Shell model calculations of nuclei around Pb · 2016-11-21 · 1. introduction 2. framework 3....

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Shell model calculations of nuclei around 208Pb

E.Teruya1 N.Yoshinaga1 K.Higashiyama2

1Department of Physics, Saitama University 2 Department of Physics, Chiba Institute of Technology

15/09/2016 INPC2016 in Adelaide

1. introduction

2. framework

3. results

4. summary

Outline of talk

・Shell model framework

・Energy levels

・E2, magnetic moments, and quadrupole moments

・ Backgrounds

・ About nuclei around 208Pb

・Truncation scheme

1. Introduction

introduction framework results summary

2

2

8

8

20

20

28

28

50

50

82

82

126

Half-life Range

Unknown

<0.1 s

0.1 - 5 s

5 - 100 s

100 s - 1 h

1 h - 1 y

1 y - 1 Gy

Stable

http://ie.lbl.gov/systematics/chart2000g.pdf

Introduction

◆ Nuclei around 208Pb

Neutron 126 Proton 82 Super-heavy

208Pb

126

82

◆ Systematic shell-model calculations

A~80, 100, 130, and so on

2

2

8

8

20

20

28

28

50

50

82

82

126

Half-life Range

Unknown

<0.1 s

0.1 - 5 s

5 - 100 s

100 s - 1 h

1 h - 1 y

1 y - 1 Gy

Stable

http://ie.lbl.gov/systematics/chart2000g.pdf

Introduction

◆ Nuclei around 208Pb Neutron 126 Proton 82 Super-heavy

208Pb

126

82

◆ Systematic shell-model calculations

A~80, 130, 200

208Ra 209Ra 210Ra 211Ra 212Ra 213Ra 214Ra 215Ra 216Ra 217Ra 218Ra 219Ra

207Fr 208Fr 209Fr 210Fr 211Fr 212Fr 213Fr 214Fr 215Fr 216Fr 217Fr 218Fr

206Rn 207Rn 208Rn 209Rn 210Rn 211Rn 212Rn 213Rn 214Rn 215Rn 216Rn 217Rn

205At 206At 207At 208At 209At 210At 211At 212At 213At 214At 215At 216At

204Po 205Po 206Po 207Po 208Po 209Po 210Po 211Po 212Po 213Po 214Po 215Po

203Bi 204Bi 205Bi 206Bi 207Bi 208Bi 209Bi 210Bi 211Bi 212Bi 213Bi 214Bi

202Pb 203Pb 204Pb 205Pb 206Pb 207Pb 208Pb 209Pb 210Pb 211Pb 212Pb 213Pb

201Tl 202Tl 203Tl 204Tl 205Tl 206Tl 207Tl 208Tl 209Tl 201Tl 201Tl 201Tl

Enlargement

2

2

8

8

20

20

28

28

50

50

82

82

126

Half-life Range

Unknown

<0.1 s

0.1 - 5 s

5 - 100 s

100 s - 1 h

1 h - 1 y

1 y - 1 Gy

Stable

http://ie.lbl.gov/systematics/chart2000g.pdf

Introduction

◆ Nuclei around 208Pb Neutron 126 Proton 82 Super-heavy

208Pb

126

82

◆ Shell model calculations

A~80, 130, 200

208Ra 209Ra 210Ra 211Ra 212Ra 213Ra 214Ra 215Ra 216Ra 217Ra 218Ra 219Ra

207Fr 208Fr 209Fr 210Fr 211Fr 212Fr 213Fr 214Fr 215Fr 216Fr 217Fr 218Fr

206Rn 207Rn 208Rn 209Rn 210Rn 211Rn 212Rn 213Rn 214Rn 215Rn 216Rn 217Rn

205At 206At 207At 208At 209At 210At 211At 212At 213At 214At 215At 216At

204Po 205Po 206Po 207Po 208Po 209Po 210Po 211Po 212Po 213Po 214Po 215Po

203Bi 204Bi 205Bi 206Bi 207Bi 208Bi 209Bi 210Bi 211Bi 212Bi 213Bi 214Bi

202Pb 203Pb 204Pb 205Pb 206Pb 207Pb 208Pb 209Pb 210Pb 211Pb 212Pb 213Pb

201Tl 202Tl 203Tl 204Tl 205Tl 206Tl 207Tl 208Tl 209Tl 201Tl 201Tl 201Tl

EDM

225Ra

EDM

Octupole

deformation

Magnetic

rotation

Low-lying νg9/2πh9/2 band

Ground state 1- (not 0-)

Enlargement

V. Margerin,

et al., PRC93

064309 (2016)

N.Cieplicka,

et al., PRC 86

054322 (2012)

L. Chen,

et al., PRL110

122502 (2013)

Introduction

・Shell model

D. Zwarts and P. W. M. Glaudemans, Z. Phys. A 320, 487 (1984).

E. Caurier, M. Rejmund, and H. Grawe, Phys. Rev. C67, 054310 (2003).

L. Coraggio, et. al., Phys. Rev. C 60, 064306 (1999).

◆ Systematic studies in theory

N=126

Z=82 L. Coraggio, et. al., Phys. Rev. C 58, 3346 (1998).

