tat I ve I y demonstrate
these eFf'ects.The experimental results Indlcl;lte that control
of the Initial s'iag condition can ef.Fect-ively Improve the, , .
rate and ef'FIciency of calcium carbldedesulphurlzatlon. It
was Found that lower solid loading Is klnetlcal!y ~avorab.le
f'or both s I ag/meta I and p (ume desu I phur! zat ! on. Oxygen
activity measur~ents show tha~,oxygen plays ~ crucial role
In desu I phur I zat ,-on, part I cu 1 ar.1 y to ach I eve' extra-:'1 ow
su I phur 1 eve 1 s. iii
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A'steedy-state. one-dimensional. three-phase model
was' developed to model the plume de~ulphurlzatlon' klnetlcs~ -'--The model permits e quantltatl"e analysis of the p,resent
" experimental' re~ults. The computed results from the model
·are Found to be conslstent'wlth, the experimental data.
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