Single-closed nuclei

J. B. McGrory and T. T. S. Kuo, Nucl. Phys. A 247, 283 (1975).

Z=82 and N=126

Introduction

・Shell model

・Nucleon pair approximation Z. Y. Xu , et. al., Phys. Rev. C 79, 054315 (2009).

◆ Systematic studies in theory

Po isotopes T. R. McGoram, et. al., Nucl. Phys. A 637, 469 (1998).

Pb, Bi, Po, At, Rn, Fr

206Pb, 210Po, 208Bi C. W. Ma and W. W. True, Phys. Rev. C 8, 2313 (1972).

Po and Rn isotopes A. Zemel and J. Dobes, Phys. Rev. C 27, 2311 (1983).

Open-shell nuclei

・Interacting-boson approximation plus quasi-particle

2

2

8

8

20

20

28

28

50

50

82

82

126

Half-life Range

Unknown

<0.1 s

0.1 - 5 s

5 - 100 s

100 s - 1 h

1 h - 1 y

1 y - 1 Gy

Stable

http://ie.lbl.gov/systematics/chart2000g.pdf

82

Introduction

◆ What about A ~200 region

Neutron holes under 126 Proton particles over 82

Super-heavy nuclei

Around 208Pb

A~200

126 208Ra 209Ra 210Ra 211Ra 212Ra 213Ra 214Ra 215Ra 216Ra 217Ra 218Ra 219Ra

207Fr 208Fr 209Fr 210Fr 211Fr 212Fr 213Fr 214Fr 215Fr 216Fr 217Fr 218Fr

206Rn 207Rn 208Rn 209Rn 210Rn 211Rn 212Rn 213Rn 214Rn 215Rn 216Rn 217Rn

205At 206At 207At 208At 209At 210At 211At 212At 213At 214At 215At 216At

204Po 205Po 206Po 207Po 208Po 209Po 210Po 211Po 212Po 213Po 214Po 215Po

203Bi 204Bi 205Bi 206Bi 207Bi 208Bi 209Bi 210Bi 211Bi 212Bi 213Bi 214Bi

202Pb 203Pb 204Pb 205Pb 206Pb 207Pb 208Pb 209Pb 210Pb 211Pb 212Pb 213Pb

201Tl 202Tl 203Tl 204Tl 205Tl 206Tl 207Tl 208Tl 209Tl 201Tl 201Tl 201Tl

N≦126

Enlargement

N≧126

N=126

2

2

8

8

20

20

28

28

50

50

82

82

126

Half-life Range

Unknown

<0.1 s

0.1 - 5 s

5 - 100 s

100 s - 1 h

1 h - 1 y

1 y - 1 Gy

Stable

http://ie.lbl.gov/systematics/chart2000g.pdf

82

Introduction

◆ What about A ~200 region

Neutron holes under 126 Proton particles over 82

Super-heavy nuclei

Around 208Pb

A~200

126 208Ra 209Ra 210Ra 211Ra 212Ra 213Ra 214Ra 215Ra 216Ra 217Ra 218Ra 219Ra

207Fr 208Fr 209Fr 210Fr 211Fr 212Fr 213Fr 214Fr 215Fr 216Fr 217Fr 218Fr

206Rn 207Rn 208Rn 209Rn 210Rn 211Rn 212Rn 213Rn 214Rn 215Rn 216Rn 217Rn

205At 206At 207At 208At 209At 210At 211At 212At 213At 214At 215At 216At

204Po 205Po 206Po 207Po 208Po 209Po 210Po 211Po 212Po 213Po 214Po 215Po

203Bi 204Bi 205Bi 206Bi 207Bi 208Bi 209Bi 210Bi 211Bi 212Bi 213Bi 214Bi

202Pb 203Pb 204Pb 205Pb 206Pb 207Pb 208Pb 209Pb 210Pb 211Pb 212Pb 213Pb

201Tl 202Tl 203Tl 204Tl 205Tl 206Tl 207Tl 208Tl 209Tl 201Tl 201Tl 201Tl

N≦126

Enlargement

E. Teruya, et al., PRC93, 064327 (2016)

N≧126

Now in progress

N=126

2. Framework

introduction framework results summary

Shell model framework

13/ 20 0.065 1.698SPE i N

13/ 20 0.050 1.659SPE i N

9/ 2 7/ 2 13/ 2 3/ 2 5/ 2 1/ 20 , 1 , 0 , 2 , 1 , 2h f i p f p

N

number of valence particles

◆ neutrons and protons in the shell 82 – 126 and 126 –

◆ particle number dependence on orbitals

82 – 126 (6 orbitals):

126 – (7 orbitals) : 9/2 11/2 15/2 5/2 1/2 7/2 3/21 , 0 , 0 , 2 , 3 , 1 , 2g i j d s g d

/2

7/21 0.896 2N

SPE f

15/ 20 0.150 1.423SPE j N N

N

:proton particles

: neutron particles

: neutron holes

(in units of MeV)

5/ 21 f

3/ 22 p

1/ 22 p

7/ 21 f

9/ 20h

0.000

0.570

0.898

2.340

3.415

3.634

2.826

3.119

0.000

proton

126

13/ 20i

82

13/ 20SPE i

13/ 20SPE i

neutron

2.578

0.779

neutron

9/ 21g

11/ 20i

15/ 20 j5/ 22d

1/ 23s

7/ 21g3/ 22d

126

0.000

1.567

2.491

2.032

5/ 21 f

3/22p

1/22p

7/21 f

9/20h

13/20i

126

82

15/ 20SPE j

0.869

5/ 21 f

3/ 22 p

1/ 22 p

7/ 21 f

9/ 20h

0.000

0.570

0.898

2.340

3.415

3.634

2.826

3.119

0.000

126

13/ 20i

82

13/ 20SPE i

13/ 20SPE i

2.578

0.779

9/ 21g

11/ 20i

15/ 20 j5/ 22d

1/ 23s

7/ 21g3/ 22d

0.000

1.567

2.491

2.032

5/ 21 f

3/22p

1/22p

7/21 f

9/20h

13/20i

126

82

15/ 20SPE j

neutron proton

126

neutron

N<126

0.869

5/ 21 f

3/ 22 p

1/ 22 p

7/ 21 f

9/ 20h

0.000

0.570

0.898

2.340

3.415

3.634

2.826

3.119

0.000

126

13/ 20i

82

13/ 20SPE i

13/ 20SPE i

2.578

0.779

9/ 21g

11/ 20i

15/ 20 j5/ 22d

1/ 23s

7/ 21g3/ 22d

0.000

1.567

2.491

2.032

5/ 21 f

3/22p

1/22p

7/21 f

9/20h

13/20i

126

82

7/ 21SPE f

15/ 20SPE j

neutron proton

126

neutron

N>126

ˆ ˆ ˆ ˆH H H H

(2) (2)H Q Q

(N 126) 0.060,

Shell model framework

strengths 𝑮𝟎 𝑮𝟐 𝑮𝟒 𝑮𝟔 𝑮𝟖 𝑮𝟏𝟎

Protons 0.145 0.013 0.400 0.400 -0.60 0.00

Neutrons N<126 0.145 0.013 0.500 0.500 1.10 2.00

Neutrons N>126 0.102 0.008 0.400 0.300 0.00 0.450

(N 126) 0.080

9/2 7/2

,

† 0 0 † 2 2 †(L) (L)

0 2

, 4,6,8,10

8 † 8 8

9/2 7/2 9/2 7/2

j jm jm

jm

L

L

h f

H c c

G P P G P P G P P

G P h f P h f

9/2 7/2

8† 8 † †

9/2 7/2M h f MP h f c c

9/2 7/2

80.50,h fG

Shell model framework

Neutron system

Diagonalization

Results

Proton system

Neutron-Proton system

500 500

Energy cut-off

Diagonalization (Lanczos)

Diagonalization

Energy cut-off

1. Diagonalization of the neutron (proton) system [Complete diagonalization] energy sort

2. Energy cut-off (500~levels from them)

3. Diagonalization of the neutron-proton system [Lanczos method]

3. Results

introduction framework results summary

Pb isotope (even)

0 2 4 6 8 10 120

1

2

3

4

5

206Pb

(MeV

)E

expt. (positive)expt. (negative)calc. (positive)calc. (negative)

I0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

204Pb

I

(Me

V)

E

0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

210Pb

I

(MeV

)E

( )

( )

( )

( )

( )( )

( )( )

( )( )

( )

( )

( )

( )

( )

( )

0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

212Pb

I

(MeV

)E

( )( )( )

( )

( )

N≦

126

N>

126

204

82 122Pb 206

82 124Pb

expt. (positive)expt. (negative)calc. (positive)calc. (negative)

210

82 128Pb 212

82 130Pb

Pb isotope (even)

0 2 4 6 8 10 120

1

2

3

4

5

206Pb

(MeV

)E

expt. (positive)expt. (negative)calc. (positive)calc. (negative)

I0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

204Pb

I

(Me

V)

E

0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

210Pb

I

(MeV

)E

( )

( )

( )

( )

( )( )

( )( )

( )( )

( )

( )

( )

( )

( )

( )

0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

212Pb

I

(MeV

)E

( )( )( )

( )

( )

N≦

126

N>

126

204

82 122Pb 206

82 124Pb

expt. (positive)expt. (negative)calc. (positive)calc. (negative)

210

82 128Pb 212

82 130Pb

3- core

excitation

3- 3-

3-

Pb isotope (odd)

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 310

1

2

3

4

5

205Pb

2I

(Me

V)

E

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 310

1

2

3

4

5

203Pb

2I

(Me

V)

E

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 31

0

1

2

3

4

5

211Pb

2I

(MeV

)E

( )( )

( )

( )( )

( )

( )

( )

( )

( )

( )

( ) ( )

N≦

126

N>

126 Low-lying states

are excellently

reproduced

203

82 121Pb205

82 123Pb

211

82 129Pb

expt. (positive)expt. (negative)calc. (positive)calc. (negative)

At isotope (odd)

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 310

1

2

3

4

5

211At

2I

(MeV

)E

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 310

1

2

3

4

5

207At

2I

(MeV

)E

expt. (positive)expt. (negative)calc. (positive)calc. (negative)

N≦

126

N>

126

207

85 122At 211

85 126At

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 31

0

1

2

3

4

5

215At

2I

(MeV

)E

( )( )

( )( )( )( )

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 31

0

1

2

3

4

5

213At

2I

(MeV

)E

( )

( )

( )( )

215

85 130At213

85 128At

At isotope (doubly-odd)

0 2 4 6 8 10 12 14 160

1

2

3

4

5

210At

I

(MeV

)E

0 2 4 6 8 10 12 14 160

1

2

3

4

5

206At

I

(MeV

)E

expt. (positive)expt. (negative)calc. (positive)calc. (negative)

N≦

126

N>

126

0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

212At

I

(MeV

)E

( )( ) ( )

( ) ( )

( ) ( )( )

( )

( )( )

( )( )

( ) ( )( )( )

( ) ( ) ( )( )( )

206

85 121At210

85 125At

212

85 127At

0 2 4 6 8 10 12 14 16

0

1

2

3

4

5

214At

I

(MeV

)E

( )( ) ( ) ( ) ( ) ( )

( )

214

85 129At

E2 transition rates

210Po 𝐞𝐱𝐩𝐭. [W.u.] 𝐜𝐚𝐥𝐜. [W.u.]

2+→0+ 0.56(12) 4.123

4+→2+ 4.46(18) 4.453

6+→4+ 3.05(9) 3.028

8+→6+ 1.12(4) 1.055

10+→8+ 0.0002

212Rn 𝐞𝐱𝐩𝐭. [W.u.] 𝐜𝐚𝐥𝐜. [W.u.]

2+→0+ 6.237

4+→2+ 1.04(4) 0.688

6+→4+ 0.40(5) 0.373

8+→6+ 0.115(6) 0.144

10+→8+ 3.950

12+→10+ 4.4(2) 2.966

Effective charge

211At 𝐞𝐱𝐩𝐭. [W.u.] 𝐜𝐚𝐥𝐜. [W.u.]

13/2-→9/2- >0.039 4.264

3/2-→5/2- 12.8(14) 9.800

3/2-→7/2- 0.40(4) 0.619

15/2-→11/2- 1.7(3) 2.271

15/2-→13/2- 0.37(8) 0.598

21/2-→17/2- 2.66(10) 2.119

0.85e e

1.50e e

Magnetic and Quaqrupole moments

212Rn 𝐞𝐱𝐩𝐭. [μN] 𝐜𝐚𝐥𝐜. [μN]

2+ +1.714

4+ 4.0(2) +3.369

6+ 5.45(5) +5.058

8+ +7.15(2) +6.726

14+ 15.0(4) +13.207

17- 17.0(8) +16.205

208Bi 𝐞𝐱𝐩𝐭. [μN] 𝐜𝐚𝐥𝐜. [μN]

5+ +4.57(13) +3.819

10- 2.671(14) +2.379 210At 𝐞𝐱𝐩𝐭. [μN] 𝐜𝐚𝐥𝐜. [μN]

11+ +9.79(3) +8.832

19+ 13.26(13) +12.746

11- 15.675(17) +13.864

205Pb 𝐞𝐱𝐩𝐭. [eb] 𝐜𝐚𝐥𝐜 .[eb]

5/2- +0.226(37) +0.206

13/2+ 0.33(5) 0.304

Magnetic moments

Quadrupole moments

209Po 𝐞𝐱𝐩𝐭. [eb] 𝐜𝐚𝐥𝐜. [eb]

13/2- 0.126(5) -0.130

17/2- 0.659(7) -0.703

0.85 , 1.50e e e e

0.00, 1.00, 1.91, 2.79s sg g g g

Summary

◆ We have carried out the shell model calculation for nuclei around 208Pb.

◆ Energy levels and electromagnetic properties were calculated. ◆ We have obtained good agreements with the experimental data.

Target nuclei : Even-even, odd-mass, and doubly-odd nuclei for Pb, Bi, Po, At, Rn, and Fr isotopes

“Large-scale shell-model calculations of nuclei around mass 210”

E. Teruya, K. Higashiyama, N. Yoshinaga, Phys Rev C 93, 064327 (2016). N≦

126

◆ We will analyze nuclear structure in future.

Back up

Truncation

Shell model framework

208Rn : 4 neutron-holes and 4 proton-particles system

◆ Neutron system

Jπ=0+ : 113 states Jπ=4+ (M=4) : 560 states

◆ Proton system

Jπ=0+ : 113 states Jπ=4+ (M=4) : 560 states

Number of all positive parity states : 4985

Number of all positive parity states : 4985

◆ Neutron-Proton system (after cut-off)

Jπ=0+ : 21422 states Jπ=6+ : 174171 states

without cut-off Jπ=0+ : 1953785 states c.f.

Shell model framework

208Rn : 4 neutron-holes and 4 proton-particles system

0 200 400 600 800 1000

101

102

103

104

105

106

0 200 400 600 800 1000

0

1

2

3

4

5

6

7

[10+5

]

cut−off

0+

6+

208Rn

cut−off

0+

6+

0 200 400 600 800 10000

1

2

3

4

5

208Rn

cut−off

(MeV

)E

0+

2+

4+ 6

+8

+

10+

12+

/

Number of states in each cut-off for the neutron-proton system

Convergence of Energy

◆ Validity of the energy cut-off

the necessity of the interaction 9/2 7/2h fH

About the necessity of the interaction 9/2 7/2h fH

9/2 7/2 9/2 7/2

8 † 8 8

9/ 2 7/ 2 9/ 2 7/ 2h f h fH G P h f P h f

9/2 7/2

8† 8 † †

9/2 7/2M h f MP h f c c

0 2 4 6 8 10 12 14 160

1

2

3

4

5

210Po

I

(MeV

)E

0 2 4 6 8 10 12 14 160

1

2

3

4

5

210Po

I

(MeV

)E

without with

28

28

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 310

1

2

3

4

5

211At

2I

(MeV

)E

1 3 5 7 9 11 13 15 17 19 21 23 25 27 29 310

1

2

3

4

5

211At

2I

(MeV

)E

0 2 4 6 8 10 12 14 160

1

2

3

4

5

212Rn

I

(MeV

)E

0 2 4 6 8 10 12 14 160

1

2

3

4

5

210Rn

I

(MeV

)E

without

without

with

with

114

Neutron-proton interaction

A necessity of the hexadecapole

interaction

The neutron-proton interaction

208Bi : 1 neutron-hole and 1 proton-particle system

13/ 2 9/ 2i h configuration: 2 ,3 , ,11

states

0 2 4 6 8 10 12 14 160

1

2

3

4

5

208Bi

I

(Me

V)

E

□ QQ only ◇ QQ + hexadecapole

2 3 4 5 6 7 8 9 10 11 12

0

0.4

0.8

1.2

1.6

2

expt. SM

I

E(M

eV

)

208Bi12583 SM (multipole)

The neutron-proton interaction

□ QQ only

◇ QQ + hexadecapole

132Sb : 1 neutron-hole and 1 proton-particle system

11/ 2 7/ 2h g configuration

2 ,3 , ,9 states

2 3 4 5 6 7 8 9 10

0

0.4

0.8

1.2

1.6

2

expt. SM

I

E(M

eV

)

132Sb8151 SM (multipole)